Band 11, Heft 19

Novel 2D van der Waals semiconductors facilitate the formation of heterostructures and thus support bandgap engineering for atomically thin modern photonic applications. When these heterostructures form a type II band structure, interlayer excitons (ILEs) are formed as a result of the ultrafast charge transfer between the layers. Here, we present for the first time a waveguide-coupled, mid-IR photodetector and modulator based on the ILE absorption. The device consists of a heterostructure of a single layer of tungsten disulfide (WS 2 ) and a few layers of hafnium disulfide (HfS 2 ) integrated to a silicon waveguide on a sapphire substrate. We measure broadband mid-IR photodetection (3.8–5.5 µm) with responsivity in the order of tens of µA/W and with no significant effect on the waveguide’s transmission. Additionally, we demonstrate waveguide-integrated, mid-IR, all-optical modulation by controlling the ILE population with the interband transition of the individual layers of the heterostructure.

Photonic and phononic topological insulators (TIs) offer numerous opportunities for manipulating light and sound with high efficiency and resiliency. On the other hand, inverse design methodologies, such as gradient-based approaches, evolutionary approaches, and deep-learning methods, provide a cost-effective strategy for developing photonic and phononic structures with unique features in steering light and sound. Here, we discuss recent advances and achievements in the development of photonic and phononic TIs employing inverse design methodologies, including one-dimensional TIs, TIs based on the quantum spin Hall effect (QSHE) and quantum valley Hall effect (QVHE), and high-order TIs in lattices with diverse symmetries. Several inversely designed photonic and phononic TIs with superior performance are exhibited. In addition, we offer our perspectives on the future of this emerging study field.

The control of the interaction between quantum emitters using nanophotonic structures holds great promise for quantum technology applications, while its theoretical description for complex nanostructures is a highly demanding task as the electromagnetic (EM) modes form a high-dimensional continuum. We here introduce an approach that permits a quantized description of the full EM field through a small number of discrete modes. This extends the previous work in ref. (I. Medina, F. J. García-Vidal, A. I. Fernández-Domínguez, and J. Feist, “Few-mode field quantization of arbitrary electromagnetic spectral densities,” Phys. Rev. Lett. , vol. 126, p. 093601, 2021) to the case of an arbitrary number of emitters, without any restrictions on the emitter level structure or dipole operators. The low computational demand of this method makes it suitable for studying dynamics for a wide range of parameters. We illustrate the power of our approach for a system of three emitters placed within a hybrid metallodielectric photonic structure and show that excitation transfer is highly sensitive to the properties of the hybrid photonic–plasmonic modes.

We demonstrate the formation of the near field with non-trivial phase distribution using surface plasmon interference devices, and experimental quantitative imaging of that phase with near-field phase microscopy. The phase distribution formed with a single device can be controlled by the polarization of the external illumination and the area of the device assigned to the object wave. A comparison of the experimental data to a numerical electromagnetic model and an analytical model assigns the origin of the near-field phase to the out-of-plane electric component of surface plasmon polaritons, and also verifies the predictive power of the models. We demonstrate a formation of near-field plane waves with different propagation directions on a single device, or even simultaneously at distinct areas of a single device. Our findings open the way to the imaging and tomography of phase objects in the near field.

We investigate the generation of entanglement between two quantum emitters through the inverse-design engineering of their photonic environment. By means of a topology-optimization approach acting at the level of the electromagnetic Dyadic Green’s function, we generate dielectric cloaks operating at different inter-emitter distances and incoherent pumping strengths. We show that the structures obtained maximize the dissipative coupling between the emitters under extremely different Purcell factor conditions, and yield steady-state concurrence values much larger than those attainable in free space. Finally, we benchmark our design strategy by proving that the entanglement enabled by our devices approaches the limit of maximum-entangled-mixed-states.

We report for the first time the direct growth of molybdenum disulfide (MoS 2 ) monolayers on nanostructured silicon-on-insulator waveguides. Our results indicate the possibility of utilizing the Chemical Vapour Deposition (CVD) on nanostructured photonic devices in a scalable process. Direct growth of 2D material on nanostructures rectifies many drawbacks of the transfer-based approaches. We show that the van der Waals material grow conformally across the curves, edges, and the silicon–SiO 2 interface of the waveguide structure. Here, the waveguide structure used as a growth substrate is complex not just in terms of its geometry but also due to the two materials (Si and SiO 2 ) involved. A transfer-free method like this yields a novel approach for functionalizing nanostructured, integrated optical architectures with an optically active direct semiconductor.

