Band 14, Heft 11 - Special Issue: Quantum Light: Creation, Integration, and Applications

In today’s rapidly evolving quantum landscape, the generation and manipulation of quantum light not only represent fundamental challenges but also herald unprecedented opportunities in communication, computing, sensing, and imaging. This special issue brings together a collection of contributions that span the entire journey, from the creation of quantum light using novel materials and emitters to its seamless integration into photonic architectures and eventual deployment in advanced quantum applications. This special issue, “ Quantum Light: Creation, Integration, and Applications ,” features a collection of three review articles, five perspectives, and 23 original research papers, highlighting both the timeliness of the topic and the remarkable breadth and richness of ongoing advancements in the field.

Solid-state single-photon emitters (SPEs) are attracting significant attention as fundamental components in quantum computing, communication, and sensing. Low-dimensional materials-based SPEs (LD-SPEs) have drawn particular interest due to their high photon extraction efficiency, ease of integration with photonic circuits, and strong coupling with external fields. The accessible surfaces of LD materials allow for deterministic control over quantum light emission, while enhanced quantum confinement and light–matter interactions improve photon emissive properties. This perspective examines recent progress in LD-SPEs across four key materials: zero-dimensional (0D) semiconductor quantum dots, one-dimensional (1D) nanotubes, two-dimensional (2D) materials, including hexagonal boron nitride (hBN) and transition metal dichalcogenides (TMDCs). We explore their structural and photophysical properties, along with techniques such as spectral tuning and cavity coupling, which enhance SPE performance. Finally, we address future challenges and suggest strategies for optimizing LD-SPEs for practical quantum applications.

Solid-state quantum emitters operating in the telecom wavelength range are pivotal for the development of scalable quantum information processing technologies. In this review, we provide a comprehensive overview of the state-of-the-art solid-state emitters of single photons targeting quantum information processing in the discrete-variable regime and telecom wavelength range. We focus on quantum dots, color centers, and erbium ion dopants, detailing their synthesis methods and their applications. The review addresses the strategies for the integration of these quantum emitters into photonic devices alongside the associated challenges. We also discuss their applications in quantum technologies, examining current limitations, including performance constraints, decoherence, and scalability. Finally, we propose future directions for advancing photonic-based quantum technologies.

Quantum super-resolution imaging provides a nonlabeling method to surpass the diffraction limit of imaging systems. This technique relies on measurement of the second-order correlation function and usually employs spatially entangled photon sources. We introduce recent methods that achieve spatial resolution enhancement through quantum approaches, particularly the imaging techniques utilizing biphoton states. The fundamental mechanisms are discussed in detail to explain why biphoton states enable super-resolution. Additionally, we introduce multiple algorithms that extract the correlation function from the readings of two-dimensional detectors. Several cases are reviewed to evaluate the advantages and prospects of quantum imaging, along with a discussion of practical developments and potential applications.

Nonlinear dynamics provide an indispensable resource for creating quantum states of light, as well as other bosonic systems. Seminal work using second- and third-order nonlinear optical crystals, cavity quantum electrodynamics, and superconducting circuits, have enabled generating squeezed states, as well as various non-Gaussian quantum states (e.g., single photons, cat states) at both infrared and microwave frequencies. Nevertheless, it remains challenging to generate quantum states of light in broad portions of the electromagnetic spectrum: for example, at terahertz frequencies and at ultraviolet and X-ray frequencies. In this Perspective, I discuss a variety of emerging material platforms, as well as emerging theoretical and experimental tools, which enable overcoming these challenges. The main argument of this Perspective is that advances in driving nonlinear dynamics of material excitations, will enable generating quantum states of these material excitations as well as quantum states of light at new frequency ranges. I will further argue that in order to realize much of the promise of this nascent field, there is a need for innovation in the laser systems used to drive these nonlinear dynamics: specifically, innovations in realizing high-power laser sources that have very low noise, having quantum statistics similar to coherent states of light which describe lower intensity laser systems. I will highlight some experimental and theoretical work, in understanding quantum noise dynamics in complex laser systems, that can address these challenges.

