Startseite Measurement of integral cross sections of some neutron induced reactions on rubidium at a TRIGA reactor: comparison with integrated data from evaluated data libraries
Artikel
Lizenziert
Nicht lizenziert Erfordert eine Authentifizierung

Measurement of integral cross sections of some neutron induced reactions on rubidium at a TRIGA reactor: comparison with integrated data from evaluated data libraries

  • M. Mezbah Uddin , M. Shuza Uddin ORCID logo EMAIL logo , Rahat Khan ORCID logo , Kamrun Naher , M. Asad Shariff ORCID logo , S. Mohammod Hossain , M. Obaidur Rahman , M. Shamsuzzoha Basunia ORCID logo und Syed M. Qaim ORCID logo
Veröffentlicht/Copyright: 30. April 2025
Radiochimica Acta
Aus der Zeitschrift Radiochimica Acta Band 113 Heft 6

Abstract

Spectrum-averaged cross sections of the reactions 85Rb(n,α)82xm + gBr, 85Rb(n,2n)84xm + gRb and 85Rb(n,p)85mKr were measured over the fast neutron spectrum with neutron energies from 0.5 to 20 MeV of a TRIGA reactor. In addition, data for the well-investigated reactions 113In(n,n´)113mIn and 115In(n,n´)115mIn were re-measured to confirm the validity of the neutron spectrum and the experimental techniques. The new results of the present measurements were used to perform integral tests of evaluated excitation functions in the latest nuclear data libraries, including ENDF/B-VIII.1, JEFF-3.3, JEFF-3.1/A, JENDL-5, IRDF-1.05, and TENDL-2023. The experimental data generally agree with the integrated values from the excitation functions within 8 %, with a few exceptions. For the reaction 85Rb(n,2n)84xm + gRb, the integrated value from the ENDF/B-VIII.1 library is higher by 17 % than the measured integral value. The JEFF-3.1/A and JENDL-5 libraries for the reaction 85Rb(n,p)85mKr appear to require improvement.

Keywords: TRIGA mark II reactor; fast neutron spectrum; nuclear reaction; spectrum-averaged cross section; integral test of differential data
Corresponding author: M. Shuza Uddin, Institute of Nuclear Science and Technology, Atomic Energy Research Establishment, Savar, Dhaka, Bangladesh, E-mail:

Acknowledgments

The authors would like to thank the staffs of Tandem Accelerator Facilities Division, INST, AERE, Savar for their help in preparation of samples. We also grateful to operations crew of the TRIGA Mark II nuclear reactor, Savar, Dhaka, for their assistance in performing the irradiations of the samples.

  1. Research ethics: Not applicable.

  2. Informed consent: Not applicable.

  3. Author contributions: All authors have accepted responsibility for the entire content of this manuscript and approved its submission.

  4. Use of Large Language Models, AI and Machine Learning Tools: None declared.

  5. Conflict of interest: The authors state no conflict of interest.

  6. Research funding: None declared.

  7. Data availability: Not applicable.

References

1. Uddin, M. S.; Sudár, S.; Hossain, S. M.; Khan, R.; Zulquarnain, M. A.; Qaim, S. M. Fast Neutron Spectrum Unfolding of a TRIGA Mark II Reactor and Measurement of Spectrum-Averaged Cross Sections: Integral Tests of Differential Cross Sections of Neutron Threshold Reactions. Radiochim. Acta 2013, 101, 613–620.10.1524/ract.2013.2073Suche in Google Scholar

2. Uddin, M. S.; Zaman, M. R.; Hossain, S. M.; Qaim, S. M. Radiochemical Measurement of Neutron−Spectrum Averaged Cross Sections for the Formation of 64Cu and 67Cu via the (n,p) Reaction at a TRIGA Mark-II Reactor: Feasibility of Simultaneous Production of the Theragnostic Pair 64Cu/67Cu. Radiochim. Acta 2014, 102, 473–480.10.1515/ract-2013-2199Suche in Google Scholar

3. Uddin, M. S.; Rafee, K. A.; Hossain, S. M.; Khan, R.; Qaim, S. M. Integral Measurement of Spectrum-Averaged Cross Sections of a Few Threshold Reactions Induced by Fast Neutrons of a TRIGA Reactor: Comparison with Integrated Data from Excitation Functions Given in Various Data Libraries. Radiochim. Acta 2020, 108, 511–516; https://doi.org/10.1515/ract-2019-3212.Suche in Google Scholar

