Band 12, Heft 4

Research regarding electrochromic (EC) materials, such materials that change their color upon application of an electrochemical stimulus, has been conducted for centuries. However, most recently, increasing efforts have been put into developing novel solutions to utilize these on-off switching materials in advanced nanoplasmonic and nanophotonic devices. Due to the significant change in dielectric properties of oxides such as WO 3 , NiO, Mn 2 O 3 and conducting polymers like PEDOT:PSS and PANI, EC materials have transcended beyond simple smart window applications and are now found in plasmonic devices for full-color displays and enhanced modulation transmission and photonic devices with ultra-high on-off ratios and sensing abilities. Advancements in nanophotonic ECDs have further decreased EC switching speed by several orders of magnitude, allowing integration in real-time measurement and lab-on-chip applications. The EC nature of such nanoscale devices promises low energy consumption with low operating voltages paired with bistability and long lifetimes. We summarize these novel approaches to EC device design, lay out the current short comings and draw a path forward for future utilization.

This broad review summarizes recent advances and “hot” research topics in nanophononics and elastic, acoustic, and mechanical metamaterials based on results presented by the authors at the EUROMECH 610 Colloquium held on April 25–27, 2022 in Benicássim, Spain. The key goal of the colloquium was to highlight important developments in these areas, particularly new results that emerged during the last two years. This work thus presents a “snapshot” of the state-of-the-art of different nanophononics- and metamaterial-related topics rather than a historical view on these subjects, in contrast to a conventional review article. The introduction of basic definitions for each topic is followed by an outline of design strategies for the media under consideration, recently developed analysis and implementation techniques, and discussions of current challenges and promising applications. This review, while not comprehensive, will be helpful especially for early-career researchers, among others, as it offers a broad view of the current state-of-the-art and highlights some unique and flourishing research in the mentioned fields, providing insight into multiple exciting research directions.

The inverse Faraday effect (IFE) generates magnetic fields by optical excitation only. Since its discovery in the 60 s, it was believed that only circular polarizations could magnetize matter by this magneto-optical phenomenon. Here, we demonstrate the generation of an IFE via a linear polarization of light. This new physical concept results from the local manipulation of light by a plasmonic nano-antenna. We demonstrate that a gold nanorod excited by a linear polarization generates non-zero magnetic fields by IFE when the incident polarization of the light is not parallel to the long axis of the rod. We show that this dissymmetry generates hot spots of local non-vanishing spin densities (local elliptical polarization state), introducing the concept of super circular light, allowing this magnetization. Moreover, by varying the angle of the incident linear polarization with respect to the nano-antenna, we demonstrate the on-demand flipping of the magnetic field orientation. Finally, this linear IFE generates a magnetic field 25 times stronger than a gold nanoparticle via a classical IFE. Because of its all-optical character, this light–matter interaction opens the way to ultrafast nanomanipulation of magnetic processes such as domain reversal, skyrmions, circular dichroism, control of the spin, its currents, and waves, among others.

Two-dimensional transition metal dichalcogenides (2D TMDs) have been demonstrated as one of the most outstanding materials not only for fundamental science but also for a wide range of photonic applications. However, an efficient way to control their excitonic properties is still needed for advanced applications with superior device performance. Here, we show that the exciton lifetime of WSe 2 monolayer can be prolonged using metamaterials. We observe a ∼100% reduction in the electron-hole recombination rate of WSe 2 monolayer placed on a hyperbolic metamaterial substrate and demonstrate that such a remarkable change results from the destructive image dipole interaction with the in-plane exciton transition dipole. Furthermore, this substantial increase in exciton lifetime leads to order-of-magnitude (10-fold) enhancement of photocurrent in the 2D WSe 2 -based hybrid photodetector with metamaterials. Tailoring the optical transition properties of 2D TMD materials with specially designed metamaterials, demonstrated here, will pave the way for developing 2D material-based optoelectronics.

Germanium-on-silicon (Ge-on-Si) single photon avalanche diodes (SPADs) have received wide attention in recent years due to their potential to be integrated with Si photonics. In this work, we propose and demonstrate a high-performance waveguide coupled Ge-on-Si separate-absorption-charge-multiplication SPAD with three electric terminals. By providing two separate voltage drops on the light absorption and multiplication regions, the drift and multiplication of carriers can be optimized separately. This indeed improves the freedom of voltage regulation for both areas. Moreover, thanks to the separate controlling, doping profile of the charge layer is greatly released compared to that of the conventional device because of the flexible carrier injection. In this scenario, the dark counts of the detector can be largely reduced through decreasing the electric field on the sidewalls of the Ge absorption region without affecting the detection efficiency. The proposed SPAD exhibits a high on-chip single photon detection efficiency of 34.62% and low dark count rates of 279 kHz at 1310 nm with the temperature of 78 K. The noise equivalent power is as low as 3.27 × 10 −16 WHz −1/2 , which is, to the best of our knowledge, the lowest of that of the reported waveguide coupled Ge-on-Si SPADs. This three-terminal SPAD enables high-yield fabrication and provides robust performance in operation, showing a wide application prospect in applications such as on-chip quantum communication and lidar.

We propose an all on-chip micro-ring resonator array spectrum detection system (MRRAS). Micro-ring resonator array as the core is used to construct the transmission matrix of the system. The theoretical analysis of the spectrum detection system is completed with waveguide transmission theory and spectrum construction method based on convex optimization algorithm. In the experiment, we obtain the priori information of the transmission matrix of the system, then detect the output intensity of unknown spectrum through MRRAS, and construct the under-determined matrix equations when the number of micro-rings is much smaller than that of reconstructed wavelengths. Convex optimization algorithm is employed to obtain the least norm solution of the under-determined matrix equations, which enables fast spectrum reconstruction. The experimental results show that the spectrum detection system is constructed using three micro-ring resonators with 4 μm radius, enabling the compact footprint. In addition, the silicon nitride based photonic platform is fully compatible with standard complementary metal oxide semiconductor (CMOS) processes. The system operating bandwidth is more than 12 nm and the resolution is better than 0.17 nm.