Frequency-bin encoding furnishes a compelling pathway for quantum information processing systems compatible with established lightwave infrastructures based on fiber-optic transmission and wavelength-division multiplexing. Yet although significant progress has been realized in proof-of-principle tabletop demonstrations, ranging from arbitrary single-qubit gates to controllable multiphoton interference, challenges in scaling frequency-bin processors to larger systems remain. In this Perspective, we highlight recent advances at the intersection of frequency-bin encoding and integrated photonics that are fundamentally transforming the outlook for scalable frequency-based quantum information. Focusing specifically on results on sources, state manipulation, and hyperentanglement, we envision a possible future in which on-chip frequency-bin circuits fulfill critical roles in quantum information processing, particularly in communications and networking.

Optical photons play unique role in transmitting information over long distances. Photonic links by the optical fiber networks compose the backbone of today’s global internet. Such fiber optics can also provide the most cost-effective quantum channels to distribute quantum information across distant stationary nodes in future large-scale quantum networks. This prospect motivates the recent emerging efforts in developing microwave-optical quantum transduction technology to interconnect microwave quantum processors. Various frequency conversion approaches are investigated to efficiently bridge the enormous electromagnetic frequency gap while preserving quantum coherence. Nonetheless, high-fidelity entanglement generation between remote quantum processing units has remained out of reach to date. Here, we summarize the state-of-the-art progresses in quantum transducer engineering and provide the perspectives on the key challenges and opportunities toward optically heralded quantum entanglement distributions.

Quantum networks, capable of transmitting arbitrary quantum states, provide a foundation for a wide range of quantum applications, including distributed quantum computing, distributed quantum sensing, and quantum communication. Photons are the natural carrier of information in quantum networks, but the exponential loss of optical fiber channels prevents the construction of large-scale quantum networks. A potential solution is implementing quantum repeaters based on quantum memories, which can efficiently establish long-distance entanglement from short-distance entanglement. In the past decades, intense efforts have been devoted to constructing large-scale quantum networks based on various atomic quantum memories. In this Perspective, we present a concise overview of current advancements in remote quantum networks, elucidate the imminent challenges that must be addressed, and discuss the future directions.

I present my perspective on sensing with quantum light. I summarise the motivations and methodology for identifying quantum enhancements in sensing over a classical sensor. In the real world, this enhancement will be a constant factor and not increase with the size of the quantum probe as is often advertised. I use a limited survey of interferometry, microscopy and spectroscopy to extract the vital challenges that must be faced to realise tangible enhancements in sensing with quantum light.

Quantum dots (QDs) are a promising source of single photons mainly due to their on-demand operation. However, their emission wavelength depends on their size and immediate surroundings in the solid-state environment. By applying a serrodyne electro-optic phase modulation, we achieve a spectral shift up to 0.01 nm (3.5 GHz) while preserving the purity and indistinguishability of the photons. This method provides an efficient and scalable approach for tuning the emission wavelength of QDs without relying on nonlinear frequency mixing or probabilistic processes. Our results show that the electro-optic phase modulation enables stable and tunable spectral shifts, making it suitable for applications such as quantum communication, quantum key distribution, and primarily integrating remote quantum dot sources into large-scale quantum networks.

B-centers in hexagonal boron nitride (hBN) are gaining significant research interest for quantum photonics applications due to precise emitter positioning and highly reproducible emission wavelengths at 436 nm. Here, we leverage the layered nature of hBN to directly measure the quantum efficiency (QE) of single B-centers. The defects were engineered in a 35 nm flake of hBN using electron beam irradiation, and the local dielectric environment was altered by transferring a 250 nm hBN flake on top of the one containing the emitters. By analyzing the resulting change in measured lifetimes, we determined the QE of B-centers in the thin flake of hBN. Additionally, we propose two approaches to quantify the QE of B-centers in thick flakes of hBN. Our results indicate that B-centers located in thin flakes can exhibit QEs higher than 40 %. Near-unity QEs are achievable under reasonable Purcell enhancement for emitters embedded in thick flakes of hBN, highlighting their promise for quantum photonics applications.

