Band 11, Heft 1

Optical imaging systems, like microscopes, cameras, and telescopes, continue to expand the scope of human observation of the world. As one of the key indicators of imaging systems, the field-of-view (FOV) is often limited by coma aberration. Expanding it generally relies on a combination of complex lenses, leading to a bulky and cumbersome system. Recently, the emergency of meta-optics provides an alternative to constructing compact and lightweight large-FOV metalens through elaborated phase modulation within a flat surface, showing great potential in surveillance, unmanned vehicles, onboard planes or satellites, medical science, and other new applications. In this article, we review recent advances of wide-angle metalenses, including operation principles, design strategies, and application demos. Firstly, basic principles of wide-angle imaging using a single metalens are interpreted. Secondly, some advanced methods for designing subwavelength structures with high angle robustness and high efficiency are discussed. Thirdly, some representative functional devices and applications are surveyed. Finally, we conclude with an outlook on future potentials and challenges that need to be overcome.

The generalized Snell’s law dictates that introducing a phase gradient at the interface of two media can shape incident light and achieve anomalous reflection or refraction. However, when the introduced phase gradient is realized via the scattering of nanoparticles in the metasurfaces, this law needs to be modified; certain conditions need to be met when the law is established. We present the conditions for establishing the “generalized Snell’s law of refraction” in all-dielectric metasurfaces under the incidence of different polarized light. These conditions can provide theoretical bases for the subsequent design of high-efficiency beam deflection metasurfaces. The relationship between the highest achievable anomalous refraction efficiency and the number of nanoparticles within one period of the metasurface is also summarized. In addition, the generalized refraction should not depend on the polarization states of incident light; however, the previous realization conditions of anomalous refraction were sensitive to the polarization states. Thus, conditions for establishing the polarization-independent generalized Snell’s law of refraction in all-dielectric metasurfaces are presented.

Regulation of hot spots exhibits excellent potential in many applications including nanolasers, energy harvesting, sensing, and subwavelength imaging. Here, hat-shaped hierarchical nanostructures with different space curvatures have been proposed to enhance hot spots for facilitating surface-enhanced Raman scattering (SERS) and plasmon-driven catalysis applications. These novel nanostructures comprise two layers of metal nanoparticles separated by hat-shaped MoS 2 films. The fabrication of this hybrid structure is based on the thermal annealing and thermal evaporation of self-assembled polystyrene spheres, which are convenient to control the metal particle size and the curvature of hat-shaped nanostructures. Based on the narrow gaps produced by the MoS 2 films and the curvature of space, the constructed platform exhibits superior SERS capability and achieves ultrasensitive detection for toxic molecules. Furthermore, the surface catalytic conversion of p-nitrothiophenol (PNTP) to p, p′-dimercaptobenzene (DMAB) was in situ monitored by the SERS substrate. The mechanism governing this regulation of hot spots is also investigated via theoretical simulations.

Bound states in the continuum (BICs) are observed in optical cavities composed of a high refractive index periodic structure embedded in significantly lower refractive index surroundings, enabling vertical confinement of the grating modes. Here, we propose a vertically nonsymmetric configuration, implemented on a high refractive index bulk substrate with a one-dimensional grating positioned on a distributed Bragg reflector (DBR). In this configuration, the grating modes are leaky, which could prohibit the creation of a BIC if the grating was implemented on uniform substrate. However, the judiciously designed DBR on which the grating is implemented reflects nonzero diffraction orders induced by the grating. We found that the laterally antisymmetric optical modes located at the center of the Brillouin zone of this structure create BICs that are robust against changes in the grating parameters, as long as the DBR reflects the diffraction orders. The configuration enables a high degree of design freedom, facilitating the realization of very high quality factor cavities in conventional all-semiconductor technology.

Single-molecule localization microscopy (SMLM) plays an irreplaceable role in biological studies, in which nanometer-sized biomolecules are hardly to be resolved due to diffraction limit unless being stochastically activated and accurately located by SMLM. For biological samples preimmobilized for SMLM, most biomolecules are cross-linked and constrained at their immobilizing sites but still expected to undergo confined stochastic motion in regard to their nanometer sizes. However, few lines of direct evidence have been reported about the detectability and influence of confined biomolecule stochastic motion on localization precision in SMLM. Here, we access the potential stochastic motion for each immobilized single biomolecule by calculating the displacements between any two of its localizations at different frames during sequential imaging of Alexa Fluor-647-conjugated oligonucleotides. For most molecules, localization displacements are remarkably larger at random frame intervals than at shortest intervals even after sample drift correction, increase with interval times and then saturate, showing that biomolecule stochastic motion is detected and confined around the immobilizing sizes in SMLM. Moreover, localization precision is inversely proportional to confined biomolecule stochastic motion, whereas it can be deteriorated or improved by enlarging the biomolecules or adding a post-crosslinking step, respectively. Consistently, post-crosslinking of cell samples sparsely stained for tubulin proteins results in a better localization precision. Overall, this study reveals that confined stochastic motion of immobilized biomolecules worsens localization precision in SMLM, and improved localization precision can be achieved via restricting such a motion.

