Band 12, Heft 23

Metasurfaces, composed of artificial meta-atoms of subwavelength size, can support strong light–matter interaction based on multipolar resonances and plasmonics, hence offering the great capability of empowering nonlinear generation. Recently, owing to their ability to manipulate the amplitude and phase of the nonlinear emission in the subwavelength scale, metasurfaces have been recognized as ultra-compact, flat optical components for a vast range of applications, including nonlinear imaging, quantum light sources, and ultrasensitive sensing. This review focuses on the recent progress on nonlinear metasurfaces for those applications. The principles and advances of metasurfaces-based techniques for image generation, including image encoding, holography, and metalens, are investigated and presented. Additionally, the overview and development of spontaneous photon pair generation from metasurfaces are demonstrated and discussed, focusing on the aspects of photon pair generation rate and entanglement of photon pairs. The recent blossoming of the nonlinear metasurfaces field has triggered growing interest to explore its ability to efficiently up-convert infrared images of arbitrary objects to visible images and achieve spontaneous parametric down-conversion. This recently emerged direction holds promising potential for the next-generation technology in night-vision, quantum computing, and biosensing fields.

We experimentally investigated the asymmetric dual-grating-gate plasmonic terahertz (THz) detector based on an InGaAs-channel high-electron-mobility transistor (HEMT) in the gate-readout configuration. Throughout the THz pulse detection measurement on the fabricated device, we discovered a new detection mechanism called the “3D rectification effect” at the positive gate bias application, which is a cooperative effect of the plasmonic nonlinearities in the channel with the diode nonlinearity in the heterobarrier between the InGaAs channel layer and the InAlAs spacer/carrier-supply/barrier layers, resulting in a giant enhancement of the detector responsivity. We also found that an undesired long-tail waveform observed on the temporal pulse photoresponse of the device is due to trapping of carriers to the donor levels in the silicon δ -doped carrier-supply layer when they tunnel through the barrier to the gate and can be eliminated completely by introducing the so-called inverted-HEMT structure. The internal current responsivity and noise-equivalent power are estimated to be 0.49 A/W (with the equivalent voltage responsivity of 4.9 kV/W with a high output impedance of 10 kΩ) and 196 pW/√Hz at 0.8 THz. These results pave the way towards the application of the plasmonic THz detectors to beyond-5G THz wireless communication systems.

Controlling coherent light–matter interactions in semiconductor microcavities is at the heart of the next-generation solid-state polaritonic devices. Organic–inorganic hybrid perovskites are potential materials for room-temperature polaritonics owing to their high exciton oscillator strengths and large exciton binding energies. Herein, we report on strong exciton-photon coupling in the micro-platelet and micro-ribbon shaped methylammonium lead bromide single crystals. Owing to high crystallinity and large refractive index, the as-grown perovskite microcrystals serve as self-hybridized optical microcavities along different orientations due to their distinct physical dimensionalities. In this regard, the perovskite micro-platelet forms a simple Fabry–Perot microcavity in out-of-plane orientation, while the micro-ribbon functions as a Fabry–Perot type waveguide microcavity within the plane of the perovskite sample. Consequently, excitons in these microcavities strongly interact with their corresponding uncoupled cavity modes, yielding multimode exciton-polaritons with Rabi splitting energies ∼205 and 235 meV for micro-platelet and micro-ribbon geometry, respectively. Furthermore, micro-ribbon geometry displays Young’s double-slit-like interference patterns, which together with the numerical simulation readily reveals the parity and the mode order of the uncoupled cavity modes. Thus, our results not only shed light on strong exciton-photon coupling in various morphologies of methylammonium lead bromide microcrystals but also open an avenue for advanced polaritonic devices.

A light source with narrowband, sufficient brightness, and low spatial coherence is required for certain applications such as optical imaging and free-space optical communication. In this study, our focus was to investigate a novel imaging laser source, specifically a low-threshold random laser enhanced by TiN nanoparticles. The results demonstrate that the random laser spectrum exhibits an impressive bandwidth of 0.23 nm, accompanied by an incredibly low spatial coherence factor of merely 0.15. Due to the low spatial coherence of random laser, the speck contrast is less than 0.02 when the light passes through a scattering system. Notably, when compared to traditional lasers, the use of a random laser yields significantly superior imaging quality in both scatterless and complex scattering environments. This finding highlights the immense potential of the random laser as a narrowband and low spatial coherence laser source for robust speckle-free imaging applications, particularly in environments with intricate scattering phenomena. Furthermore, this breakthrough can be extended to various other domains, including free-space optical communication.

Graphene aerogels have implied great potential for electromagnetic wave absorption. However, the investigation of their design for broadband absorption in the terahertz (THz) range remains insufficient. Here, we propose an anisotropic honeycomb stack metamaterial (AHSM) based on graphene to achieve ultrawideband THz absorption. The absorption mechanism is elucidated using the effective medium method, offering deeper physics insights. At low THz frequencies, the impedance matching from the air to the AHSM can be improved by reducing the chemical potential of graphene for high absorption. There is a suppression of absorption at the intermediate frequencies due to constructive interference, which can be avoided by shortening the sizes of honeycomb edges. With the aim to elevate absorption at high frequencies, one can increase the stack layer number to enhance multiple reflections and destructive interference within the metastructure. Based on the above principles, we design an AHSM that achieves a broadband absorbance of over 90 % from 1 THz to 10 THz. This absorption can tolerate a wide range of incident angles for both TE and TM wave excitations. Our research will provide a theoretical guide to future experimental exploration of graphene aerogels for THz metamaterial absorber applications.