We conducted low-temperature photoluminescence (PL) spectroscopy experiments on individual WS 2 and MoSe 2 nanoribbons prepared by gold-assisted exfoliation from the slanted surface of bulk crystals with a vicinal and stepwise pattern. The nanoribbons are predominantly monolayer and have widths varying from hundreds of nanometers down to tens of nanometers. Most MoSe 2 NRs display an emission profile similar to 2D excitons of MoSe 2 monolayers. In contrast, WS 2 nanoribbons are characterized with sharp emission peaks that can be attributed to the emission from localized excitons or trions. Moreover a broad low energy emission peak can be also observed from some of the WS 2 nanoribbons, which originates from bilayer regions. In this manuscript, we analyze spectral diffusion behavior along with pump power and temperature dependence of the localized exciton emission peaks, shedding light on potential of TMDC nanoribbons in sensing and opto-electronic applications.

Silicon nitride (SiN) is a key material for quantum photonics due to its wide transparency window, high refractive index, low optical losses, and semiconductor foundry compatibility. We study the formation of single-photon emitters in SiN films grown by plasma-enhanced chemical vapor deposition (PECVD), exploring their photophysical properties and dependence on growth conditions. Emitters were observed across the entire range of nitrogen-to-silicon precursor ratios, from silicon-rich to nitrogen-rich conditions, enabled by the low background fluorescence. We demonstrate single-photon emitters in SiN films with a higher refractive index (1.8–1.9) compared to our previous reports (∼1.7). Notably, nitrogen-rich, thinner films yield particularly bright emitters with shorter emission lifetimes, likely due to more efficient annealing. Silicon-rich SiN films exhibit red-shifted emission, suggesting that composition may provide a mechanism for wavelength tuning. These findings establish the feasibility of emitters formation in foundry standard PECVD tools, advancing the scalability and lab-to-fab transition of SiN-based quantum photonic technologies.

Solid-state quantum light sources based on semiconductor quantum dots (QDs) are increasingly employed in photonic quantum information applications. Especially when moving towards real-world scenarios outside shielded lab environments, the efficient and robust coupling of nanophotonic devices to single-mode optical fibers offers substantial advantage by enabling “plug-and-play” operation. In this work we present a fiber-pigtailed cavity-enhanced source of flying qubits emitting single indistinguishable photons at clock-rates exceeding 1 GHz. This is achieved by employing a fully deterministic technique for fiber-pigtailing optimized QD-devices based on hybrid circular Bragg grating (hCBG) micro-cavities. The fabricated fiber-pigtailed hCBGs feature emission lifetimes of < 80 ${< } 80$ ps, corresponding to a Purcell factor of ∼9, a suppression of multi-photon emission events with g (2) (0) < 1 %, a photon-indistinguishability > 80 ${ >} 80$ % and a measured single-photon coupling efficiency of 53 % in a high numerical aperture single-mode fiber, corresponding to 1.2 Megaclicks per second at the single-photon detectors under 80 MHz excitation clock-rates. Furthermore, we show that high multi-photon suppression and indistinguishability prevail for excitation clock-rates exceeding 1 GHz. Our results show that Purcell-enhanced fiber-pigtailed quantum light sources based on hCBG cavities are a prime candidate for applications of quantum information science.

Thin films provide nanoscale confinement together with compatibility with photonic and microwave architectures, making them ideal candidates for chip-scale quantum devices. In this work, we propose a thin film fabrication approach yielding the epitaxial growth of Eu 3+ doped Y 2 O 3 on silicon. We combine two of the most prominent thin film deposition techniques: chemical vapor deposition (CVD) and molecular beam epitaxy (MBE). We report sub-megahertz optical homogeneous linewidths up to 8 K for the Eu 3+ dopants in the film, and lowest value of 270 kHz. This result constitutes a ten-fold improvement with respect to previous reports on the same material, opening promising perspectives for the development of scalable and compact quantum devices containing rare-earth ions.

