Abstract
The flow in a downward divergent channel turns out to be an interesting experimental setup for the observation of upward floating bubbles that appear to be levitating in view of the observer. A more detailed analysis of this flow and its characteristic parameters is necessary for better understanding of this phenomenon. The boundary layer theory was used to derive the velocity field for the experimental setup. The actual flow of a liquid in the presence of a bubble was studied experimentally by measuring the position of the bubble; the data were then statistically processed by an image analysis. Observation of the bubble positions distribution showed that it is reasonable to assume a flat velocity profile of the liquid in the channel and that the bubbles do not tend to move into the boundary layer. In our experiments, volume of the air bubbles floating in water was 200 mm3 and of that of bubbles floating in aqueous glycerin was 300 mm3. Thus, the experiment used in this work is suitable for reliable determination of instantaneous and average bubble rising velocities as well as of those of horizontal and vertical oscillations.
Acknowledgements
The authors especially thank Jarda J. Ulbrecht for carefully reading and appropriate language corrections of the manuscript. This research was financially supported by grant no. 104/07/1110 from the Grant Agency of the Czech Republic and the project ICT-National Feasibility Study (No. LO1406).
Symbols
| az | acceleration of the bubble in the upward direction | m s−2 |
| cp | specific heat capacity | J kg−1 K−1 |
| D | local diameter of diverging tube | m |
| d | equivalent bubble diameter | m |
| Eo | Eötvös number | |
| Mo | Morton number | |
| N | number of counts | |
| Re | Reynolds number | |
| r | radius of divergent tube | m |
| t | time | s |
| U | liquid velocity outside the boundary m s−1 | layer |
| u(z, r) | liquid velocity as a function of vertical and radial position | m s−1 |
| uB | rise velocity of the bubble | m s−1 |
| V | volumetric flow rate | m3 s−1 |
| VB | bubble volume | mm3 |
| We | Weber number | |
| Z | distance from the leading edge of the tube | m |
| z | vertical position | m |
| α | angle of bubble inclination | rad |
| δ∗ | boundary layer displacement thickness | m |
| δ1% | boundary layer thickness | m |
| μ | liquid viscosity | Pa s |
| ρ | liquid density | kg m−3 |
| σ | surface tension | mN m−1 |
References
Alves, S. S., Orvalho, S. P., & Vasconcelos, J. M. T. (2005). Effect of bubble contamination on rise velocity and mass transfer. Chemical Engineering Science, 60, 1–9. DOI: 10.1016/j.ces.2004.07.053.10.1016/j.ces.2004.07.053Suche in Google Scholar
Badam, V. K., Buwa, V., & Durst, F. (2007). Experimental investigations of regimes of bubble formation on submerged orifices under constant flow condition. The Canadian Journal of Chemical Engineering, 85, 257–267. DOI: 10.1002/cjce.5450850301.10.1002/cjce.5450850301Suche in Google Scholar
Bardina, J., Lyrio, A., Kline, S. J., Ferziger, J. H., & Johnston, J. P. (1981). A prediction method for planar diffuser flows. Journal of Fluids Engineering, 103, 315–321. DOI: 10.1115/1.3241739.10.1115/1.3241739Suche in Google Scholar
Bordas, M. L., Cartellier, A., Sechet, P., & Boyer, C. (2006). Bubbly flow through fixed beds: Microscale experiments in the dilute regime and modeling. AICHE Journal, 52, 3722– 3743. DOI: 10.1002/aic.10980.10.1002/aic.10980Suche in Google Scholar
Fox, R. W., & Kline, S. J. (1962). Flow regimes in curved sub-sonic diffusers. Journal of Basic Engineering, 84, 303–312. DOI: 10.1115/1.3657307.10.1115/1.3657307Suche in Google Scholar