Metafibers, by integrating metasurface at the optical fiber tip, are emerging as the significant optical coupling platforms for nanophotonics and fiber-optic communities. Here, we propose a plasmonic metafiber for converting the fundamental mode to first-order mode in fiber, and as proof of device performance, demonstrate an all-fiber Q -switched cylindrical vector laser using the metafiber. Based on polarization-dependent plasmonic resonance, a polarization-independent mode conversion metasurface is designed theoretically and numerically, fabricated directly on fiber facet, and packaged as an all-fiber component with efficiency up to 21% at 1550-nm band. Using the metafiber in an all-fiber laser, Q -switched azimuthally polarized beam (APB) and radially polarized beam (RPB) are delivered at wavelength of 1548.5 nm with pulse durations from ∼7 to ∼2 μs when pump power increases from 30 to 120 mW. The mode purities of the APB and RPB are 86.5% and 90.7%, respectively. This work outlines a new strategy to integrate metasurfaces into “all-in-fiber” systems and offers a reliable route to construct next-generation laser sources, such as all-fiber ultrafast structured lasers.

While the strong coupling between cavity modes and quantum emitters has been investigated in various systems, multiple surface plasmon modes in single nanostructures strongly coupling with excitons are rarely explored. Here, we investigate the strong coupling between three surface plasmon modes in silver nanowires and excitons in monolayer WSe 2 at room temperature. Four plasmon-exciton polariton (plexciton) states are observed in the scattering spectra. The photoluminescence (PL) spectra of the hybrid system show clear splitting due to strong coupling, and the energies of the emission corresponding to the two lower plexciton states agree with that of the scattering very well. In addition, we show that the plasmon-exciton interaction in this system can be efficiently tuned by controlling the excitation power. These results reveal the fundamental properties of strong coupling between multiple plasmon modes and excitons, deepen the understanding of the correlation between scattering and PL spectra of plasmon-exciton strong coupling systems, and open up a new way to actively control the coupling between plasmonic nanostructures and two-dimensional semiconductors.

Barium fluoride, an inorganic scintillation material used for the detection of X-ray and/or gamma-ray radiation, has been receiving increasing attention in the field of radiation measurements in fast-timing applications. To make full use of its timing properties, its slow emission around the ultraviolet region, more specifically, the 300 nm region needs to be suppressed. Although doping ions, such as lanthanum, yttrium, and cadmium, can suppress the slow component, such techniques can lose information of interacted radiations. Consequently, a suppression technique that does not suffer from information loss while maintaining precise timing measurements would be desirable. In this study, we proposed aluminum nano-disk-based plasmonic filters to suppress slow emissions while maintaining fast emissions around 195 and 220 nm and a usability of the slow component. Finite-difference time-domain simulations and experimental results exhibited good agreement, with over 90% of slow components being adequately suppressed without sacrificing fast components, proving that aluminum nanodisks can be used for ultraviolet filters. Moreover, based on the designed filter performance, we conducted coincidence time resolution simulations for positron–electron annihilation gamma rays from an analytical perspective. The simulations indicated the designed filters could maintain high timing performance. Consequently, the proposed plasmonic ultraviolet filter was suitable for maximizing the potential of barium fluoride scintillators.

Most of the previous TMDC-photon coupling devices were mainly based on A exciton due to its high oscillator strength and large exciton binding energy. Less effort has been focused on the modulation of the emission of B exciton and Rydberg states in TMDCs, especially in monolayer WS 2 . Here, we demonstrate that the photoluminescence (PL) emission of WS 2 -microcavity coupling devices can be tailored in a broad visible wavelength range (490 nm–720 nm). In contrast to the intrinsic PL emission of monolayer WS 2 , 25-fold enhanced B exciton emission and significant PL emission from the 2s Rydberg state can be observed. From the transient absorption (TA) measurements, the strongly coupled hybrid states based on B exciton can be remarkably fingerprinted. Furthermore, the strongly enhanced PL emission from the coupled B exciton has been demonstrated due to the strongly increased lower polariton (LP) state population and the internal conversion pathway being blocked in the strong coupling regime. Besides, the remarkable PL emission from the 2s Rydberg state is also revealed and confirmed by the additional ground state bleaching signal in TA spectra. These physical mechanisms about tailoring the PL emission in low dimensional TMDCs can provide significant references for constructing highly efficient optoelectronic devices.

Replica symmetry breaking (RSB) has been widely recognized as a statistical analysis approach to understand the disorder and nonlinear interactions in complex systems ranging from atoms to the cosmic scale. However, it is challenging to analyze the nonlinear optical characteristics of random laser (RL) in disordered gain medium via RSB due to the lack of a general RSB-based statistical analysis framework. In this work, we report the tunable RSB in polymer fiber RL, where the effects of temperature and different structures on RSB are investigated experimentally and theoretically. It experimentally proves that RSB in RL is not robust, and disorder and temperature are responsible for tunable RSB in RL, which contributes to the improvement of the statistical analysis framework for investigating the optical principles of RL using RSB. And the finding of the tunable RSB allows to investigate the dynamical differences for various RL systems, which broadens the directions for the use of spin-glass theory to explore the physical mechanism of RL.