4. Uddin, M. S.; Uddin, M. M.; Khan, R.; Hasan, M. M.; Shariff, M. A.; Rahman, M. O.; Qaim, S. M. Measurement of Spectrum-Averaged Cross Sections of the (n,p) and (n,n´) Reactions on Strontium by Fast Neutrons of a TRIGA Reactor: Comparison with Integrated Data from Excitation Functions of Various Data Libraries. Radiochim. Acta 2023, 111, 665–670.10.1515/ract-2023-0155Suche in Google Scholar

5. Molla, N. I.; Qaim, S. M. A Systematic Study of (n,p) Reactions at 14.7 MeV. Nucl. Phys. A 1977, 283, 269; https://doi.org/10.1016/0375-9474(77)90431-6.Suche in Google Scholar

6. Otuka, N.; Dupont, E.; Semkova, V.; Pritychenko, B.; Blokhin, A. I.; Aikawa, M.; Babykina, S.; Bossant, M.; Chen, G.; Dunaeva, S.; Forrest, R. A.; Fukahori, T.; Furutachi, N.; Ganesan, S.; Ge, Z.; Gritzay, O. O.; Herman, M.; Hlavač, S.; Katō, K.; Lalremruata, B.; Lee, Y. O.; Makinaga, A.; Matsumoto, K.; Mikhaylyukova, M.; Pikulina, G.; Pronyaev, V. G.; Saxena, A.; Schwerer, O.; Simakov, S. P.; Soppera, N.; Suzuki, R.; Takács, S.; Tao, X.; Taova, S.; Tárkányi, F.; Varlamov, V. V.; Wang, J.; Yang, S. C.; Zerkin, V.; Zhuang, Y. Towards a More Complete and Accurate Experimental Data Library (EXFOR): International Collaboration between Nuclear Reaction Data Centres (NRDC). Nucl. Data Sheets 2014, 120, 272–276; https://doi.org/10.1016/j.nds.2014.07.065.Suche in Google Scholar

7. Konno, C.; Ikeda, Y.; Oishi, K.; Kawade, K.; Yamamoto, H.; Maekawa, H. Activation Cross Section Measurements at Neutron Energy from 13.3 to 14.9 MeV. JAERI Reports No.1329, 1993.Suche in Google Scholar

8. Yuan, X.; Zhao, W.; Yu, W.; Lu, H. Cross Sections of 85Rb and 87Rb for Fast Neutrons. Chinese J. Nucl. Phys. 1990, 12, 289.Suche in Google Scholar

9. Pepelnik, R.; Anders, B.; Bahal, B. M.; Farooq, M., 14 MeV Neutron Activation Cross Sections. Ges.Kernenergie-Verwertung, Schiffbau and Schiffahrt; Geesthacht: Germany, No.86-E-29, 1986.10.1080/00337578608208324Suche in Google Scholar

10. Bormann, M.; Dreyer, F.; Neuert, H.; Riehle, I.; Zielinski, U. Measurements of Some Fast Neutron Cross Sections with the Activation Method. Nuclear Data For Reactors Conf., Paris; published by IAEA: Vienna, Vol. 1, 1966; p. 225.Suche in Google Scholar

11. Bormann, M.; Behrend, A.; Riehle, I.; Vogel, O. Measurement of (n,2n) Excitation Functions. Nucl. Phys. A 1968, 115, 309; https://doi.org/10.1016/0375-9474(68)90006-7.Suche in Google Scholar

12. Bormann, M.; Feddersen, H.-K.; Holscher, H.-H.; Wagner, H.; Scobel, W. Excitation Functions of Some (n,2n) and (n,alpha) Reactions between 13 and 18 MeV Neutron Energies. Report from Euratom-countries + Euratom to EANDC No.150, 1972; p. 30.Suche in Google Scholar

13. Bormann, M.; Feddersen, H.-K.; Holscher, H.-H.; Scobel, W.; Wagner, H. (n,2n) Excitation Functions for Fe-54, Ge-70, Se-74, Rb-85, Sr-86,88, Y-89, Mo-92, and Hg-204 in the Neutron Energy Region 13-18 MeV. Z. Phys. A: Hadrons Nucl. 1976, 277, 203.10.1007/BF01433714Suche in Google Scholar

14. Augustyniak, W.; Herman, M.; Marcinkowski, A. Cross-sections for the Fast Neutron Induced Reactions on Rubidium Isotopes. Acta Phys. Pol. Part B 1976, 7, 347.Suche in Google Scholar

15. Zhu, C.; Chen, Y.; Mou, Y.; Zheng, P.; He, T.; Wang, X.; An, L.; Guo, H. Measurements of (n,2n) Reaction Cross Sections at 14 MeV for Several Nuclei. Nucl. Sci. Eng. 2011, 169, 188; https://doi.org/10.13182/nse10-35.Suche in Google Scholar