Intrinsic structural phase is a crucial foundation for the fundamental physical properties, and for creating innovative devices with unprecedented performances and unique functionalities. Long-range ferromagnetic orders of van der Waals CrI 3 are strongly tied with interlayer stacking orders. However, the intrinsic structure of few-layer CrI 3 still remains elusive; the predicted monoclinic phase has not yet been experimentally detected in bare few-layer CrI 3 . Here we uncover the intrinsic structure of few-layer CrI 3 with interlayer antiferromagnetic coupling, which unambiguously show monoclinic stacking in both bare and hBN-encapsulated bilayer and tri-five-layer CrI 3 throughout an entire temperature range from 300 to 10 K. An exotic spring damping effect from hBN encapsulation layers is experimentally observed in hBN/CrI 3 /hBN heterostructures, which partly hinders interlayer sliding of CrI 3 . This work demonstrates the intrinsic monoclinic crystal phase of few-layer CrI 3 and associated correlation with magnetic orders, opening up numerous opportunities for creating magnetic texture by stacking design.

CRISPR-Cas systems (clustered regularly interspaced short palindromic repeats) have shown great potential as efficient gene editing tools in disease therapeutics. Although numerous CRISPR-Cas systems have been developed, detailed mechanisms of target recognition and DNA cleavage are still unclear. In this work, we dynamically observe the entire process of conjugation, target recognition and DNA cleavage by single particle spectroscopy of CRISPR-Cas systems on single particle surfaces (gold) with the unique advantage of extended time periods. We show the CRISPR-Cas system, comprised of Cas endonuclease and single guide RNA, is stable and functional on single particle surfaces. Owing to the photostability of single particle surfaces, we directly observe in real time the entire dynamic process of conjugation, target recognition and DNA cleavage without photobleaching. We find heterogeneity in target recognition and DNA cleavage processes in which individual spectra vary significantly from one another as well as from the ensemble. We believe an in depth understanding of heterogeneities in CRISPR-Cas systems can overcome potential barriers in precision medicine and personalized disease therapeutics.

Optical resonators are structures that utilize wave interference and feedback to confine light in all three dimensions. Depending on the feedback mechanism, resonators can support either standing- or traveling-wave modes. Over the years, the distinction between these two different types of modes has become so prevalent that nowadays it is one of the main characteristics for classifying optical resonators. Here, we show that an intermediate link between these two rather different groups exists. In particular, we introduce a new class of photonic resonators that supports a hybrid optical mode, i.e. at one location along the resonator the electromagnetic fields associated with the mode feature a purely standing-wave pattern, while at a different location, the fields of the same mode represent a pure traveling wave. The proposed concept is general and can be implemented using chip-scale photonics as well as free-space optics. Moreover, it can be extended to other wave phenomena such as microwaves and acoustics.

Although hot-carrier-based photodetection using plasmonic effects has been widely investigated, photodetectors of this type with an external quantum efficiency (EQE) > 1 % ${ >}1\%$ and an active area of < 1 ${< }1$ mm 2 remain out of reach even in the visible frequencies. In this work, a novel hot-electron-based, non-trench-type photodetector exploiting pure photoexcitation in a thin aluminum (Al) film and leaky plasmonic modes at and between its heterojunctions is proposed, analyzed, and experimentally demonstrated. Combining diffracted-order-resolved analytical analysis and numerical computations unravels the optical absorption mechanism of the innovative design. Leaky surface plasmon resonance (with leakage radiation into the air) produced by a propagating diffracted order and quasibound supermodes (with power leakage via coupled gap plasmon polariton and bound surface plasmon polariton modes) excited by evanescent diffracted orders are shown to significantly contribute to the absorptance in the preferred thin Al film where hot electrons are generated. At 638.9 nm and electric bias −0.9951 V, the measured per-unit-area responsivity, detectivity, and the external quantum efficiency reach 298.1444 μA/mW/mm 2 , 4.3809 × 10 9 cm Hz 1/2 /W, and 2.6878%, respectively, from an active area of 4.6457 × 10 −2 mm 2 . The performance is among the best of those previously reported operating at similar wavelengths and biases. The RC time constant is estimated to be about 1.673 μs from the current-voltage measurements. The physical insight into the innovative, experimentally demonstrated device could lay the groundwork for the practical use of low-voltage, metal-based photodetection.

Planar optical elements have attracted widespread attentions because of their precise light modulation. Liquid crystals (LCs) are well known for their applications in the current displaying field, and show great potential in planar optical elements with the development and innovation of LC micro-operation technology. However, previous researches on LC elements mainly involved only one type of optical manipulation, which inevitably limited the functional diversity. In this work, we propose a multifunctional LC element which integrates the surface display into a binary-phase focusing lens by controlling the complex amplitude of the incident light. The light modulation of the anisotropic LC molecule satisfies a sinusoidal variation, which can be regarded as the combination of a continuous amplitude modulation and a binary phase modulation. The element with millimeter size is then fabricated, and the experimental measurements agree well with our design with a high-definition surface pattern and high-quality optical focusing/imaging performance. Furthermore, as the complex amplitude modulation changes from sine to cosine function after rotating the sample by 45°, a bifocal lens with two different focal lengths is also demonstrated. We expect the proposed multifunctional LC elements can find applications in information multiplexing, image displaying, etc.