Band 12, Heft 16

Fano resonance due to coupling of plasmon mode and Bragg modes is revealed without strong angular dependence based on Au nanoparticle on distributed Bragg reflectors (Au NPoDBRs). This Fano interference involves three-modes-coupling: the nanoparticle’s plasmon resonance, dispersive Bragg modes, and non-dispersive Bragg modes. It can be interpreted as a consequence of two processes: plasmonic coupling between dispersive Bragg modes and broad plasmon mode, and the strong coupling between narrowed plasmonic mode and non-dispersive Bragg mode. This Fano interference shows little dependence on the incidence angle but high tunability with the top-layer thickness, which is exploitable for novel nanophotonic devices with dispersion engineering.

Thermal effects are well known to influence the electronic and optical properties of materials through several physical mechanisms and are the basis for various optoelectronic devices. The thermo-optic (TO) effect, the refractive index variation with temperature (d n /d T ), is one of the most common mechanisms used for tunable optical devices, including integrated optical components, metasurfaces, and nano-antennas. However, when a static and fixed operation is required, i.e., temperature invariant performance – this effect becomes a drawback and may lead to undesirable behavior through drifting of the resonance frequency, amplitude, or phase, as the operating temperature varies over time. In this work, we present a systematic approach to mitigate thermally induced optical fluctuations in nanophotonic devices. By using hybrid subwavelength resonators composed from two materials with opposite TO dispersions (d n /d T < 0 and d n /d T > 0), we are able to compensate for TO shifts and engineer nanophotonic components with zero effective TO coefficient (d n eff /d T ≈ 0). We demonstrate temperature invariant resonant frequency, amplitude, and phase response in meta-atoms and metasurfaces operating across a wide temperature range and broad spectral band. Our results highlight a path towards temperature invariant nanophotonics, which can provide constant and stable optical response across a wide range of temperatures and be applied to a plethora of optoelectronic devices. Controlling the sign and magnitude of TO dispersion extends the capabilities of light manipulation and adds another layer to the toolbox of optical engineering in nanophotonic systems.

In this study, we experimentally showcase the microfiber evanescent-field photothermal gas detection by exploiting all-fiber MHz-level frequency shift scheme. Based on the acousto-optic interaction effect, the low-frequency shifts of 0.9 MHz and 1.83 MHz can be obtained through the cyclic conversion between the transverse core modes LP 01 and LP 11 in the few-mode fiber. Our proposed all-fiber frequency shifters show flexible MHz-level up(down) frequency shifts with superior sideband rejection ratio (over 40 dB) and low insertion loss (less than 1 dB). Furthermore, an all-fiber heterodyne interferometric detection system is implemented by leveraging the above low-frequency shifters, in which around 1-μm-diameter microfiber is investigated for photothermal gas detection. A pump-probe configuration is employed to obtain the photothermal effect induced by the gas absorption of the modulated evanescent field. By demodulating the phase of the beat signal output by the interferometer, an equivalent detection limit (1 σ ) of 32 ppm and a response time of 22 s are achieved for ammonia, as well as 0.24 % instability within 48 pump cycles. Given its compact all-fiber configuration and high sensitivity with fast response, the experimental results can pave the way for widespread applications like heterodyne detection, fiber optical sensors, and interplanetary coherent communications.

We propose and experimentally demonstrate a single chip metasurface for simultaneous chiral and achiral imaging and polarimetric detecting using a high efficiency three dimensional plasmonic metalens (3D-PM) with capability of designed separation of different circular polarizations. The proposed 3D-PM combines both propagating and geometric phases so that two orthogonal circular polarization components of the incidence can be precisely separated and imaged into two channels and the incident polarization state can be detected with differentiation of the two channels. One single set of an array of Au layer covered anisotropic polymethyl methacrylate elliptical nanopillars is employed, in which height of each nanopillar is added as a new design degree of freedom to realize both full phase manipulation (0–2 π ) and high efficiency (>0.85) with coupled equivalent Fabry–Pérot cavity and localized surface plasmons. At design wavelength of 1550 nm, experimental results show that optical resolution of both chiral and achiral images approaches the diffraction limit, extinction ratio of circular polarizations in two channels is ∼33:1, and the energy efficiency reaches ∼63 %. The proposed 3D-PM provides a new and simple way for chiral/achiral imaging and polarimetric measurement, and can be applied in integrated optics, optical communication, and biomolecule detection.