Europium-doped nanocrystals constitute a promising material for a scalable future quantum computing platform. Long-lived nuclear spin states could serve as qubits addressed via coherent optical transitions. In order to realize an efficient spin-photon interface, we couple the emission from a single nanoparticle to a fiber-based microcavity under cryogenic conditions. The spatial and spectral tunability of the cavity permits us to place individual nanoparticles in the cavity, to measure the inhomogeneous linewidth of the ions, and to show a multi-modal Purcell-enhancement of two transition in Eu 3+ . A halving of the free-space lifetime to 1.0 ms is observed, corresponding to a 140-fold enhancement of the respective transition. Furthermore, we observe a narrow optical linewidth of 3.3 MHz for a few-ion ensemble in the center of the inhomogeneous line. The results represent an important step towards the efficient readout of single Eu 3+ ions, a key requirement for the realization of single-ion-level quantum processing nodes in the solid state.

Charge-trapping defects in crystalline solids play important roles in applications ranging from microelectronics, optical storage, sensing and quantum technologies. On one hand, depleting trapped charges in the host matrix reduces charge noise and enhances coherence of solid-state quantum emitters. On the other hand, stable charge traps can enable high-density optical storage systems. Here we report all-optical control of charge-trapping defects via optical charge trapping (OCT) spectroscopy of a rare-earth ion doped oxide (Y 2 O 3 ). Charge trapping is realized by low intensity optical excitation in the 200–375 nm range. Charge detrapping or depletion is carried out by optically stimulated luminescence (OSL) under 532 nm stimulation. Using a Pr-doped Y 2 O 3 polycrystalline ceramic host matrix, we observe charging pathways via the inter-band optical absorption of Y 2 O 3 and via the 4f-5d transitions of Pr 3+ . We demonstrate effective control of the density of trapped charges within the Y 2 O 3 matrix at ambient environment. These results point to a viable method for controlling the local charge environment in rare-earth doped crystals via all-optical means, and pave the way for further development of efficient optical storage technologies with ultrahigh storage capacity, as well as for the localized control of quantum coherence in rare-earth doped solids.

Nonlinear optical effects such as frequency conversion form the basis for many practical light sources. In a variety of settings, the performance of such sources is limited by quantum noise. In many nonlinear systems, this quantum noise gets strongly amplified, as a result of the large sensitivity of the nonlinear dynamics to changes in the initial conditions − a feature common to many nonlinear systems. Here, we develop a general theory of quantum noise resulting from nonlinear dynamics initiated by many-photon Gaussian quantum states. The theory provides guidelines to find the optimal quantum state to inject to maximally suppress the noise at the output. As a concrete example of the concept and theory, we consider the nonlinear optical phenomenon of supercontinuum generation by a femtosecond pulse, a famously noise-generating process, which is important in a range of applications in materials characterization and life science. By seeding supercontinuum generation with pulsed squeezed vacuum, one can achieve order-of-magnitude magnitude reduction of intensity and phase noise simultaneously, over a broad band of wavelengths, passively, and with no change in spectrum. The large magnitude and bandwidth of this effect is challenging to achieve by other means of stabilization, pointing to a promising approach for controlling quantum noise in a variety of nonlinear systems.

Nonclassical states of light are fundamental in various applications, spanning quantum computation to enhanced sensing. Fast free electrons, which emit light into photonic structures through the mechanism of spontaneous emission, represent a promising platform for generating diverse types of states. Indeed, the intrinsic connection between the input electron wave function and the output light field suggests that electron-shaping schemes, based on light-induced scattering, facilitate their synthesis. In this article, we present a theoretical framework capable of predicting the final optical density matrix emitted by a generic N -electron state that can also account for post-sample energy filtering. By using such a framework, we study the modulation-dependent fluctuations of the N -electron emission and identify regions of superradiant scaling characterized by Poissonian and super-Poissonian statistics. In this context, we predict that high- N modulated electron pulses can yield a tenfold shot-noise suppression in the estimation of the electron-light coupling when the output radiation intensity is analyzed. In the single-electron case, we show how coherent states with nearly 90 % purity can be formed by pre-filtering a portion of the spectrum after modulation, and how non-Gaussian states are generated after a precise energy measurement. Furthermore, we present a strategy combining a single-stage electron modulation and post-filtering to harness tailored light states, such as squeezed vacuum, cat, and triangular cat states, with fidelities close to 100 %.

