Measurement of spectrum-averaged cross sections of the (n,p) and (n,n′) reactions on strontium by fast neutrons of a TRIGA reactor: comparison with integrated data from excitation functions of various data libraries
-
M. Shuza Uddin
, M. Mezbah Uddin
Abstract
Integral cross sections of the reactions 84Sr(n,p)84Rb, 86Sr(n,p)86Rb and 87Sr(n,n′)87mSr, over the fast neutron spectrum of a TRIGA reactor above 0.5 MeV, were measured for the first time. The results were used for integral tests of the evaluated excitation functions in the data libraries, ENDF/B-VIII.0, ROSFOND-2010, JEFF-3.3, JENDL-5 and TENDL-2021. The integral measurements are generally consistent with the integrated values within 12 %, except for a few cases. The two data libraries ENDF/B-VIII.0 and ROSFOND-2010 appear to need some improvement with regard to the reactions investigated in this work.
Acknowledgements
The authors thank the operation crew of the TRIGA Mark II nuclear reactor, Savar, Dhaka, for their help in performing irradiations of samples. M.S. Uddin wants to thank the head of ENRPD for permission to use gamma-ray counting system.
-
Author contributions: All the authors have accepted responsibility for the entire content of this submitted manuscript and approved submission.
-
Research funding: None declared.
-
Conflict of interest statement: The authors declare no conflicts of interest regarding this article.
References
1. Uddin, M. S., Sudár, S., Hossain, S. M., Khan, R., Zulquarnain, M. A., Qaim, S. M. Fast neutron spectrum unfolding of a TRIGA Mark II reactor and measurement of spectrum-averaged cross sections: integral tests of differential cross sections of neutron threshold reactions. Radiochim. Acta 2013, 101, 613–620; https://doi.org/10.1524/ract.2013.2073.Suche in Google Scholar
2 Uddin, M. S., Zaman, M. R., Hossain, S. M., Qaim, S. M. Radiochemical measurement of neutron-spectrum averaged cross sections for the formation of 64Cu and 67Cu via the (n,p) reaction at a TRIGA Mark-II reactor: feasibility of simultaneous production of the theragnostic pair 64Cu/67Cu. Radiochim. Acta 2014, 102, 473–480.10.1515/ract-2013-2199Suche in Google Scholar
3. Uddin, M. S., Rafee, K. A., Hossain, S. M., Khan, R., Qaim, S. M. Integral measurement of spectrum-averaged cross sections of a few threshold reactions induced by fast neutrons of a TRIGA reactor: comparison with integrated data from excitation functions given in various data libraries. Radiochim. Acta 2020, 108, 511–516; https://doi.org/10.1515/ract-2019-3212.Suche in Google Scholar
4. Calamand, A. Cross sections for fission neutron spectrum induced reactions. In Handbook on Nuclear Activation Cross Sections. Technical Report No. 156; IAEA: Vienna, 1974, p. 273.Suche in Google Scholar
5. Molla, N. I., Qaim, S. M. A systematic study of (n,p) reactions at 14.7 MeV. Nucl. Phys. A 1977, 283, 269.10.1016/0375-9474(77)90431-6Suche in Google Scholar
6. Konno, C., Ikeda, Y., Oishi, K., Kawade, K., Yamamoto, H., Maekawa, H. Activation cross section measurements at neutron energy from 13.3 to 14.9 MeV. JAERI Reports No. 1329, 1993.Suche in Google Scholar
7. He, G., Luo, J., Liu, Z., Kong, X. Cross-section measurements for (n,2n), (n,p) and (n,α) reactions on strontium at the neutron energy about 14 MeV. Ann. Nucl. Energy 2006, 33, 37–42; https://doi.org/10.1016/j.anucene.2005.09.001.Suche in Google Scholar
