Band 10, Heft 17 - Special Issue: Nonradiating photonics with resonant dielectric nanostructures

From theoretical model to experimental realization, the bound state in the continuum (BIC) is an emerging area of research interest in the last decade. In the initial years, well-established theoretical frameworks explained the underlying physics for optical BIC modes excited in various symmetrical configurations. Eventually, in the last couple of years, optical-BICs were exploited as a promising tool for experimental realization with advanced nanofabrication techniques for numerous breakthrough applications. Here, we present a review of the evolution of BIC modes in various symmetry and functioning mediums along with their application. More specifically, depending upon the nature of the interacting medium, the excitations of BIC modes are classified into the pure dielectric and lossy plasmonic BICs. The dielectric constituents are again classified as photonic crystal functioning in the subwavelength regime, influenced by the diffraction modes and metasurfaces for interactions far from the diffraction regime. More importantly, engineered functional materials evolved with the pure dielectric medium are explored for hybrid-quasi-BIC modes with huge-quality factors, exhibiting a promising approach to trigger the nanoscale phenomena more efficiently. Similarly, hybrid modes instigated by the photonic and plasmonic constituents can replace the high dissipative losses of metallic components, sustaining the high localization of field and high figure of merit. Further, the discussions are based on the applications of the localized BIC modes and high-quality quasi-BIC resonance traits in the nonlinear harmonic generation, refractometric sensing, imaging, lasing, nanocavities, low loss on-chip communication, and as a photodetector. The topology-controlled beam steering and, chiral sensing has also been briefly discussed.

Optically resonant dielectric and semiconductor metasurfaces are an emerging and promising area of nanophotonics and light–matter interaction at the nanoscale. Recently, active tuning of the linear response and nonlinear effects of these components has received an increasing amount of interest. However, so far these research directions have remained separated with only few sporadic works that study their combination beginning to appear in the literature. The evolution of nonlinear metasurfaces based on dielectric and semiconductor materials toward reconfigurable and dynamic components could potentially answer the demand of integrated on-chip components that realize essential functionalities such as frequency conversion, active switching, optical isolation, and all-optical routing. This review provides an overview of recent investigations in this field, reviews the main physical phenomena enabling the dynamic control of the nonlinear response and compares the temporal dynamics of the diverse approaches that have been explored so far. Finally, future directions of dynamic nonlinear metasurfaces are outlined.

Bound states in the continuum (BICs) emerge throughout physics as leaky/resonant modes that remain, however, highly localized. They have attracted much attention in photonics, and especially in metasurfaces. One of their most outstanding features is their divergent Q-factors, indeed arbitrarily large upon approaching the BIC condition (quasi-BICs). Here, we investigate how to tune quasi-BICs in magneto-optic (MO) all-dielectric metasurfaces. The impact of the applied magnetic field in the BIC parameter space is revealed for a metasurface consisting of lossless semiconductor spheres with MO response. Through our coupled electric/magnetic dipole formulation, the MO activity is found to manifest itself through the interference of the out-of-plane electric/magnetic dipole resonances with the (MO-induced) in-plane magnetic/electric dipole, leading to a rich, magnetically tuned quasi-BIC phenomenology, resembling the behavior of Brewster quasi-BICs for tilted vertical-dipole resonant metasurfaces. Such resemblance underlies our proposed design for a fast MO switch of a Brewster quasi-BIC by simply reversing the driving magnetic field. This MO-active BIC behavior is further confirmed in the optical regime for a realistic Bi:YIG nanodisk metasurface through numerical calculations. Our results present various mechanisms to magneto-optically manipulate BICs and quasi-BICs, which could be exploited throughout the electromagnetic spectrum with applications in lasing, filtering, and sensing.

Second harmonic generation through nonlinear nano-photonic structures is important in both classical and quantum applications. It is commonly expected that the second harmonic frequency can always be generated as long as appropriate quadratic nonlinearity is provided by the material and the phase-matching condition is satisfied. Here, we present an anomaly to this common wisdom by showing that second-harmonic dipoles generated in a nonlinear photonic crystal slab can be completely nonradiative. As a result, no energy is transferred from the fundamental frequency to the second harmonic even when the phase-matching condition is satisfied – a phenomenon we call “resonance-forbidden second-harmonic generation”. Through numerical simulation, we identify two mechanisms that can achieve this phenomenon: symmetry protection and parameter tuning. The finite-size effect and the topological origin of this phenomenon are also discussed.

