Startseite Analysis of the dynamics of laser induced plume propagation from liquid matrix using fast photography
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Analysis of the dynamics of laser induced plume propagation from liquid matrix using fast photography

  • Xing Fan EMAIL logo , Jian Xiao , Guang-Zhou Hu , Yun-Peng Zhao , Shi-Gang Kang EMAIL logo , Jin-Li Lu und Hong-Ru Fan
Veröffentlicht/Copyright: 2. Februar 2016
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Chemical Papers
Aus der Zeitschrift Chemical Papers Band 70 Heft 6

Abstract

Glycerol, a liquid matrix material for matrix-assisted laser desorption ionization mass spectrometry, was irradiated by a tunable pulsed infrared laser at wavelengths of 2.80 μm, 2.94 μm, 3.10 μm and 3.50 μm, covering the OH and CH stretch vibrations. A fast photography system was introduced to analyze the dynamic process of plume propagation induced by laser ablation up to 1000 μs of the delay time. Propagation distance of the plume front was measured and the corresponding velocities were calculated; they varied with the wavelength and decreased with the delay time. At the tunable wavelength of the peak of the OH absorption (3.0 μm), theoretical calculations indicate that energy deposition from the pulsed laser is in the regime of stress confinement. The mode of energy deposition depends on the wavelength of the OH vibration and its distance from the absorption maxima. However, stages after a 10 μs delay at various wavelengths show a certain similarity in the distance of plume propagation, which can be well fitted by a drag model.

Keywords: laser ablation; fast photography; plume propagation; dynamics analysis; drag model

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Received: 2015-6-28
Revised: 2015-11-5
Accepted: 2015-11-26
Published Online: 2016-2-2
Published in Print: 2016-6-1

© 2016 Institute of Chemistry, Slovak Academy of Sciences

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https://doi.org/10.1515/chempap-2016-0012
Schlagwörter für diesen Artikel
laser ablation; fast photography; plume propagation; dynamics analysis; drag model

Artikel in diesem Heft

  1. Original Paper
  2. A practical approach to non-spectral interferences elimination in inductively coupled plasma optical emission spectrometry
  3. Original Paper
  4. Two 1,8-naphthalimide-based proton-receptor fluorescent probes for pH determination
  5. Original Paper
  6. Fabrication of amperometric cholesterol biosensor based on SnO2 nanoparticles and Nafion-modified carbon paste electrode
  7. Original Paper
  8. Preparation and catalytic performance of quaternary ammonium base resin for methanolysis of natural phosphatidylcholine
  9. Original Paper
  10. Optimisation of microwave-assisted extraction from Phyllanthus amarus for phenolic compounds-enriched extracts and antioxidant capacity
  11. Original Paper
  12. Red clover (Trifolium pratense L.) honey: volatiles chemical-profiling and unlocking antioxidant and anticorrosion capacity
  13. Original Paper
  14. Application of vacuum membrane distillation for concentration of organic solutions‡
  15. Original Paper
  16. Correlations for mixing energy in processes using Rushton turbine mixer‡
  17. Original Paper
  18. Recovery of Au(III) ions by Au(III)-imprinted hydrogel
  19. Original Paper
  20. Initiation behaviour in hydrogenation of pyrolysis gasoline over presulphided Ni-Mo-Zn/Al2O3 catalyst
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