Degradation of methyl orange using dielectric barrier discharge water falling film reactor
-
Baowei Wang
,
Meng Xu
Abstract
The dielectric barrier discharge (DBD) technique based cylindrical water falling film reactor was used for degrading an azo dye methyl orange (MO). The primary conditions affecting the degradation of methyl orange were systematically investigated. After 30 min plasma treatment, the degradation rate of MO was as high as 93.7% with gas velocity of 300 mL/min and the input energy of 72.5W. The influences of initial pH and conductivity of MO solution were also explored. The results indicated that the optimum pH value was 3.02 and 99.1% removal of MO was achieved within 30 min. Three catalytic systems DBD/Fe2+, DBD/PS (persulfate) and DBD/Fe2+/PS were examined to improve the degradation rate and the chemical oxygen demand (COD) removal rate of MO. The highest degradation rate (100%) and COD removal rate (72.4%) happened in DBD/Fe2+/PS system. The degradation products were analyzed by LC-MS in DBD system and DBD/Fe2+/PS system respectively, and then the possible degradation pathways of MO were proposed.
Acknowledgement
Financial supports from the National Key R&D Program of China (2016YFB0600701) are gratefully acknowledged.
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Artikel in diesem Heft
- Editorial
- Excitation Kinetics of Oxygen O(1D) State in Low-Pressure Oxygen Plasma and the Effect of Electron Energy Distribution Function
- Using amino-functionalized Fe3O4-WO3 nanoparticles for diazinon removal from synthetic and real water samples in presence of UV irradiation
- Treatment of high salinity wastewater using CWPO process for reuse
- Electrochemical Advanced Oxidation Processes (EAOP) to degrade per- and polyfluoroalkyl substances (PFASs)
- Effect of feedstock impurities on activity and selectivity of V-Mo-Nb-Te-Ox catalyst in ethane oxidative dehydrogenation
- Photocatalytic Degradation of Azo Dyes Over Semiconductors Supported on Polyethylene Terephthalate and Polystyrene Substrates
- Effects of calcination temperature on sol-gel synthesis of porous La2Ti2O7 photocatalyst on degradation of Reactive Brilliant Red X3B
- ClO2-oxidation-based demulsification of oil-water transition layer in oilfields: An experimental study
- Semi-permanent hair dyes degradation at W/WO3 photoanode under controlled current density assisted by visible light
- Degradation of PVA (polyvinyl alcohol) in wastewater by advanced oxidation processes
- Degradation of imidacloprid insecticide in a binary mixture with propylene glycol by conventional fenton process
- Gemini surfactant-assisted synthesis of BiOBr with superior visible light-induced photocatalytic activity towards RhB degradation
- Photocatalytic paraquat degradation over TiO2 modified by hydrothermal technique in alkaline solution
- Enhancement of Profenofos Remediation Using Stimulated Bioaugmentation Technique
- Mechanistic insight on the sonolytic degradation of phenol at interface and bulk using additives
- Biosolubilization of low-grade rock phosphate by mixed thermophilic iron-oxidizing bacteria
- Degradation of methyl orange using dielectric barrier discharge water falling film reactor
- Rapid prediction of hydrogen peroxide concentration eletrogenerated with boron doped diamond electrodes