Bound states in the continuum (BICs), i.e. highly-localized modes with energy embedded in the continuum of radiating waves, have provided in the past decade a new paradigm in optics and photonics, especially at the nanoscale, with a range of applications from nanophotonics to optical sensing and laser design. Here, we introduce the idea of a crystal made of BICs, in which an array of BICs is indirectly coupled via a common continuum of states resulting in a tight-binding dispersive energy miniband embedded in the spectrum of radiating waves. The results are illustrated for a chain of optical cavities side-coupled to a coupled-resonator optical waveguide with nonlocal contact points.

Dressed states forming when quantum emitters or atoms couple to a photonic bath underpin a number of phenomena and applications, in particular nonradiating effective interactions occurring within photonic bandgaps. Here, we present a compact formulation of the resolvent-based theory for calculating atom-photon dressed states built on the idea that the atom behaves as an effective impurity. This establishes an explicit connection with the standard impurity problem in condensed matter. Moreover, it allows us to formulate and settle – independently of the bath Hamiltonian – a number of properties previously known only for specific models or not entirely formalized. The framework is next extended to the case of more than one emitter, which is used to derive a general expression of dissipationless effective Hamiltonians explicitly featuring the overlap of single-emitter dressed bound states.

Optical resonances arising from quasi-bound states in the continuum (QBICs) have been recently identified in nanostructured dielectrics, showing ultrahigh quality factors accompanied by very large electromagnetic field enhancements. In this work, we design a periodic array of gallium phosphide (GaP) elliptical cylinders supporting, concurrently, three spectrally separated QBIC resonances with in-plane magnetic dipole, out-of-plane magnetic dipole, and electric quadrupole characters. We numerically explore this system for second-harmonic generation and degenerate four-wave mixing, demonstrating giant per unit cell conversion efficiencies of up to ∼ 2 W −1 and ∼ 60 W −2 , respectively, when considering realistic introduced asymmetries in the metasurface, compatible with current fabrication limitations. We find that this configuration outperforms by up to more than four orders of magnitude the response of low-Q Mie or anapole resonances in individual GaP nanoantennas with engineered nonlinear mode-matching conditions. Benefiting from the straight-oriented electric field of one of the examined high-Q resonances, we further propose a novel nanocavity design for enhanced spectroscopies by slotting the meta-atoms of the periodic array. We discover that the optical cavity sustains high-intensity fields homogeneously distributed inside the slot, delivering its best performance when the elliptical cylinders are cut from end to end forming a gap, which represents a convenient model for experimental investigations. When placing an electric point dipole inside the added aperture, we find that the metasurface offers ultrahigh radiative enhancements, exceeding the previously reported slotted dielectric nanodisk at the anapole excitation by more than two orders of magnitude.

Lithium niobate (LN), as a nonlinear material with a large nonlinear susceptibility, has been widely employed in second harmonic generation (SHG) up to ultraviolet (UV) frequency range due to its broad low-absorption window. In nanophotonics, it is possible to harness the Mie resonances associated with the single dielectric particles to boost the nonlinear light–matter interactions. Here, we fabricate single Mie-resonant LN nanospheres on a SiO 2 substrate via the femtosecond (fs) laser ablation technique. By exploiting the magnetic dipole (MD) Mie resonance, UV SHG from the LN nanosphere is significantly enhanced with a measured conversion efficiency of 4.45 × 10 −8 under the excitation of an fs laser at 750 nm. The single LN nanospheres achieved in this work could serve as Mie resonators for building nonlinear nanophotonic devices such as frequency converters and quantum light sources, etc.

Large-area and transparent all-dielectric metasurfaces sustaining photonic bound states in the continuum (BICs) provide a set of fundamental advantages for ultrasensitive biosensing. BICs bridge the gap of large effective mode volume with large experimental quality factor. Relying on the transduction mechanism of reactive sensing principle, herein, we first numerically study the potential of subwavelength confinement driven by topological decoupling from free space radiation for BIC-based biosensing. Then, we experimentally combine this capability with minimal and low-cost optical setup, applying the devised quasi-BIC resonator for PNA/DNA selective biosensing with real-time monitoring of the binding event. A sensitivity of 20 molecules per micron squared is achieved, i.e. ≃0.01 pg. Further enhancement can easily be envisaged, pointing out the possibility of single-molecule regime. This work aims at a precise and ultrasensitive approach for developing low-cost point-of-care tools suitable for routine disease prescreening analyses in laboratory, also adaptable to industrial production control.