8. Bayhurst, B. P., Prestwood, R. J. (n,p) and (n,α) excitation functions of several nuclei from 7.0 to 19.8 MeV. J. Inorg. Nucl. Chem. 1961, 23, 173–185.10.1016/0022-1902(61)80244-3Suche in Google Scholar
9. Kayashima, K., Nagao, A., Kumabe, I. Activation cross section on Ti, Mn, Cu, Zn, Sr, Y, Cd, In and Te for 14.6 neutrons. Japanese report to NEANDC No. 61U, 1979; p. 94.Suche in Google Scholar
10. Levkovskii, V. N., Kovelskaya, G. E., Vinitskaya, G. P., Stepanov, V. M., Sokolskii, V. V. Cross sections of the (n,p) and (n,alpha) reactions at 14.8 MeV. Soviet J. Nucl. Phys. 1969, 8, 4.Suche in Google Scholar
11. Levkovskii, V. N. Empirical behavior of the (n,p) reaction cross-sections for 14–15 MeV neutrons. J. Exper. Theor. Phys. 1964, 18, 213.Suche in Google Scholar
12. Strohal, P., Cindro, N., Eman, B. Reaction mechanism and shell effects from the interaction of 14.6 MeV neutrons with nuclei. Nucl. Phys. 1962, 30, 49; https://doi.org/10.1016/0029-5582(62)90031-7.Suche in Google Scholar
13. Koning, A. J., Rochman, D., Sublet, J.-C., Dzysiuk, N., Fleming, M., van der Marck, S. TENDL: complete nuclear data library for innovative nuclear science and technology. Nucl. Data Sheets 2019, 155, 1; https://doi.org/10.1016/j.nds.2019.01.002.Suche in Google Scholar
14. Brown, D. A., Chadwick, M. B., Capote, R., Kahler, A. C., Trkov, A., Herman, M. W., Sonzogni, A. A., Danon, Y., Carlson, A. D., Dunn, M., Smith, D. L., Hale, G. M., Arbanas, G., Arcilla, R., Bates, C. R., Beck, B., Becker, B., Brown, F., Casperson, R. J., Conlin, J., Cullen, D. E., Descalle, M.-A., Firestone, R., Gaines, T., Guber, K. H., Hawari, A. I., Holmes, J., Johnson, T. D., Kawano, T., Kiedrowski, B. C., Koning, A. J., Kopecky, S., Leal, L., Lestone, J. P., Lubitz, C., Márquez Damián, J. I., Mattoon, C. M., McCutchan, E. A., Mughabghab, S., Navratil, P., Neudecker, D., Nobre, G. P. A., Noguere, G., Paris, M., Pigni, M. T., Plompen, A. J., Pritychenko, B., Pronyaev, V. G., Roubtsov, D., Rochman, D., Romano, P., Schillebeeckx, P., Simakov, S., Sin, M., Sirakov, I., Sleaford, B., Sobes, V., Soukhovitskii, E. S., Stetcu, I., Talou, P., Thompson, I., van der Marck, S., Welser-Sherrill, L., Wiarda, D., White, M., Wormald, J. L., Wright, R. Q., Zerkle, M., Zerovnik, G., Zhu1, Y. ENDF/B-VIII.0: the 8th major release of the nuclear reaction data library with CIELO-project cross sections, new standards and thermal scattering data. Nucl. Data Sheets 2018, 148, 1; https://doi.org/10.1016/j.nds.2018.02.001.Suche in Google Scholar
15. Russian File of Evaluated Neutron Data, released 2010, ROSFOND-2010. http://www.ippe.ru/podr/abbn/english/libr/rosfond.php.Suche in Google Scholar
16. Plompen, A. J. M., Cabellos, O., De Saint Jean, C., Fleming, M., Algora, A., Angelone, M., Archier, P., Bauge, E., Bersillon, O., Blokhin, A., Cantargi, F., Chebboubi, A., Diez, C., Duarte, H., Dupont, E., Dyrda, J., Erasmus, B., Fiorito, L., Fischer, U., Flammini, D., Foligno, D., Gilbert, M. R., Granada, J. R., Haeck, W., Hambsch, F.-J., Helgesson, P., Hilaire, S., Hill, I., Hursin, M., Ichou, R., Jacqmin, R., Jansky, B., Jouanne, C., Kellett, M. A., Kim, D. H., Kim, H. I., Kodeli, I., Koning, A. J., Konobeyev, A.Y., Kopecky, S., Kos, B., Krása, A., Leal, L. C., Leclaire, N., Leconte, P., Lee, Y. O., Leeb, H., Litaize, O., Majerle, M., Márquez, J., Damián, I., Michel-Sendis, F., Mills, R. W., Morillon, B., Noguère, G., Pecchia, M., Pelloni, S., Pereslavtsev, P., Perry, R. J., Rochman, D., Röhrmoser, A., Romain, P., Romojaro, P., Roubtsov, D., Sauvan, P., Schillebeeckx, P., Schmidt, K. H., Serot, O., Simakov, S., Sirakov, I., Sjöstrand, H., Stankovskiy, A., Sublet, J. C., Tamagno, P., Trkov, A., van der Marck, S., Álvarez-Velarde, F., Villari, R., Ware, T. C., Yokoyama, K., Žerovnik, G.: The joint evaluated fission and fusion nuclear data library, JEFF-3.3. Eur. Phys. J. 2020, A56, 181; https://doi.org/10.1140/epja/s10050-020-00141-9.Suche in Google Scholar