16. Zhu, C.; Wang, J.; Jiang, L.; Zheng, P. Measurement of 85Rb(n,2n)84Rb Reaction Cross-Section from 12 MeV up to 19.8 MeV. Chinese Phys. C 2020, 44, 034001; https://doi.org/10.1088/1674-1137/44/3/034001.Suche in Google Scholar

17. Luo, J.; Jiang, L.; He, L. Measurement of Cross Sections and Isomeric Cross- Section Ratios for the (n,2n) Reactions on 85,87Rb in Energies between 13 and 15 MeV. Radiochim. Acta 2018, 106, 709; https://doi.org/10.1515/ract-2018-2951.Suche in Google Scholar

18. Ghorai, S. K.; Vos, R.; Cooper, J. R.; Alford, W. L. The (n,2n) Cross Sections of 85Rb, 87Rb and 144Sm. Nucl. Phys. A 1974, 223, 118; https://doi.org/10.1016/0375-9474(74)90280-2.Suche in Google Scholar

19. Csikai, J.; Peto, G. Influence of Direct Inelastic Scattering on (n,2n) Cross-Sections. Acta Phys. Hung. 1967, 23, 87.10.1007/BF03157358Suche in Google Scholar

20. ENDF/B-VIII.1. U.S. Evaluated Nuclear Data Library, 2024. Nucl. Data Sheets 2018, 148, 1.Suche in Google Scholar

21. Plompen, A. J. M.; Cabellos, O.; De Saint Jean, C.; Fleming, M.; Algora, A.; Angelone, M.; Archier, P.; Bauge, E.; Bersillon, O.; Blokhin, A.; Cantargi, F.; Chebboubi, A.; Diez, C.; Duarte, H.; Dupont, E.; Dyrda, J.; Erasmus, B.; Fiorito, L.; Fischer, U.; Flammini, D.; Foligno, D.; Gilbert, M. R.; Granada, J. R.; Haeck, W.; Hambsch, F.-J.; Helgesson, P.; Hilaire, S.; Hill, I.; Hursin, M.; Ichou, R.; Jacqmin, R.; Jansky, B.; Jouanne, C.; Kellett, M. A.; Kim, D. H.; Kim, H. I.; Kodeli, I.; Koning, A. J.; Konobeyev, A. Yu.; Kopecky, S.; Kos, B.; Krása, A.; Leal, L. C.; Leclaire, N.; Leconte, P.; Lee, Y. O.; Leeb, H.; Litaize, O.; Majerle, M.; Márquez, J.; Damián, I.; Michel-Sendis, F.; Mills, R. W.; Morillon, B.; Noguère, G.; Pecchia, M.; Pelloni, S.; Pereslavtsev, P.; Perry, R. J.; Rochman, D.; Röhrmoser, A.; Romain, P.; Romojaro, P.; Roubtsov, D.; Sauvan, P.; Schillebeeckx, P.; Schmidt, K. H.; Serot, O.; Simakov, S.; Sirakov, I.; Sjöstrand, H.; Stankovskiy, A.; Sublet, J. C.; Tamagno, P.; Trkov, A.; van der Marck, S.; Álvarez-Velarde, F.; Villari, R.; Ware, T. C.; Yokoyama, K.; Žerovnik, G. The Joint Evaluated Fission and Fusion Nuclear Data Library, JEFF-3.3. Eur. Phys. J. A 2020, 56, 181; https://doi.org/10.1140/epja/s10050-020-00141-9.Suche in Google Scholar

22. Forrest, R. A.; Kopecky, J.; Sublet, J.-C. JEFF-3.1/A Library, the European Activation File: EAF-2003 Cross Section Library – UKAEA; Report FUS 486, 2002.Suche in Google Scholar

23. Iwamoto, O.; Iwamoto, N.; Kunieda, S.; Minato, F.; Nakayama, S.; Abe, Y.; Tsubakihara, K.; Okumura, S.; Ishizuka, C.; Yoshida, T.; Chiba, S.; Otuka, N.; Sublet, J.-C.; Iwamoto, H.; Yamamoto, K.; Nagaya, Y.; Tada, K.; Konno, C.; Matsuda, N.; Yokoyama, K.; Taninaka, H.; Oizumi, A.; Fukushima, M.; Okita, S.; Chiba, G.; Sato, S.; Ohta, M.; Kwon, S. Japanese Evaluated Nuclear Data Library Version 5: JENDL-5. J. Nucl. Sci. Technol. 2023, 60, 1; https://doi.org/10.1080/00223131.2022.2141903.Suche in Google Scholar