The polarizations of optical fields, besides field intensities, provide more degrees of freedom to manipulate coherent light–matter interactions. Here, we propose how to achieve a coherent switch of optomechanical entanglement in a polarized-light-driven cavity system. We show that by tuning the polarizations of the driving field, the effective optomechanical coupling can be well controlled and, as a result, quantum entanglement between the mechanical oscillator and the optical transverse electric mode can be coherently and reversibly switched to that between the same phonon mode and the optical transverse magnetic mode. This ability to switch optomechanical entanglement with such a vectorial device can be important for building a quantum network being capable of efficient quantum information interchanges between processing nodes and flying photons.

A pulling motion of supercavitating plasmonic nanoparticle (NP) by a single plane wave has received attention for the fundamental physics and potential applications in various fields ( e.g. , bio-applications, nanofabrication, and nanorobotics). Here, the supercavitating NP depicts a state where a nanobubble encapsulates the NP, which can be formed via the photo-thermal heating process in a liquid. In this letter, we theoretically study the optical force on a supercavitating titanium nitride (TiN) NP by a single plane wave at near-infrared wavelengths to explore optical conditions that can potentially initiate the backward motion of the NP against the wave-propagating direction. An analysis with vector spherical harmonics is used to quantify the optical force on the NP efficiently. Next, the vector field line of the optical force is introduced to visualize the light-driven motion of the NP in a nanobubble. Finally, we characterize the vector field lines at various optical conditions ( e.g. , various sizes of NP and nanobubble, and wavelength), and we find a suitable window of the optical state which can potentially activate the backward motion of the supercavitating TiN NP.

Tapered fiber (TF) and D-shaped fiber (DF) are two types of widely investigated devices in facilitating evanescent-field interactions with external materials. Although they have been found to be particularly useful in various ultrafast regimes, to date there is still no clear or systematic investigation on their local nonlinearities as well as the exerted influences on ultrafast behaviors. Herein, we present such thorough investigation through local nonlinearity engineering on TF and then in contrast with a DF as a reference. Optically deposited black phosphorus quantum dots (BPQDs) are used for saturable absorption. The nanometer-scale extremely small sizes of the BPQDs helpfully eliminate size-induced uncertainties or distortions during both device fabrication and the latter light–matter interaction. For the TF, in the experiment, it is found that the local nonlinear effect starts to be rather appreciable as the TF shrinks to a moderate thickness. Remarkably in comparison, the local nonlinearity of the DF itself can even be neglected reasonably, but after coating with BPQDs, it possesses a much larger modulation depth than any of the used BPQDs-coated TFs with different thicknesses/lengths. Further, we theoretically analyze the related locally nonlinear effects and reveal, for the first time, the direct origin of saturable absorption with evanescent-field-based general structures.

Lung cancer is the most frequently life-threatening disease and the prominent cause of cancer-related mortality among human beings worldwide, where poor early diagnosis and expensive detection costs are considered as significant reasons. Here, we try to tackle this issue by proposing a novel label-free and low-cost strategy for rapid detection and distinction of lung cancer cells relying on plasmonic toroidal metasurfaces at terahertz frequencies. Three disjoint regions are displayed in identifiable intensity-frequency diagram, which could directly help doctors determine the type of lung cancer cells for clinical treatment. The metasurface is generated by two mirrored gold split ring resonators with subwavelength sizes. When placing analytes on the metasurface, apparent shifts of both the resonance frequency and the resonance depth can be observed in the terahertz transmission spectra. The theoretical sensitivity of the biosensor over the reflective index reaches as high as 485.3 GHz/RIU. Moreover, the proposed metasurface shows high angular stability for oblique incident angle from 0 to 30°, where the maximum resonance frequency shift is less than 0.66% and the maximum transmittance variation keeps below 1.33%. To experimentally verify the sensing strategy, three types of non-small cell lung cancer cells (Calu-1, A427, and 95D) are cultured with different concentrations and their terahertz transmission spectra are measured with the proposed metasurface biosensor. The two-dimensional fingerprint diagram considering both the frequency and transmittance variations of the toroidal resonance dip is obtained, where the curves for different cells are completely separated with each other. This implies that we can directly distinguish the type of the analyte cells and its concentration by only single spectral measurement. We envisage that the proposed strategy has potential for clinical diagnosis and significantly expands the capabilities of plasmonic metamaterials in biological detection.

In a wide range of applications such as healthcare treatment, environmental monitoring, food processing and storage, and semiconductor chip manufacturing, relative humidity (RH) sensing is required. However, traditional fiber-optic humidity sensors face the challenges of miniaturization and indirectly obtaining humidity values. Here, we propose and demonstrate an optical barcode technique by cooperating with RH meta-tip, which can predict the humidity values directly. Such RH meta-tip is composed of fiber-optic sensor based on surface plasmon resonance (SPR) effect and graphene oxide film as humidity sensitizer. While SPR sensor is composed of multimode fiber (MMF) integrated with metallic metasurface. Dynamic time warping (DTW) algorithm is used to obtain the warp path distance (WPD) sequence between the measured reflection spectrum and the spectra of the precalibrated database. The distance sequence is transformed into a pseudo-color barcode, and the humidity value is corresponded to the lowest distance, which can be read by human eyes. The RH measurement depends on the collective changes of the reflection spectrum rather than tracking a single specific resonance peak/dip. This work can open up new doors to the development of a humidity sensor with direct RH recognition by human eyes.