Second-harmonic generation (SHG) facilitated by plasmonic nanostructures has drawn considerable attention, owing to its efficient frequency up-conversion at the nanoscale and potential applications in on-chip integration and nanophotonic devices. Herein, we present a nanodimer array fabricated by nanoimprinting, composed of nanofinger-pair symmetrically leaning at an off-angle with a well-defined sub-nanometric gap. Commonly, geometric symmetry would suppress the far-field SHG due to the near-field cancelling of symmetric surface SH polarization. However, we find that the light-induced surface SH polarization distribution along the wave-vector of incidence could be influenced by the off-angle, which is consistent to the requirement of SH polarization symmetry-breaking in symmetric metallic nanocavity. A dramatic enhancement of far-field SHG is achieved by tuning the off-angle of nanofinger-pair, even approaching up to over 4 orders of magnitude for an optimal value. The demonstration of SHG enhancement on our well-defined plasmonic nanodimer provides a new way of on-chip integration to activate high-efficient SH radiation, which might be potential for applications in novel nonlinear optical nanodevices with remarkable efficiency and sensitivity.

Solid-state quantum emitters (QE) can produce single photons required for quantum information processing. However, their emission properties often exhibit poor directivity and polarisation definition resulting in considerable loss of generated photons. Here we propose and numerically evaluate Mie metasurface designs for outcoupling photons from an embedded and randomly-positioned QE. These Mie metasurface designs can provide over one order of magnitude enhancement in photon outcoupling with only several percent of photons being lost. Importantly, the Mie metasurfaces provide the enhancement in photon outcoupling without the need for strict QE position alignment and without affecting the intrinsic QE emission rate (Purcell enhancement). Electric dipole modes are key for achieving the enhancement and they offer a path for selective outcoupling for photons emitted with specific polarisation, including the out-of-plane polarisation. Mie metasurfaces can provide an efficient, polarisation-selective and scalable platform for QEs.

Heterogeneously integrated hybrid photonic crystal cavities enable strong light–matter interactions with solid state, optically addressable quantum memories. A key challenge to realizing high quality factor ( Q ) hybrid photonic crystals is the reduced index contrast on the substrate compared to suspended devices in air. This challenge is particularly acute for color centers in diamond because of diamond’s high refractive index, which leads to increased scattering loss into the substrate. Here, we develop a design methodology for hybrid photonic crystals utilizing a detailed understanding of substrate-mediated loss, which incorporates sensitivity to fabrication errors as a critical parameter. Using this methodology, we design robust, high-Q, GaAs-on-diamond photonic crystal cavities, and by optimizing our fabrication procedure, we experimentally realize cavities with Q approaching 30,000 at a resonance wavelength of 955 nm.

Color centers in silicon have recently gained considerable attention as single-photon sources and as spin qubit-photon interfaces. However, one of the major bottlenecks to the application of silicon color centers is their low overall brightness due to a relatively slow emission rate and poor light extraction from silicon. Here, we increase the photon collection efficiency from an ensemble of a particular kind of color center, known as W centers, by embedding them in circular Bragg grating cavities resonant with their zero-phonon-line emission. We observe a ≈5-fold enhancement in the photon collection efficiency (the fraction of photons extracted from the sample and coupled into a single-mode fiber), corresponding to an estimated ≈11-fold enhancement in the photon extraction efficiency (the fraction of photons collected by the first lens above the sample). For these cavities, we observe lifetime reduction by a factor of ≈ 1.3 ${\approx} 1.3$ . For W centers in resonant bowtie-shaped cavities, we observed a ≈3-fold enhancement in the photon collection efficiency, corresponding to a ≈6-fold enhancement in the photon extraction efficiency, and observed a lifetime reduction factor of ≈ 1.1 ${\approx} 1.1$ . The bowtie cavities thus preserve photon collection efficiency and Purcell enhancement comparable to circular cavities while providing the potential for utilizing in-plane excitation methods to develop a compact on-chip light source.