17. Iwamoto, O., Iwamoto, N., Kunieda, S., Minato, F., Nakayama, S., Abe, Y., Tsubakihara, K., Okumura, S., Ishizuka, C., Yoshida, T., Chiba, S., Otuka, N., Sublet, J.-C., Iwamoto, H., Yamamoto, K., Nagaya, Y., Tada, K., Konno, C., Matsuda, N., Yokoyama, K., Taninaka, H., Oizumi, A., Fukushima, M., Okita, S., Chiba, G., Sato, S., Ohta, M., Kwon, S. Japanese evaluated nuclear data library version 5: JENDL-5. J. Nucl. Sci. Technol. 2023, 60, 1; https://doi.org/10.1080/00223131.2022.2141903.Suche in Google Scholar
18. Fitzgerald, J. JF Computing Services, 17 Chapel Road, Stanford in the Vale, Oxfordshire, SN7 8LE; Copyright © Jim Fitzgerald, 1991–2016. Last updated 8th October 2016.Suche in Google Scholar
19. Abriola, D., Abriola, D., Bostan, M., Erturk, S., Fadil, M., Galan, M., Juutinen, S., Kibédi, T., Kondev, F., Luca, A., Negret, A., Nica, N., Pfeiffer, B., Singh, B., Sonzogni, A., Timar, J., Tuli, J., Venkova, T., Zuber, K. Nuclear data sheets for A = 84. Nucl. Data Sheets 2009, 110, 2815; https://doi.org/10.1016/j.nds.2009.10.002.Suche in Google Scholar
20. Johnson, T. D., Kulp, W. D. Nuclear data sheets for A = 87. Nucl. Data Sheets 2015, 129, 1; https://doi.org/10.1016/j.nds.2015.09.001.Suche in Google Scholar
21. Negret, A., Singh, B. Nuclear data sheets for A = 86. Nucl. Data Sheets 2015, 124, 1; https://doi.org/10.1006/ndsh.2001.0017.Suche in Google Scholar
22. Nesaraja, C., Geraedts, D. S., Singh, B. Nuclear data sheets for A = 58. Nucl. Data Sheets 2010, 111, 897; https://doi.org/10.1016/j.nds.2010.03.003.Suche in Google Scholar
23. Huang, X., Kang, M. Nuclear data sheets for A = 198. Nucl. Data Sheets 2016, 133, 221; https://doi.org/10.1016/j.nds.2016.02.002.Suche in Google Scholar
24. NuDat3. Decay Radiation Database version of 2023; National Nuclear Data Center. https://www.nndc.bnl.gov/nudat3/.Suche in Google Scholar
25. Trkov, A., Griffin, P. J., Simakov, S. P., Greenwood, L. R., Zolotarev, K. I., Capote, R., Aldama, D. L., Chechev, V., Destouches, C., Kahler, A. C., Konno, C., KoštálM., Majerle, M., Malambu, E., Ohta, M., Pronyaev, V. G., Radulovic, V., Sato, S., Schulc, M., SimečkováE., Vavtar, I., Wagemans, J., White, M., Yashima, H. IRDFF-II: a new neutron metrology library. Nucl. Data Sheets 2020, 163, 1; https://doi.org/10.1016/j.nds.2019.12.001.Suche in Google Scholar
26. Farina Arbocco, F., Vermaercke, P., Smits, K., Sneyers, L., Strijckmans, K. Experimental determination of k0, Q0 factors, effective resonance energies and neutron cross-sections for 37 isotopes of interest in NAA. J. Radioanal. Nucl. Chemistry 2014, 302, 655; https://doi.org/10.1007/s10967-014-3281-0.Suche in Google Scholar
27. Krane, K. S. Cross sections and isomer ratios in the Rb(n,γ) and Sr(n,γ) reactions. Eur. Phys. J. A 2021, 57, 19; https://doi.org/10.1140/epja/s10050-020-00299-2.Suche in Google Scholar
28. Mannhart, W., Vonach, H. Isomeric cross section ratios for the 2-P-1/2 and 1-G-9/2 shell model states formed by thermal neutron capture. Zeitschrift fuer Physik 1968, 210, 13; https://doi.org/10.1007/bf01379867.Suche in Google Scholar