High beam quality, large-area output, and small footprint are significant pursuing goals for vertical-cavity surface-emitting lasers (VCSELs), which impose strict requirements on tight light confinements with minimized radiation losses. To achieve this, bound states in the continuum (BICs) have been demonstrated as an effective way of trapping light. Here, we combine BICs and photonic bandgaps to realize a quasi-BIC single-mode photonic crystal (PhC) laser on a colloidal quantum dots (CQDs)/silicon oxide (SiO 2 ) hybrid integrated platform. The PhC cavity is a defect-free hexagonal heterostructure with three regions, and the thin CQDs film is embedded within the SiO 2 nanopillar planar array as both an optical gain material and a backbone for the PhC. The mode gaps between different regions provide the lateral confinement while the quasi-BICs near the Γ-point generate the small-divergence vertical radiation coupling, resulting in a well-defined emission concentrating within ±1.85° of the normal surface direction and an optical pumping energy density threshold of 216.75 μJ/cm 2 . Our results demonstrate the design flexibility and versatility of the quasi-BIC laser even with a low contrast of a refractive index between the PhC slab and the substrate, which has potential applications in cavity quantum electrodynamics, nonlinear optics, and integrated photonics.

Modifying the light–matter interactions in the plasmonic structures and the two-dimensional (2D) materials not only advances the deeper understanding of the fundamental studies of many-body physics but also provides the opportunities for exploration of novel 2D plasmonic polaritonic devices. Here, we report the plasmon-exciton coupling in the hybrid system with a plasmonic metasurface which can confine the electric field in an extremely compact mode volume. Because of the 2D feature of the designed and fabricated Al plasmonic metasurface, the confined electronic field is distributed in the plane with the same orientation as that of the exciton dipole moment in the transition metal dichalcogenides monolayers. By finely tuning the geometric size of the plasmonic nanostructures, we can significantly modify the dispersion relation of the coupled plasmon and the exciton. Our system shows a strong coupling behavior with an achieved Rabi splitting up to ∼200 meV at room temperature, in ambient conditions. The effective tailoring of the plasmon-exciton coupling with the plasmonic metasurfaces provides the testing platform for studying the quantum electromagnetics at the subwavelength scale as well as exploring plasmonic polariton Bose–Einstein condensation at room temperature.

The surface-response formalism (SRF), where quantum surface-response corrections are incorporated into the classical electromagnetic theory via the Feibelman parameters, serves to address quantum effects in the optical response of metallic nanostructures. So far, the Feibelman parameters have been typically obtained from many-body calculations performed in the long-wavelength approximation, which neglects the nonlocality of the optical response in the direction parallel to the metal–dielectric interface, thus preventing to address the optical response of systems with extreme field confinement. To improve this approach, we introduce a dispersive SRF based on a general Feibelman parameter d ⊥ ( ω , k ‖ ), which is a function of both the excitation frequency, ω , and the wavenumber parallel to the planar metal surface, k ‖ . An explicit comparison with time-dependent density functional theory (TDDFT) results shows that the dispersive SRF correctly describes the plasmonic response of planar and nonplanar systems featuring extreme field confinement. This work thus significantly extends the applicability range of the SRF, contributing to the development of computationally efficient semiclassical descriptions of light–matter interaction that capture quantum effects.

Exciton resonances in monolayer transition-metal dichalcogenides (TMDs) provide exceptionally strong light–matter interaction at room temperature. Their spectral line shape is critical in the design of a myriad of optoelectronic devices, ranging from solar cells to quantum information processing. However, disorder resulting from static inhomogeneities and dynamical fluctuations can significantly impact the line shape. Many recent works experimentally evaluate the optical properties of TMD monolayers placed on a substrate and the line shape is typically linked directly to the material’s quality. Here, we highlight that the interference of the substrate and TMD reflections can strongly influence the line shape. We further show how basic, room-temperature reflection measurements allow investigation of the quantum mechanical exciton dynamics by systematically controlling the substrate reflection with index-matching oils. By removing the substrate contribution with properly chosen oil, we can extract the excitonic decay rates including the quantum mechanical dephasing rate. The results provide valuable guidance for the engineering of exciton line shapes in layered nanophotonic systems.