Thin-film lithium niobate (TFLN) has emerged as a promising platform for integrated photonics due to its exceptional material properties. The application of freeform topology optimization to TFLN devices enables the realization of compact designs with complex functionalities and high efficiency. However, the stringent fabrication constraints of TFLN present significant challenges for optimization, particularly in nonlinear photonic devices. In this work, we propose an inverse design methodology that successfully addresses these challenges and demonstrates the development of an efficient freeform TFLN mode converter. The numerically optimized mode converter achieves a transmission efficiency of 67.60 % and a mode purity of 84.58 %. Experimental validation through nonlinear processes, including second harmonic generation and spontaneous parametric down-conversion, shows that the fabricated devices improve the efficiency of these processes by factors of two and three, respectively, compared to devices without freeform designs. The proposed inverse design framework provides a powerful tool for advancing the development of TFLN-based devices, with broad applicability to nonlinear and quantum photonics.

The reliable measurement and accurate control of the temperature within nanophotonic devices is a key prerequisite for their application in both classical and quantum technologies. Established approaches use sensors that are attached in proximity to the components, which only offers a limited spatial resolution and thus impedes the measurement of local heating effects. Here, we, therefore, study an alternative temperature sensing technique that is based on measuring the luminescence of erbium emitters directly integrated into nanophotonic silicon waveguides. To cover the entire temperature range from 295 K to 2 K, we investigate two different approaches: The thermal activation of nonradiative decay channels for temperatures above 200 K and the thermal depopulation of spin and crystal field levels at lower temperatures. The achieved sensitivity is 0.22(4) %/K at room temperature and increases up to 420(50) %/K at approximately 2 K. Within a few-minute measurement interval, we thus achieve a measurement precision that ranges from 0.04(1) K at the lowest studied temperature to 6(1) K at ambient conditions. In the future, the measurement time can be further reduced by optimizing the excitation pulse sequence and the fiber-to-chip coupling efficiency. Combining this with spatially selective implantation promises precise thermometry from ambient to cryogenic temperatures with a spatial resolution down to a few nanometers.

We study the collective photon decay of multiple quantum emitters embedded in a thin high-index dielectric layer such as hexagonal boron nitride (hBN), with and without a metal substrate. We first explore the significant role that guided modes including surface plasmon modes play in the collective decay of identical single-photon emitters (super- and subradiance). Surprisingly, on distances relevant for collective emission, the guided or surface-plasmon modes do not always enhance the collective emission. We identify configurations with inhibition, and others with enhancement of the dipole interaction due to the guided modes. We interpret our results in terms of local and cross densities of optical states. In the same structure, we show a remarkably favorable configuration for enhanced Förster resonance energy transfer between a donor and acceptor in the dielectric layer on a metallic substrate. We compare our results to theoretical limits for energy transfer efficiency.

Classical coupled harmonic oscillator models are capable of describing the optical and infrared response of nanophotonic systems where a cavity photon couples to dipolar matter excitations. The distinct forms of coupling adopted in these classical models lead to different results in the ultrastrong coupling regime. To clarify the specific classical model required to address particular configurations, we establish a connection between each oscillator model and the equivalent cavity Quantum Electrodynamics description. We show that the proper choice of coupled harmonic oscillator model depends on the presence or absence of the diamagnetic term in the quantum models, linked to whether transverse or longitudinal electromagnetic fields mediate the coupling. This analysis also shows how to exploit the classical oscillator models to extract measurable information of the optical response, as demonstrated in three canonical photonic systems, and to describe the opening of the Reststrahlen band in the bulk dispersion of phononic materials.