Highly stable pulsed fiber lasers are key optical components in optical communication, optical sensing, and precision micromachining systems due to the high beam quality, high peak power, and compact configurations. However, the available optical modulators in the fiber laser suffer from the operation bandwidth limitations and poor long-term physicochemical stability. Here, we have investigated the broadband nonlinear optical absorption behavior of the chromium iodide (CrI 3 ) film, which exhibits broadband saturable absorption towards the mid-infrared regime and excellent long-term stability. The conventional soliton fiber laser operating at telecom wavelength has been obtained from an Er 3+ -doped fiber laser (EDFL) utilizing CrI 3 film with a signal-to-noise ratio (SNR) of 92.4 dB and a pulse width of 492 fs. In addition, a passively Q-switched operation around 2.8 μm has also been obtained from an Er 3+ -doped ZBLAN fiber laser (EDZFL) modulated by the CrI 3 film with a SNR of 46.8 dB and a pulse width of 766 ns. The demonstration shows that the CrI 3 film exhibits robust broadband optical modulation, and may make inroads for developing highly stable ultrafast optoelectronic devices.

As a high-degree-of-freedom approach to manipulate the electromagnetic wave, metasurfaces are widely used in high-capacity information technology. Extensive investigations have explored multiplexing techniques using polarization, incident angle, wavelength, and infinite-dimensional multiplexing through Orbital Angular Momentum (OAM). However, due to the limited spatial resolution and array size of the metasurface, the number of multiplexing channels that can be actually realized is limited. Therefore, research on the combination of OAM multiplexing and polarization degrees of freedom is of great significance. Here, we propose and experimentally demonstrate a metasurface holography multiplexing scheme based on multiple polarization channels combined with OAM. Taking advantage of the orthogonal independence of spin angular momentum and orbital angular momentum, multiple OAM multiplexing holograms are constructed in multiple different spin-polarization channels. Utilizing the well-established compatibility between OAM multiplexing and polarization multiplexing, we successfully integrated two multiplane holograms and 15 OAM multiplexing holograms on a single metasurface. Subsequently, we introduced an optical nested encryption framework designed for parallel communication. This work facilitates high-capacity and high-security holography by employing multiplexing metasurfaces, thereby providing innovative design concepts for optical communication, information encryption, and related domains.

In structured light tweezers, it is a challenging technical issue to realize the complete circular motion of the trapped particles parallel to the optical axis. Herein, we propose and generate a novel optical skipping rope via combining beam shaping technology, Fourier shift theorem, and beam grafting technology. This optical skipping rope can induce the transverse orbital angular momentum (OAM) (i.e., nominal OAM, whose direction is perpendicular to the optical axis) and transfer it to the particles, so that the particles have a transverse torque, thereby causing the particles to rotate parallel to the optical axis. Experimentally, our optical tweezers validate that the designed optical skipping rope realizes the orbital motion of polystyrene particles parallel to the optical axis. Additionally, the experiments also demonstrate that the optical skipping ropes manipulate particles to move along the oblique coil trajectory and three-dimensional (3D) cycloidal trajectory. Using the laser beam induced OAM, this innovative technology increases the degree of freedom for manipulating particles, which is of great significance for the application of optical tweezers in optical manipulation, micromechanics, and mimicry of celestial orbits.

Multidimensional manipulation of photonic spin Hall effect (PSHE) has attracted considerable interest due to its potential in a wide variety of spin-based applications. Plenty of research efforts have been devoted to transverse or longitudinal spin-dependent splitting; however, the splitting pattern that can self-rotate in a three-dimensional (3-D) space appears to be missing in literature. In this paper, we introduce a novel 3-D rotational PSHE, which can be realized and tuned using well-designed Pancharatnam–Berry phase metasurfaces. To demonstrate this phenomenon, we first show that when a single dielectric metasurface is used, the lobe-structured spin-splitting patterns on the transverse planes rotate and evolve along the propagation path. Then, we present that under two cascaded metasurfaces, the rotation angle of the splitting patterns are tunable by adjusting the relative rotation angle between the two metasurfaces. Finally, we manifest that the lobe number of the two spin-dependent splitting patterns can be independently controlled once we introduce a dynamic phase, which produces an asymmetrical rotational PSHE. The demonstrated phenomena can be used to achieve active manipulation of spin photons in multiple dimensions, and the developed device might find potential applications in various areas, e.g., optical microscopy.

Spectrometer miniaturization is desired for handheld and portable applications, yet nearly no miniaturized spectrometer is reported operating within terahertz (THz) waveband. Computational strategy, which can acquire incident spectral information through encoding and decoding it using optical devices and reconstruction algorithms, respectively, is widely employed in spectrometer miniaturization as artificial intelligence emerges. We demonstrate a computational miniaturized THz spectrometer, where a plasmonic filter array tailors the spectral response of a blocked-impurity-band detector. Besides, an adaptive deep-learning algorithm is proposed for spectral reconstructions with curbing the negative impact from the optical property of the filter array. Our spectrometer achieves modest spectral resolution (2.3 cm −1 ) compared with visible and infrared miniaturized spectrometers, outstanding sensitivity (e.g., signal-to-noise ratio, 6.4E6: 1) superior to common benchtop THz spectrometers. The combination of THz optical devices and reconstruction algorithms provides a route toward THz spectrometer miniaturization, and further extends the applicable sphere of the THz spectroscopy technique.