24. IRDFF v.1.05: International Reactor Dosimetry and Fusion File, 2014. https://nds.iaea.org/IRDFFv105/.Suche in Google Scholar

25. Koning, A. J.; Rochman, D.; Sublet, J.-Ch.; Dzysiuk, N.; Fleming, M.; van der Marck, S. TENDL: Complete Nuclear Data Library for Innovative Nuclear Science and Technology. Nucl. Data Sheets 2019, 155, 1; https://doi.org/10.1016/j.nds.2019.01.002.Suche in Google Scholar

26. Calamand, A. Cross Sections for Fission Neutron Spectrum Induced Reactions. In Handbook on Nuclear Activation Cross Sections. Technical Report No. 156; IAEA: Vienna, 1974; p. 273.Suche in Google Scholar

27. Ζaidi, J. Η.; Karim, H. M. A.; Qaim, S. M. Fission Neutron Spectrum Averaged Cross Sections of Some Threshold Reactions on Xenon: Evaluation of 123I-Production Using Fast Neutrons. Radiochim. Acta 1985, 38, 123–130; https://doi.org/10.1524/ract.1985.38.3.123.Suche in Google Scholar

28. Zaidi, J. H.; Karim, H. M. A.; Arif, M.; Qureshi, I. H.; Qaim, S. M.; Stöcklin, G. Fission Neutron Spectrum Averaged Cross Sections of Some Threshold Reactions on Molybdenum: Estimation of Radioactive Impurities in (n,γ)-produced 99Mo-99mTc Generator System. Radiochim. Acta 1990, 49, 107–112; https://doi.org/10.1524/ract.1990.49.3.107.Suche in Google Scholar

29. Fitzgerald, J. JF Computing Services, 17 Chapel Road, Stanford in the Vale, Oxfordshire, SN7 8LE. Copyright © Jim Fitzgerald, 1991–2016, Last updated 8th October 2016.Suche in Google Scholar

30. Mughabghab, S. Atlas of Neutron Resonances, 6th Edition, Vol. 2, Resonance Properties and Thermal Cross Sections Z = 61-102; Elsevier: Amsterdam, 2018.Suche in Google Scholar

31. Nesaraja, C. D.; Geraedts, S. D.; Singh, B. Nuclear Data Sheets for A = 58. Nucl. Data Sheets 2010, 111, 897; https://doi.org/10.1016/j.nds.2010.03.003.Suche in Google Scholar

32. Tuli, J. K.; Browne, E. Nuclear Data Sheets for A = 82. Nucl. Data Sheets 2019, 157, 260; https://doi.org/10.1016/j.nds.2019.04.002.Suche in Google Scholar

33. Abriola, D.; Bostan, M.; Erturk, S.; Fadil, M.; Galan, M.; Juutinen, S.; Kibédi, T.; Kondev, F.; Luca, A.; Negret, A.; Nica, N.; Pfeiffer, B.; Singh, B.; Sonzogni, A.; Timar, J.; Tuli, J.; Venkova, T.; Zuber, K. Nuclear Data Sheets for A = 84. Nucl. Data Sheets 2009, 110, 2815; https://doi.org/10.1016/j.nds.2009.10.002.Suche in Google Scholar

34. Singh, B.; Chen, J. Nuclear Data Sheets for A = 85. Nucl. Data Sheets 2014, 116, 1; https://doi.org/10.1016/j.nds.2014.01.001.Suche in Google Scholar

35. Blachot, J. Nuclear Data Sheets for A = 115. Nucl. Data Sheets 2012, 113, 2391; https://doi.org/10.1016/j.nds.2012.10.002.Suche in Google Scholar

36. Blachot, J. Nuclear Data Sheets for A = 113. Nucl. Data Sheets 2010, 111, 1471; https://doi.org/10.1016/j.nds.2010.05.001.Suche in Google Scholar

37. Huang, X.; Kang, M. Nuclear Data Sheets for A = 198. Nucl. Data Sheets 2016, 133, 221; https://doi.org/10.1016/j.nds.2016.02.002.Suche in Google Scholar

38. NuDat3: Decay Radiation Database version of 2023. National Nuclear Data Center, Brookhaven, USA, July 2023. https://www.nndc.bnl.gov/nudat3/.Suche in Google Scholar