We demonstrate a novel all-dielectric magnetophotonic structure that consists of two-dimensional arrays of bismuth substituted iron-garnet nanocylinders supporting both localized (Fabry–Perot-like) and lattice (guided-like) optical modes. Simultaneous excitation of the two kinds of modes provides a significant enhancement of the Faraday effect by 3 times and transverse magneto-optical Kerr effect by an order of magnitude compared to the smooth magnetic film of the same effective thickness. Both magneto-optical effects are boosted in wide spectral and angular ranges making the nanocylinder array magnetic dielectric structures promising for applications with short and tightly focused laser pulses.

Recently, in addition to exploring the application of new saturable absorber devices in fiber lasers, soliton dynamics has also become a focus of current research. In this article, we report an ultrashort pulse fiber laser based on VSe 2 /GO nanocomposite and verify the formation process of soliton and soliton molecules by the numerical simulation. The prepared VSe 2 /GO-based device shows excellent saturable absorption characteristics with a modulation depth of 14.3% and a saturation absorption intensity of 0.93 MW/cm 2 . The conventional soliton is obtained with pulse width of 573 fs, which is currently the narrowest pulse width based on VSe 2 -related material, and has a signal-to-noise ratio of 60.4 dB. In addition, the soliton molecules are realized based on the VSe 2 /GO for the first time and have a pulse interval of ∼2.2 ps. We study the soliton dynamics through numerical simulation and reveal that before the formation of the soliton, it undergoes multiple nonlinear stages, such as soliton mode-locking, soliton splitting, and soliton oscillation. Furthermore, the results of numerical simulation are agreed well with the experimental data. These results indicate that the VSe 2 /GO might be another promising saturable absorber material for ultrafast photonics, and deepen the understanding of soliton dynamics in ultrafast fiber lasers.

Graphitic carbon nitride (g-C 3 N 4 ) featuring a stable heptazine ring structure and high polymerization degree, was indexed as a high thermochemical stability material, attracting rising research enthusiasm for diverse applications. However, the poor near-infrared (NIR) optical absorption and resulting limited NIR applications were pronounced for g-C 3 N 4 due to its large bandgap of 2.7 eV. In the present work, sulfur-doping was manifested by first-principles calculations to introduce impurity level and result in anisotropic spin splitting in g-C 3 N 4 for enhancing broadband nonlinear optical characteristics in NIR regime. The modified sulfur-doped g-C 3 N 4 (S-C 3 N 4 ) exhibited the maximum effective nonlinear absorption coefficient to be −0.82 cm/GW. Pulse duration within hundred nanoseconds was realized with high modulation stability employing S-C 3 N 4 as saturable absorber in Q-switching operations. Moreover, broadband ultrafast photonics properties were successfully demonstrated in constructed ytterbium-doped and erbium-doped fiber lasers, generating highly stable dissipative soliton and traditional soliton mode-locking pulses. The presented S-C 3 N 4 nanomaterial with remarkable nonlinear optical performances might explicitly boost the development and application of g-C 3 N 4 materials in advanced optoelectronic and ultrafast photonic devices.

First- and second-order topological phases, capable of inherent protection against disorder of materials, have been recently experimentally demonstrated in various artificial materials through observing the topologically protected edge states. Topological phase transition represents a new class of quantum critical phenomena, which is accompanied by the changes related to the bulk topology of energy band structures instead of symmetry. However, it is still a challenge to directly observe the topological phase transitions defined in terms of bulk states. Here, we theoretically and experimentally demonstrate the direct observation of multifarious topological phase transitions with real-space indicator in a single photonic chip, which is formed by integration of 324 × 33 waveguides supporting both first- and second-order topological phases. The trivial-to-first-order, trivial-to-second-order and first-to-second-order topological phase transitions signified by the band gap closure can all be directly detected via photon evolution in the bulk. We further observe the creation and destruction of gapped topological edge states associated with these topological phase transitions. The bulk-state-based route to investigate the high-dimensional and high-order topological features, together with the platform of freely engineering topological materials by three-dimensional laser direct writing in a single photonic chip, opens up a new avenue to explore the mechanisms and applications of artificial devices.

We ask the question “what happens to Bloch waves in gratings synthetically moving at near the speed of light?”. First we define a constant refractive index (CRI) model in which Bloch waves remain well defined as they break the light barrier, then show their dispersion rotating through 360° from negative to positive and back again. Next we introduce the effective medium approximation (EMA) then refine it into a 4-wave model which proves to be highly accurate. Finally using the Bloch waves to expand a pulse of light we demonstrate sudden inflation of pulse amplitude combined with reversal of propagation direction as a luminal grating is turned on.