Kline, S. J., Bardina, J. G., & Strawn, R. C. (1983). Correlation of the detachment of two-dimensional turbulent boundary layers. AIAA Journal, 21, 68–73. DOI: 10.2514/3.8029.10.2514/3.8029Suche in Google Scholar
Kulkarni, A. A., & Joshi, J. B. (2005). Bubble formation and bubble rise velocity in gas–liquid systems: A review. Industrial & Engineering Chemistry Research, 44, 5873–5931. DOI: 10.1021/ie049131p.10.1021/ie049131pSuche in Google Scholar
Lehr, F., Millies, M., & Mewes, D. (2002). Bubble-size distributions and flow fields in bubble columns. AICHE Journal, 48, 2426–2443. DOI: 10.1002/aic.690481103.10.1002/aic.690481103Suche in Google Scholar
Lin, T. J., Tsuchiya, K., & Fan, L. S. (1998). Bubble flow characteristics in bubble columns at elevated pressure and temperature. AIChE Journal, 44, 545–560. DOI: 10.1002/aic.690440306.10.1002/aic.690440306Suche in Google Scholar
Machačová, K., Raška, P., Wichterle, K., Večeř, M., & Růžička, M. (2005). Periodicity of the motion of wobbling ellipsoidal bubbles. In Proceedings of the 52nd Conference CHISA 2005, October 17–20, 2005 (0215). Srní, Czech Republic: Czech Society of Chemical Engineering. (in Czech)Suche in Google Scholar
Machačová, K., Wichterle, K., & Večeř, M. (2006). Motion periodicity of wobbling ellipsoidal bubbles. In J. Markoš, & V. Štefuca (Eds.), Proceedings of the 33rd International Conference of Slovak Society of Chemical Engineering, May 21– 25, 2001 (P062, pp. 270–273). Tatranské Matliare, Slovakia: Slovak Society of Chemical Engineering.Suche in Google Scholar
Mendelson, H. D. (1967). The prediction of bubble terminal terminal velocity from wave theory. AICHE Journal, 13, 250– 253. DOI: 10.1002/aic.690130213.10.1002/aic.690130213Suche in Google Scholar
Moo-Young, M., Fulford, G., & Cheyne, I. (1971). Bubble motion studies in a countercurrent flow apparatus. Industrial & Engineering Chemistry Fundamentals, 10, 157–160. DOI: 10.1021/i160037a027.10.1021/i160037a027Suche in Google Scholar
Mudde, R. F. (2005). Gravity-driven bubbly flows. Annual Review of Fluid Mechanics, 37, 393–423. DOI: 10.1146/ annurev.fluid.37.061903.175803.10.1146/ annurev.fluid.37.061903.175803Suche in Google Scholar
Ravelet, F., Colin, C., & Risso, F. (2011). On the dynamics and breakup of a bubble rising in a turbulent flow. Physics of Fluids, 23, 103301. DOI: 10.1063/1.3648035.10.1063/1.3648035Suche in Google Scholar
Ribeiro, C. P., Jr., & Mewes, D. (2006). On the effect of liquid temperature upon bubble coalescence. Chemical Engineering Science, 61, 5704–5716. DOI: 10.1016/j.ces.2006.04.043.10.1016/j.ces.2006.04.043Suche in Google Scholar
Roizard, C., Mokrani, F., Le Gall, H., & Midoux, N. (1993). Gas-absorption in a centrifugal reactor: hydrodynamics. Chemical Engineering Science, 48, 2599–2608. DOI: 10.1016/ 0009-2509(93)80270-z.10.1016/ 0009-2509(93)80270-zSuche in Google Scholar
Schlichting, H., & Gersten, K. (2000). Boundary-layer theory (8th ed.). Berlin, Germany: Springer.10.1007/978-3-642-85829-1Suche in Google Scholar
Schulze, G., & Schlünder, E. U. (1985). Physical absorption of single gas bubbles in degassed and preloaded water. Chemical Engineering and Processing: Process Intensification, 19, 27–37. DOI: 10.1016/0255-2701(85)80002-7.10.1016/0255-2701(85)80002-7Suche in Google Scholar
Smutná, K., Wichterle, K., & Večeř, M. (2008). Study on behavior of bubbles rising in various liquids. In Proceedings of the 18th International Conference CHISA 2008, August 24– 28, 2008 (P1.14). Prague, Czech Republic: Czech Society of Chemical Engineering.Suche in Google Scholar