Epsilon-near-zero (ENZ) materials have recently emerged as a promising platform for infrared nanophotonics. A significant challenge in the design of ENZ-based optics is to control the dispersion of ENZ modes that otherwise have a flat profile near the ENZ frequency. Strong coupling with an optical cavity is a promising approach to ENZ dispersion engineering, which however has limitations due to the lack of tunability or nanofabrication demands of the cavity employed. Here, we theoretically and numerically show that much of the limitations of previous approaches can be overcome by strongly coupling the ENZ mode to an unpatterned Fabry–Perot cavity. We demonstrate this unprecedented ENZ dispersion control in coupled cavities by designing tunable infrared polarizers that can absorb s and reflect p -polarized components, or vice versa, for almost any oblique angle of incidence, i.e. omnidirectional polarizers. The feasibility of active control is also demonstrated using a phase change material within the cavity, which predicts dynamic switchability of polariton dispersions across multiple resonant levels at mid-infrared wavelengths. These results are expected to advance the current understanding of strongly coupled ENZ interactions and demonstrate their potential in tailoring dispersions for active and passive control of light.

Tunnel nanojunctions based on inelastic electron tunneling (IET) have been heralded as a breakthrough for ultra-fast integrated light sources. However, the majority of electrons tend to tunnel through a junction elastically, resulting in weak photon-emission power and limited efficiency, which have hindered their practical applications to date. Resonant tunneling has been proposed as a way to alleviate this limitation, but photon-emissions under resonant tunneling conditions have remained unsatisfactory for practical IET-based light sources due to the inherent contradiction between high photon-emission efficiency and power. In this work, we introduce a novel approach that leverages much stronger resonant tunneling enhancement achieved by multiple metallic quantum wells, which has enabled the internal quantum efficiency to reach ∼1 and photon-emission power to reach ∼0.8 µW/µm 2 . Furthermore, this method is applicable with different electronic lifetimes ranging from 10 fs to 100 fs simultaneously, bringing practical implementation of IET-based sources one step closer to reality.

This study proposes and demonstrates a novel label-free DNA biosensor using high quality optical microcavity functionalized by 3D DNA nanostructure probes. To achieve ultra-low limit DNA biosensing, optical sensing interface of the hollow-core, thin wall-thickness microcavity was functionalized by self-assembled DNA tetrahedral nanostructure (DTN) probes with size of 17 bp and length of ∼5.8 nm. High efficiency binding of the DTN probes with the optical sensor interface and the target ssDNA are achieved. Whispering gallery mode (WGM) spectra with high- Q factor of >10 7 are excited and traced for DNA detection inside the microfluidic channel of the microcavity, with a small sample volume of nL. Incorporation of nanoscale DTN probes onto surface of the optical microcavity makes it an effective way for increasing efficient probe density and eliminating entanglement between DNA probes, thus ∼1000 times lower detection limit is achieved as compared to using 1D ssDNA probes. Due to its desirable merits of label-free, ultra-low LoD, real time and compact size, the proposed DNA biosensor has broad application prospects in bioengineering and medical diagnosis.

Weyl semimetals hold great promise in revolutionizing nonreciprocal optical components due to their unique topological properties. By exhibiting nonreciprocal magneto-optical effects without necessitating an external magnetic field, these materials offer remarkable miniaturization opportunities and reduced energy consumption. However, their intrinsic topological robustness poses a challenge for applications demanding tunability. In this work, we introduce an innovative approach to enhance the tunability of their response, utilizing multilayered configurations of twisted anisotropic Weyl semimetals. Our design enables controlled and reversible isolation by adjusting the twist angle between the anisotropic layers. When implemented in the Faraday geometry within the mid-IR frequency range, our design delivers impressive isolation, exceeding 50 dB, while maintaining a minimal insertion loss of just 0.33 dB. Moreover, the in-plane anisotropy of Weyl semimetals eliminates one or both polarizers of conventional isolator geometry, significantly reducing the overall dimensions. These results set the stage for creating highly adaptable, ultra-compact optical isolators that can propel the fields of integrated photonics and quantum technology applications to new heights.