We present a study of hybrid light–matter excitations in cavity QED materials using the Dicke–Ising model as a theoretical framework. Leveraging linear response theory, we derive the exact excitations of the system in the thermodynamic limit. Our results demonstrate that the cavity can localize spin excitations, leading to the formation of bound polaritons, where the cavity acts as an impurity of the two-excitation band, localizing spin-wave pairs around single-spin domains. We derive the condition for the existence of these bound states and discuss its satisfiability in different regimes. Finally, we show that these effects persist in finite systems using exact-diagonalization calculations.

Plasmonic nanocavities enable access to the quantum properties of matter but are often simplified to single mode models despite their complex multimode structure. Here, we show that off-resonant plasmonic modes in fact play a crucial role in strong coupling and determine the onset of a novel collective interaction. Our analysis reveals that n strongly coupled plasmonic modes introduce up to n ( n + 1)/2 oscillation frequencies that depend on their coupling strengths and detuning’s from the quantum emitter. Furthermore, we identify three distinct regions as the coupling strength increases: (1) single mode, (2) multimode and (3) collective multimode strong coupling. Our findings enhance the understanding of quantum dynamics in realistic plasmonic environments and demonstrate their potential to achieve ultra-fast energy transfer in light-driven quantum technologies.

Photonic quantum metrology enables the measurement of physical parameters with precision surpassing classical limits by using quantum states of light. However, generating states providing a large metrological advantage is hard because standard probabilistic methods suffer from low generation rates. Deterministic protocols using non-linear interactions offer a path to overcome this problem, but they are currently limited by the errors introduced during the interaction time. Thus, finding strategies to minimize the interaction time of these non-linearities is still a relevant question. In this work, we introduce and compare different deterministic strategies based on continuous and programmable Jaynes–Cummings and Kerr-type interactions, aiming to maximize the metrological advantage while minimizing the interaction time. We find that programmable interactions provide a larger metrological advantage than continuous operations at the expense of slightly larger interaction times. We show that while for Jaynes–Cummings non-linearities the interaction time grows with the photon number, for Kerr-type ones it decreases, favoring the scalability to big photon numbers. Finally, we also optimize different measurement strategies for the deterministically generated states based on photon-counting and homodyne detection.

Converting phonons to photons with optomechanical interaction provides a pathway to realize single phonon counting, which is instrumental in the quantum applications of mechanical systems such as entanglement generation, thermometry, and study of macroscopic quantum phenomenon. In this process, the key requirement is high-extinction, narrow-bandwidth, and stable filtering of the parametric optical pump. Here, we propose to lift this necessity by counting fluorescence emission from a rare earth embedded optomechanical cavity. By doing so, we show that an equivalent filtering effect can be achieved due to spectral hole burning and cavity Purcell effect. To demonstrate this, we designed, fabricated, and characterized an integrated piezo-optomechanical Fabry–Perot cavity on the erbium-doped thin-film lithium niobate platform. By collecting fluorescence from the optomechanical sideband, we show that 93 dB suppression of the pump can be achieved with 10 dB loss of signal, resulting in an increase of 83 dB in sideband-pump ratio. Our results facilitate a route to realize filterless single phonon counting and also create new opportunities to study the interaction between solid state emitters and mechanical systems.

Cathodoluminescence microscopy is now a well-established and powerful tool for probing the photonic properties of nanoscale materials, but in many cases, nanophotonic materials are easily damaged by the electron-beam doses necessary to achieve reasonable cathodoluminescence signal-to-noise ratios. Two-dimensional materials have proven particularly susceptible to beam-induced modifications, yielding both obstacles to high spatial-resolution measurement and opportunities for beam-induced patterning of quantum photonic systems. Here pan-sharpening techniques are applied to cathodoluminescence microscopy in order to address these challenges and experimentally demonstrate the promise of pan-sharpening for minimally-perturbative high-spatial-resolution spectrum imaging of beam-sensitive materials.