39. Trkov, A.; Griffin, P. J.; Simakov, S. P.; Greenwood, L. R.; Zolotarev, K. I.; Capote, R.; Aldama, D. L.; Chechev, V.; Destouches, C.; Kahler, A. C.; Konno, C.; Koštál, M.; Majerle, M.; Malambu, E.; Ohta, M.; Pronyaev, V. G.; Radulovic, V.; Sato, S.; Schulc, M.; Simečková, E.; Vavtar, I.; Wagemans, J.; White, M.; Yashima, H. IRDFF-II: A New Neutron Metrology Library. Nucl. Data Sheets 2020, 163, 1; https://doi.org/10.1016/j.nds.2019.12.001.Suche in Google Scholar

40. Qaim, S. M.; Sudár, S.; Scholten, A. J.; Koning, A. J.; Coenen, H. H. Evaluation of Excitation Functions of 100Mo(p,d+pn)99Mo and 100Mo(p,2n)99mTc Reactions: Estimation of Long-Lived Tc-Impurity and its Implication on the Specific Activity of Cyclotron-Produced 99mTc. Appl. Radiat. Isot. 2014, 85, 101–113; https://doi.org/10.1016/j.apradiso.2013.10.004.Suche in Google Scholar PubMed

41. Uddin, M. S.; Scholten, B.; Basunia, M. S.; Sudár, S.; Spellerberg, S.; Voyles, A. S.; Zaneb, H.; Morrell, J. T.; Rios, J.; Spahn, I.; Bernstein, L. A.; Neumaier, B.; Qaim, S. M. Accurate Determination of Production Data of the Non-standard Positron Emitter 86Y via the 86Sr(p,n)-Reaction. Radiochim. Acta 2020, 108, 747–757.10.1515/ract-2020-0021Suche in Google Scholar

42. Birn, I.-G.; Strohmaier, B.; Freiesleben, H.; Qaim, S. M. Isomeric Cross-Section Ratios for the Formation of 75m,gGe. Phys. Rev. C 1995, 52, 2546–2551; https://doi.org/10.1103/physrevc.52.2546.Suche in Google Scholar PubMed

43. Nesaraja, C. D.; Sudár, S.; Qaim, S. M. Cross Section for the Formation of 69m,gZn and 71m,gZn in Neutron Induced Reactions Near Their Thresholds: Effect of Reaction Channel on the Isomeric Cross Section Ratio. Phys. Rev. C 2003, 68, 024603.Suche in Google Scholar
Received: 2025-02-18
Accepted: 2025-04-14
Published Online: 2025-04-30
Published in Print: 2025-06-26

© 2025 Walter de Gruyter GmbH, Berlin/Boston

Artikel in diesem Heft

  1. Frontmatter
  2. Original Papers
  3. Synthesis of amide imidazole-based functionalized ionic liquid for separation of Th/Pu
  4. Measurement of integral cross sections of some neutron induced reactions on rubidium at a TRIGA reactor: comparison with integrated data from evaluated data libraries
  5. Production and purification of research scale 161Tb using cation-exchange semi-preparative HPLC for radiopharmaceutical applications
  6. The enhancement of mtrABDEF gene expressions in Shewanella azerbaijanica, through acclimation in high uranium concentrations
  7. Temporal variation of radon in soil and water in Kosovo
  8. Investigation of some radiation interaction parameters with aluminum–boron alloys
  9. Radiation shielding performance of lead-borate glasses with rare-earth oxides: a comparative analysis
https://doi.org/10.1515/ract-2025-0019
Schlagwörter für diesen Artikel
TRIGA mark II reactor; fast neutron spectrum; nuclear reaction; spectrum-averaged cross section; integral test of differential data

Artikel in diesem Heft

  1. Frontmatter
  2. Original Papers
  3. Synthesis of amide imidazole-based functionalized ionic liquid for separation of Th/Pu
  4. Measurement of integral cross sections of some neutron induced reactions on rubidium at a TRIGA reactor: comparison with integrated data from evaluated data libraries
  5. Production and purification of research scale 161Tb using cation-exchange semi-preparative HPLC for radiopharmaceutical applications
  6. The enhancement of mtrABDEF gene expressions in Shewanella azerbaijanica, through acclimation in high uranium concentrations
  7. Temporal variation of radon in soil and water in Kosovo
  8. Investigation of some radiation interaction parameters with aluminum–boron alloys
  9. Radiation shielding performance of lead-borate glasses with rare-earth oxides: a comparative analysis
Jetzt anmelden und 20% sparen
Institutioneller Zugang
Wie funktioniert Authentifizierung?
Haben Sie eine Idee, wie wir unsere Website verbessern können?
Bitte schreiben Sie uns.
© 2025 De Gruyter Brill
Heruntergeladen am 7.11.2025 von https://www.degruyterbrill.com/document/doi/10.1515/ract-2025-0019/html?lang=de
Button zum nach oben scrollen