Optical sensors typically provide compact, fast and precise means of performing quantitative measures for almost any kind of measurand that is usually probed electronically. High-contrast grating (HCG) resonators are known to manifest an extremely sharp and sensitive optical resonance and can constitute a highly suitable sensing platform. In this paper we present two advanced high-contrast grating designs improving the sensing performances of conventional implementations. These configurations, namely pedestal and half-buried HCGs, allow to enhance the shift of the photonic resonance while maintaining the spectral features of the standard configuration. First, the spectral feature of the HCGs was numerically optimized to express the sharpest possible resonance when the structure is immersed in serum. Second, the sensing properties of conventional and advanced HCG implementations were studied by modelling the biological entities to be sensed as a thin dielectric coating layer of increasing thickness. Pedestal HCGs were found to provide a ∼12% improvement in sensitivity and a six-fold improvement in resonance quality factor ( Q -factor), while buried HCGs resulted in a ∼58% improvement in sensitivity at the expense of a slightly broader resonance. Such structures may serve as an improved sensitive biosensing platform for near-infrared spectroscopy.

Based on the insights into the phenomenon of bound states in the continuum, a novel approach utilizing the momentum-space polarization morphologies of periodic structures to generate vortex beams (VBs) has been proposed. Such periodic structures modulate beams in a nonlocal way and require no precise alignment. However, the efficiency of such an approach has not been analyzed in detail, and the efficiency in previous realizations is far from optimized. Here, we analyze the factors affecting the efficiency of nonlocal VB generation. We show that the maximal efficiency cannot exceed 25% if the periodic structure carries only singlet resonances. To go beyond this limit, we propose two approaches to improve efficiency. We theoretically analyze the mechanisms and verify the approaches by full-wave simulations. Both of the approaches serve to improve the generation efficiency by several folds.

All-dielectric metasurfaces supporting photonic bound states in the continuum (BICs) are an exciting toolkit for achieving resonances with ultranarrow linewidths. However, the transition from theory to experimental realization can significantly reduce the optical performance of BIC-based nanophotonic systems, severely limiting their application potential. Here, we introduce a combined numerical/experimental methodology for predicting how unavoidable tolerances in nanofabrication such as random geometrical variations affect the performance of different BIC metasurface designs. We compare several established all-dielectric BIC unit cell geometries with broken in-plane inversion symmetry including tilted ellipses, asymmetric double rods, and split rings. Significantly, even for low fabrication-induced geometrical changes, both the BIC resonance amplitude and its quality factor (Q-factor) are significantly reduced. We find that the all-dielectric ellipses maintain the highest Q-factors throughout the geometrical variation range, whereas the rod and split ring geometries fall off more quickly. The same behavior is confirmed experimentally, where geometrical variation values are derived from automated processing of sets of scanning electron microscopy (SEM) images. Our methodology provides crucial insights into the performance degradation of BIC metasurfaces when moving from simulations to fabricated samples and will enable the development of robust, high-Q, and easy to manufacture nanophotonic platforms for applications ranging from biomolecular sensing to higher harmonic generation.

We study the effect of structural disorder on the transition from the bound states in the continuum (BICs) to quasi-BICs by the example of the periodic photonic structure composed of two layers of parallel dielectric rods. We uncover the specificity in the robustness of the symmetry-protected and accidental BICs against various types of structural disorder. We analyze how the spatial mode localization induced by the structural disorder results in an effective reduction of the system length and limits the Q factor of quasi-BICs. Our results are essential for the practical implementation of BICs especially in natural and self-assembled photonic structures, where the structural disorder plays a crucial role.

Lithium niobate integrated photonics has recently received significant attention because it exploits the attractive properties of lithium niobate on an integrated platform which provides strong optical confinement as well as high photonic integration density. Although many optical functionalities of lithium niobate have been demonstrated on a chip in the telecom band, the visible and near-visible regimes are less explored. This is mainly because devices with a relatively smaller feature size are required which increases fabrication difficulty. Here, we explored the acousto-optic effect of lithium niobate on a chip at near-visible wavelengths (765–781 nm) and demonstrated acousto-optic modulation with the modulation frequency up to 2.44 GHz. We adopted an etchless process for the device fabrication and applied the principle of bound states in the continuum to optimize the device performance. By demonstrating functionality at near-visible wavelengths, our devices will enable many on-chip applications ranging from frequency metrology to quantum information processing.