Stanovsky, P., Ruzicka, M. C., Martins, A., & Teixeira, J. A. (2011). Meniscus dynamics in bubble formation: A parametric study. Chemical Engineering Science, 66, 3258–3267. DOI: 10.1016/j.ces.2011.02.004.10.1016/j.ces.2011.02.004Suche in Google Scholar
Tanaka, Y., Osumi, T., & Tsuchiya, K. (2007). Correlating mass transfer coefficient for bubbles of different sizes: from microspheres to large caps. In Proceedings of the 6th International Conference on Multiphase Flow, ICMF 2007, July 9–13, 2007. Leipzig, Germany: ERCOFTAC.Suche in Google Scholar
Tomiyama, A., Celata, G. P., Hosokawa, S., & Yoshida, S. (2002). Terminal velocity of single bubbles in surface tension force dominant regime. International Journal of Multiphase Flow, 28, 1497–1519. DOI: 10.1016/s0301-9322(02)00032-0.10.1016/s0301-9322(02)00032-0Suche in Google Scholar
Tsuge, H. (1986). Hydrodynamics of bubble formation from submerged orifices. In N. P. Cheremisinoff (Ed.) Encyclopedia of fluid mechanics: Supplement 3: Advances in flow dynamics (pp. 191–232). Houston, TX, USA: Gulf Publishing Company.Suche in Google Scholar
Vasconcelos, J. M. T., Orvalho, S. P., & Alves, S. S. (2002). Gas–liquid mass transfer to single bubbles: Effect of surface contamination. AICHE Journal, 48, 1145–1154. DOI: 10.1002/aic.690480603.10.1002/aic.690480603Suche in Google Scholar
Vecer, M., Lestinsky, P., Wichterle, K., & Ruzicka, M. (2012). On bubble rising in countercurrent flow. International Journal of Chemical Reactor Engineering, 10, A30. DOI: 10.1515/1542-6580.2995.10.1515/1542-6580.2995Suche in Google Scholar
Vejrazka, J., Fujasová, M., Stanovsky, P., Ruzicka, M. C., & Drahoš, J. (2008). Bubbling controlled by needle movement. Fluid Dynamics Research, 40, 521–533, DOI: 10.1016/j. fluiddyn.2007.12.008.10.1016/j. fluiddyn.2007.12.008Suche in Google Scholar
Wang, G. F., Lowry, M., Zhong, Z. M., & Geng, L. (2005). Direct observation of frits and dynamic air bubble formation in capillary electrochromatography using confocal fluorescence microscopy. Journal of Chromatography A, 1062, 275–283. DOI: 10.1016/j.chroma.2004.11.052.10.1016/j.chroma.2004.11.052Suche in Google Scholar PubMed
Wellek, R. M., Agrawal, A. K., & Skelland, A. H. P. (1966). Shape of liquid drops moving in liquid media. AICHE Journal, 12, 854–862. DOI: 10.1002/aic.690120506.10.1002/aic.690120506Suche in Google Scholar
Wichterle, K., Wichterlová, J., & Kulhánková, L. (1999). Technika levitujících bublin pro studium přenosu hybnosti a hmoty. In Proceedings of the 46th Conference CHISA 99, October 18–21, 1999. Srní, Czech Republic: Czech Society of Chemical Engineering. (in Czech)Suche in Google Scholar
Wichterle, K., Kulhánková, L., & Wichterlová, J. (2000). Bubbleriseinswirl flow. In Proceedings of the 14th International Congress CHISA 2000, August 27–31, 2000 (P1.38). Prague, Czech Republic: Czech Society of Chemical Engineering.Suche in Google Scholar
Wichterle, K. (2001). Dynamics of rising bubbles. In Proceedings of the 28th International Conference of Slovak Society of Chemical Engineering, May 21–25, 2001 (pp. 72–73). Tatranské Matliare, Slovakia: Slovak Society of Chemical Engineering.Suche in Google Scholar
Wichterle, K., Wichterlová, J., & Kulhánková, L. (2005). Breakup of bubbles rising in liquids of low and moderate viscosity. Chemical Engineering Communications, 192, 550– 556. DOI: 10.1080/00986440590495034.10.1080/00986440590495034Suche in Google Scholar