29. Foglio Para, A., Mandelli Bettoni, M. Isomeric cross section ratios for some reactions. Energia Nucleare (Milan) 1967, 14, 228.Suche in Google Scholar
30. Hans, H. S., Sehgal, M. L., Gill, P. S. Thermal neutron cross sections for producing isomers (II). Nucl. Phys. 1960, 20, 183; https://doi.org/10.1016/0029-5582(60)90168-1.Suche in Google Scholar
31. Kramer, H. H., Wahl, W. H. Formation of Se-77m, Sr-87m, Cd-111m, and Ba-137m by reactor spectrum neutrons for use in activation analysis. Nucl. Sci. Eng. 1965, 22, 373; https://doi.org/10.13182/nse65-a20941.Suche in Google Scholar
32. Van der Linden, R., De Corte, F., Van Den Winkel, P., Hoste, J. A compilation of infinite dilution resonance integrals. J. Radioanal. Nucl. Chem. 1972, 11, 133; https://doi.org/10.1007/bf02518625.Suche in Google Scholar
33. Heft, R. E. A consistent set of nuclear-parameter values for absolute instrumental neutron activation analysis. In Conference on Computers in Activation Analysis, Mayaguez; Carpenter, B. S., D’Agostino, M. D., Yule, H. P., Eds. Department of Energy: Washington, DC, 1979; pp. 495–510.Suche in Google Scholar
34. Simonits, A., De Corte, F., El Nimr, T., Moens, L., Hoste, J. Comparative study of measured and critically evaluated resonance integral to thermal cross-section ratios. Part II. J. Radioanal. Nucl. Chem. 1984, 81, 397; https://doi.org/10.1007/bf02135391.Suche in Google Scholar
© 2023 Walter de Gruyter GmbH, Berlin/Boston
Artikel in diesem Heft
- Frontmatter
- Original Papers
- Excitation functions of the 197Au(p,pxn) and 197Au(p,xn) reactions
- Measurement of spectrum-averaged cross sections of the (n,p) and (n,n′) reactions on strontium by fast neutrons of a TRIGA reactor: comparison with integrated data from excitation functions of various data libraries
- Extraction of uranium and rare earths from mineralized ferruginous sandstone, southwestern Sinai
- Cesium ion removal from low-level radioactive wastewater utilizing synthesized cobalt hexacyanoferrate-sand composite
- Separation of 71,72As from alpha-particle induced reaction on gallium oxide target using naturally occurring alkaloid caffeine
- Quality characteristics of white button mushrooms (Agaricus bisporus) affected by gamma irradiation and volatile oils during storage
- A closer inspection of the structural, mechanical, optical and radiation shielding properties of GeO2-doped magnesium-telluroborate glasses
Artikel in diesem Heft
- Frontmatter
- Original Papers
- Excitation functions of the 197Au(p,pxn) and 197Au(p,xn) reactions
- Measurement of spectrum-averaged cross sections of the (n,p) and (n,n′) reactions on strontium by fast neutrons of a TRIGA reactor: comparison with integrated data from excitation functions of various data libraries
- Extraction of uranium and rare earths from mineralized ferruginous sandstone, southwestern Sinai
- Cesium ion removal from low-level radioactive wastewater utilizing synthesized cobalt hexacyanoferrate-sand composite
- Separation of 71,72As from alpha-particle induced reaction on gallium oxide target using naturally occurring alkaloid caffeine
- Quality characteristics of white button mushrooms (Agaricus bisporus) affected by gamma irradiation and volatile oils during storage
- A closer inspection of the structural, mechanical, optical and radiation shielding properties of GeO2-doped magnesium-telluroborate glasses