We propose and theoretically and numerically investigate integrated diffraction gratings for the Bloch surface wave (BSW) platform, which have subwavelength or near-subwavelength period. We demonstrate that, in the oblique incidence geometry of a transverse-electric polarized BSW and with a properly chosen band gap configuration of the photonic crystal supporting the surface waves, the proposed structures operate in the scattering-free regime, when the energy of the incident BSW is divided between the reflected and transmitted BSWs with the same polarization corresponding to the propagating diffraction orders of the grating, and not scattered away from the propagation surface. In this regime, the studied integrated gratings support high-Q resonances and bound states in the continuum not only in the subwavelength case when only the specular (zeroth) diffraction orders propagate, but also in the case when non-evanescent zeroth and −1st diffraction orders satisfy the so-called Littrow mounting condition. The proposed integrated gratings on the BSW platform can be used as efficient narrowband spatial or spectral filters operating in reflection, or as BSW beam splitters or deflectors operating in transmission. The obtained results may find application in two-dimensional photonic circuits for steering the BSW propagation.

Resonant modes of high contrast dielectric disk have finite Q -factors in the subwavelength range due to radiation leakage into the surrounding space. That leakage can be reduced considerably (a few times) by exploiting of the mechanism of destructive interference of two modes for avoided crossing of resonances (ACR) (Rybin et al. M. V. Rybin, K. L. Koshelev, Z. F. Sadrieva, et al., “High-Q Supercavity Modes in Subwavelength Dielectric Resonators,” Phys. Rev. Lett. , vol. 119, p. 243901, 2017.). In the present paper we report suppression of radiation leakage by a few orders in magnitude via the ACR in the structure of three and four different coaxial disks. For fine multi-scale tuning of disks we reveal the ultrahigh- Q resonances of order 10 5 for the case of three disks and of order 10 6 for the case of four coaxial disks of equal radii.

Bound states in the continuum (BIC) have been at the forefront of research in optics and photonics over the past decade. It is of great interest to study the effects associated with quasi-BICs in the simplest structures, where quasi-BICs are very pronounced. An example is a dielectric cylinder, and in a number of works, quasi-BICs have been studied both in single cylinders and in structures composed of cylinders. In this work, we studied the properties of quasi-BICs during the transition from a homogeneous dielectric cylinder in an air environment to a ring with narrow walls while increasing the diameter of the inner air cylinder gradually. The results demonstrate the quasi-BIC crossover from the strong-coupling to the weak-coupling regime, which manifests itself in the transition from the avoided crossing of branches to their intersection with the quasi-BIC being preserved on only one straight branch. In the regime of strong-coupling and quasi-BIC, three waves interfere in the far-field zone: two waves corresponding to the resonant modes of the structure and the wave scattered by the structure as a whole. The validity of the Fano resonance concept is discussed since it describes the interference of only two waves under weak coupling conditions.

We introduce two tractable analytical models to describe dynamic effects at resonant light scattering by subwavelength particles. One of them is based on a generalization of the temporal coupled-mode theory, and the other employs the normal mode approach. We show that sharp variations in the envelope of the incident pulse may initiate unusual, counterintuitive dynamics of the scattering associated with interference of modes with fast and slow relaxation. To exhibit the power of the models, we apply them to explain the dynamic light scattering of a square-envelope pulse by an infinite circular cylinder made of GaP, when the pulse carrier frequency lies in the vicinity of the destructive interference at the Fano resonances. We observe and explain intensive sharp spikes in scattering cross-sections just behind the leading and trailing edges of the incident pulse. The latter occurs when the incident pulse is over and is explained by the electromagnetic energy released in the particle at the previous scattering stages. The accuracy of the models is checked against their comparison with results of the direct numerical integration of the complete set of Maxwell’s equations and occurs very high. The models’ advantages and disadvantages are revealed, and the ways to apply them to other types of dynamic resonant scattering are discussed.