Wichterle, K., Večeř, M., & Růžička, M. C. (2014). Asymmetric deformation of bubble shape: cause or effect of vortex-shedding? Chemical Papers, 68, 74–79. DOI: 10.2478/ s11696-013-0406-9.10.2478/ s11696-013-0406-9Suche in Google Scholar
© Institute of Chemistry, Slovak Academy of Sciences
Artikel in diesem Heft
- Review
- Bimetallic nickel and palladium complexes for catalytic applications
- Original Paper
- Enantiomeric purity control of R-cinacalcet in pharmaceutical product by capillary electrophoresis
- Original Paper
- Sensitive electrogravimetric immunoassay of hepatitis B surface antigen through hyperbranched polymer bridge linked to multiple secondary antibodies
- Original Paper
- Plant waste residues as inducers of extracellular proteases for a deuteromycete fungus Trichoderma atroviride
- Original Paper
- Bioremediation of PCB-contaminated sediments and evaluation of their pre- and post-treatment ecotoxicity
- Original Paper
- Simple and efficient treatment of high-strength industrial waste water using commercial zero-valent iron
- Original Paper
- UV light-assisted mineralisation and biodetoxification of Ponceau S with hydroxyl and sulfate radicals
- Original Paper
- Measuring free ellagic acid: influence of extraction conditions on recovery by studying solubility and UV-Visible spectra
- Original Paper
- Effect of sample pre-treatment on isoflavones quantification in soybean
- Original Paper
- TG-DTA-FTIR analysis and isoconversional reaction profiles for thermal and thermo-oxidative degradation processes in black chokeberry (Aroniamelanocarpa)
- Original Paper
- Flow field in a downward diverging channel and its application
- Original Paper
- Use of dodecanoyl isothiocyanate as building block in synthesis of target benzothiazine, quinazoline, benzothiazole and thiourea derivatives
- Short Communication
- Solvent-free synthesis of 6-unsubstituted dihydropyrimidinones using 2-pyrrolidonium bisulphate as efficient catalyst
Artikel in diesem Heft
- Review
- Bimetallic nickel and palladium complexes for catalytic applications
- Original Paper
- Enantiomeric purity control of R-cinacalcet in pharmaceutical product by capillary electrophoresis
- Original Paper
- Sensitive electrogravimetric immunoassay of hepatitis B surface antigen through hyperbranched polymer bridge linked to multiple secondary antibodies
- Original Paper
- Plant waste residues as inducers of extracellular proteases for a deuteromycete fungus Trichoderma atroviride
- Original Paper
- Bioremediation of PCB-contaminated sediments and evaluation of their pre- and post-treatment ecotoxicity
- Original Paper
- Simple and efficient treatment of high-strength industrial waste water using commercial zero-valent iron
- Original Paper
- UV light-assisted mineralisation and biodetoxification of Ponceau S with hydroxyl and sulfate radicals
- Original Paper
- Measuring free ellagic acid: influence of extraction conditions on recovery by studying solubility and UV-Visible spectra
- Original Paper
- Effect of sample pre-treatment on isoflavones quantification in soybean
- Original Paper
- TG-DTA-FTIR analysis and isoconversional reaction profiles for thermal and thermo-oxidative degradation processes in black chokeberry (Aroniamelanocarpa)
- Original Paper
- Flow field in a downward diverging channel and its application
- Original Paper
- Use of dodecanoyl isothiocyanate as building block in synthesis of target benzothiazine, quinazoline, benzothiazole and thiourea derivatives
- Short Communication
- Solvent-free synthesis of 6-unsubstituted dihydropyrimidinones using 2-pyrrolidonium bisulphate as efficient catalyst