We present a 1D reflective multi-level structural color design that incorporates Mie, plasmonic, and diffractive mechanisms in the same pixel. Comprised of a metallodielectric grating made of TiO x nanowires sandwiched between Ag thin film and Ag substrate, the design can exhibit either a Mie resonance or a localized plasmonic resonance depending on the polarization of incident light, resulting in dramatically different color states. Due to the periodicity, the grating also diffracts light, providing an additional color state. Since diffraction can be turned on or off by the degree of coherence of the incoming light, both Mie and plasmonic colors can be modulated using objective lenses with different numerical apertures. Exploiting the different color generating modes, we encode four layers of information in a pixel array, where each layer is unveiled using a different combination of excitation and imaging settings. These results introduce new possibilities for data encryption, anticounterfeiting, and data storage.

Single-photon emitters are a pivotal element in quantum technologies, but the generation of single photons along well-defined directions generally involves sophisticated configurations. Here, we propose a photon source capable of generating single photons with high efficiency along guided modes. Specifically, we consider a quantum emitter placed in a periodically patterned linear waveguide. The latter is designed to host a single guided mode over the spectral range of interest and display a divergence in the photonic density of states at an emission wavelength close to the period. Photons are preferentially emitted along the waveguide near that spectral region. We predict that nearly all of the emission can be made to occur along the waveguide with a reduction in the temporal uncertainty by two orders of magnitude. Our study opens a conceptually new direction in the production of single photons with a high degree of directionality and reduced temporal uncertainty.

Functional devices for terahertz (THz) polarization detection in transmission mode are highly desired in integrated applications, but traditional polarization measurement systems are bulky and highly cost. The combination between all-silicon metasurfaces and focused beams carrying polarization information has offered a new opportunity for miniaturized polarization detection behavior. Here, we investigate and experimentally demonstrate a new scheme for realizing efficiently miniaturized polarization detection behavior based on the polarization multiplexing encoding technique. The full-Stokes parameter matrix of the incident polarization state can be reconstructed in a single snapshot by using a microprobe to record, pixel by pixel, the complex amplitude information contained in a pre-designed plane. Subsequently, the polarization detection capability of the proposed design principle is evaluated using random polarization states defined on the surface of a standard Poincaré sphere (PS). Such a scheme offers potential applications for the development of compact photonic meta-platforms for polarization detection in transmission mode, being highly favored in polarization high-resolution imaging, remote sensing, and THz communications.

The ultraviolet (UV) wavelength regime is attracting increasing attention because of its growing demand in semiconductor lithography, spectroscopy, and imaging applications owing to its high spatial resolution and high photon energy. However, beam shape control, beam delivery, and wavefront manipulation of UV laser beams usually require highly dedicated optics because of the strong UV absorption of most optical materials and the high surface precision required for tailoring short wavelengths, thus limiting a broader application of UV wavelengths. Here, we demonstrate a novel dynamic UV harmonic beam pattern control by manipulating the near-infrared (NIR) wavefront of the fundamental wavelength of a femtosecond pulse laser. The temporal and spatial coherences in an optical harmonic generation are known to be well preserved. Therefore, the spatial beam distribution of UV harmonic beams ( λ = 400 and 266 nm for second and third harmonics, respectively) could be readily controlled by tailoring the wavefront of the driving infrared (IR) beam, and this approach can be expanded to higher-order harmonics in the vacuum ultraviolet (VUV) or extreme ultraviolet (EUV) regimes. Moreover, this enables fast polarization-sensitive UV beam switching at a speed of 6.7 frames/s in a depth-resolving manner. To efficiently separate the UV beam from the strong fundamental IR background beam, a non-collinear harmonic generation configuration is introduced. This facile dynamic UV beam control technique enables arbitrary wavefront control of UV laser beams for high-precision laser patterning, polarization-sensitive encryption, and 3D holograms.

How to simultaneously obtain the depth, edge, and other light information of the scene to accurately perceive the physical world is an important issue for imaging systems. However, such tasks usually require bulky optical components and active illumination methods. Here, we design and experimentally validate a single geometric metasurface that can achieve depth measurement or edge detection under incoherent or coherent light respectively. Double helix point source function is utilized, and three verification experiments are carried out, including double-helix beam calibration, 2D object and 3D object detection, respectively. Additionally, two-dimensional edge detection can also be achieved. This compact imaging system can enable new applications in various fields, from machine vision to microscopy.