The phenomenon of anapole has attracted considerable attention in the field of metamaterials as a possible realization of radiationless objects. We comprehensively study this phenomenon in the cluster-based systems of dielectric particles by considering conditions of anapole manifestation in both single trimers of disk-shaped particles and metamaterial composed on such trimers. Our analytical approach is based on the multipole decomposition method and the secondary multipole decomposition technique. They allow us to associate the anapole with the multipole moments of the trimer and the separate multipole moments of its constitutive particles. The manifestation of anapole in a two-dimensional metamaterial (metasurface) is confirmed by checking the resonant states in the reflected field as well as from the electromagnetic near-field patterns obtained from the full-wave numerical simulation. It is demonstrated that the anapole excitation in trimers results in the polarization-independent suppression of reflection with the resonant enhancement of local electromagnetic fields in the metasurface. Finally, experimental verification of the theoretical results is presented and discussed.

All-dielectric nanophotonics has become one of the most active fields of research in modern optics, largely due to the opportunities offered by the simultaneous resonant control of electric and magnetic components of light at the nanoscale. In this rapidly evolving scenario, the possibility to design artificial Huygens sources by overlapping electric and magnetic resonances has established a new paradigm in flat optics, bringing devices closer to efficient wavefront shaping with direct phase engineering at the level of the individual meta-atoms. However, their efficiency is fundamentally limited by the near-field coupling between the constituents of the metalattice. In this work, we challenge this well-conceived notion and propose an alternative concept to achieve phase control and full transmission in metasurfaces, based on the unusual properties of the nonradiating sources known as hybrid anapoles (HAs). We analyze theoretically an array of such sources and demonstrate that HAs are characterized by negligible coupling with their neighbors. Therefore, in contrast to Huygens particles, the proposed sources can operate as individual meta-atoms even in highly compact designs, becoming robust against strong disorder and preserving its characteristics when deposited on dielectric substrates. Remarkably, the phase of the transmitted wave can be modulated with negligible reflection. To illustrate the capabilities of our platform, we also utilize a disordered HA array to implement a controlled phase modulation to an ultrafast Gaussian pulse. The results of our study represent a departure from the currently established designs and open an avenue toward the realization of new devices for flat optics with unprecedented efficiency.

Nonradiating sources of energy realized under a wave scattering on high-index dielectric nanoparticles have attracted a lot of attention in nano-optics and nanophotonics. They do not emit energy to the far-field, but simultaneously provides strong near-field energy confinement. Near-field wireless power transfer technologies suffer from low efficiency and short operation distance. The key factor to improve efficiency is to reduce the radiation loss of the resonators included in the transmitter and receiver. In this paper, we develop a wireless power transfer system based on nonradiating sources implemented using colossal permittivity dielectric disk resonator and a subwavelength metal loop. We demonstrate that this nonradiating nature is due to the hybrid anapole state originated by destructive interference of the fields generated by multipole moments of different parts of the nonradiating source, without a contribution of toroidal moments. We experimentally investigate a wireless power transfer system prototype and demonstrate that higher efficiency can be achieved when operating on the nonradiating hybrid anapole state compared to the systems operating on magnetic dipole and magnetic quadrupole modes due to the radiation loss suppression.

Radio frequency identification (RFID) is a widely used wireless technology for contactless data exchange. Owing to international standardization and one-way security nature of the communication protocol, RFID tags, holding sensitive information, may be a subject to theft. One of the major security loopholes is the so-called far-field attack, where unauthorized interrogation is performed from a distance, bypassing the user’s verification. This loophole is a penalty of using a dipole-like RFID tag antenna, leaking wireless information to the far-field. Here we introduce a new concept of anapole-enabled security, prohibiting far-field attacks by utilizing fundamental laws of physics. Our design is based on radiationless electromagnetic states (anapoles), which have high near-field concentration and theoretically nulling far-field scattering. The first property enables performing data readout from several centimeters (near-field), while the second prevents attacks from a distance, regardless an eavesdropper’s radiated power and antenna gain. Our realization is based on a compact 3 cm high-index ceramic core–shell structure, functionalized with a thin metal wire and an integrated circuit to control the tag. Switching scheme was designed to provide a modulation between two radiation-less anapole states, blocking both up and down links for a far-field access. The anapole tag demonstrates more than 20 dB suppression of far-field interrogation distance in respect with a standard commercial tag, while keeping the near-field performance at the same level. The proposed concept might significantly enhance the RFID communication channel in cases, where information security prevails over cost constrains.