Band 8, Heft 7

On-chip plasmon-induced transparency (PIT) possessing the unique properties of controlling light propagation states is a promising way to on-chip ultrafast optical connection networks as well as integrated optical processing chips. On-chip PIT has attracted enormous research interests, the latest developments of which have also yield progress in nanophotonics, material science, nonlinear optics, and so on. This review summarizes the realization methods, novel configurations, diversiform materials, and the improved performance indexes. Finally, a brief outlook on the remaining challenges and possible development direction in the pursuit of the application of a practical on-chip photonic processor based on PIT is also afforded.

Photonic metasurfaces, that is, two-dimensional arrangements of designed plasmonic or dielectric resonant scatterers, have been established as a successful concept for controlling light fields at the nanoscale. While the majority of research so far has concentrated on passive metasurfaces, the direct integration of nanoscale emitters into the metasurface architecture offers unique opportunities ranging from fundamental investigations of complex light-matter interactions to the creation of flat sources of tailored light fields. While the integration of emitters in metasurfaces as well as many fundamental effects occurring in such structures were initially studied in the realm of nanoplasmonics, the field has recently gained significant momentum following the development of Mie-resonant dielectric metasurfaces. Because of their low absorption losses, additional possibilities for emitter integration, and compatibility with semiconductor-based light-emitting devices, all-dielectric systems are promising for highly efficient metasurface light sources. Furthermore, a flurry of new emission phenomena are expected based on their multipolar resonant response. This review reports on the state of the art of light-emitting metasurfaces, covering both plasmonic and all-dielectric systems.

Plasmonic nanostructures can concentrate light and enhance light-matter interactions in the subwavelength domain, which is useful for photodetection, light emission, optical biosensing, and spectroscopy. However, conventional plasmonic devices and systems are typically optimized for the operation in a single wavelength band and thus are not suitable for multiband nanophotonics applications that either prefer nanoplasmonic enhancement of multiphoton processes in a quantum system at multiple resonant wavelengths or require wavelength-multiplexed operations at nanoscale. To overcome the limitations of “single-resonant plasmonics,” we need to develop the strategies to achieve “multiresonant plasmonics” for nanoplasmonic enhancement of light-matter interactions at the same locations in multiple wavelength bands. In this review, we summarize the recent advances in the study of the multiresonant plasmonic systems with spatial mode overlap. In particular, we explain and emphasize the method of “plasmonic mode hybridization” as a general strategy to design and build multiresonant plasmonic systems with spatial mode overlap. By closely assembling multiple plasmonic building blocks into a composite plasmonic system, multiple nonorthogonal elementary plasmonic modes with spectral and spatial mode overlap can strongly couple with each other to form multiple spatially overlapping new hybridized modes at different resonant energies. Multiresonant plasmonic systems can be generally categorized into three types according to the localization characteristics of elementary modes before mode hybridization, and can be based on the optical coupling between: (1) two or more localized modes, (2) localized and delocalized modes, and (3) two or more delocalized modes. Finally, this review provides a discussion about how multiresonant plasmonics with spatial mode overlap can play a unique and significant role in some current and potential applications, such as (1) multiphoton nonlinear optical and upconversion luminescence nanodevices by enabling a simultaneous enhancement of optical excitation and radiation processes at multiple different wavelengths and (2) multiband multimodal optical nanodevices by achieving wavelength multiplexed optical multimodalities at a nanoscale footprint.

The ability of metallic nanostructures to confine light at the sub-wavelength scale enables new perspectives and opportunities in the field of nanotechnology. Making use of this unique advantage, nano-optical trapping techniques have been developed to tackle new challenges in a wide range of areas from biology to quantum optics. In this work, starting from basic theories, we present a review of research progress in near-field optical manipulation techniques based on metallic nanostructures, with an emphasis on some of the most promising advances in molecular technology, such as the precise control of single biomolecules. We also provide an overview of possible future research directions of nanomanipulation techniques.

Due to the advantages of narrow energy distribution of plasmonic hot-electrons in Ag and the high density of states in the TiO 2 conduction band, an Ag/TiO 2 composite is considered to be an ideal combination to construct a plasmonic hot-electron photodetector with high detectivity and a high response speed. In this work, we fabricate a porous Ag/TiO 2 -Schottky-diode based plasmonic hot-electron photodetector. This detector shows a high detectivity of 9.8 × 10 10 cmHz 1/2 /W and a fast response speed, with a rise and fall time of 112 μs and 24 μs, respectively, under 450 nm light illumination at zero bias voltage. In addition, the height of the Ag/TiO 2 Schottky barrier can be decreased by removing the chemisorbed oxygen from the surface of TiO 2 with ultraviolet light illumination, and as a result, the responsivity of the Ag/TiO 2 plasmonic hot-electron photodetector at 450 nm can increase from 3.4 mA/W to 7.4 mA/W.

Data-driven design approaches based on deep learning have been introduced in nanophotonics to reduce time-consuming iterative simulations, which have been a major challenge. Here, we report the first use of conditional deep convolutional generative adversarial networks to design nanophotonic antennae that are not constrained to predefined shapes. For given input reflection spectra, the network generates desirable designs in the form of images; this allows suggestions of new structures that cannot be represented by structural parameters. Simulation results obtained from the generated designs agree well with the input reflection spectrum. This method opens new avenues toward the development of nanophotonics by providing a fast and convenient approach to the design of complex nanophotonic structures that have desired optical properties.

Metasurfaces are engineered thin surfaces comprising two-dimensional (2D) arrays of sub-wavelength-spaced and sub-wavelength-sized resonators. Metasurfaces can locally manipulate the amplitude, phase, and polarization of light with high spatial resolution. In this paper, we report numerical and experimental results of a vortex-beam-generating metasurface fabricated specifically for infrared (IR) and terahertz (THz) wavelengths. The designed metasurface consists of a 2D array of dielectric cross-shaped resonators with spatially varying length, thereby providing the desired spatially varying phase shift to the incident light. The metasurface was found to be insensitive to the polarization of the incident light. The dimensions of the cross-resonators were calculated using rigorous finite-difference time-domain analysis. The spectral scalability via physical scaling of the meta-resonators is demonstrated using two vortex-generating optical elements operating at 8.8 μm (IR) and 0.78 THz. The vortex beam generated in the mid-IR spectral range was imaged using a Fourier transform IR (FTIR) imaging miscroscope equipped with a focal plane array detector. This design could be used for efficient wavefront shaping and various optical imaging applications in the mid-IR spectral range, where polarization insensitivity is desired.

Tailoring the fluorescence emission of quantum emitters to a desired direction is a crucial issue to achieve high efficient photodetection and realize unique optoelectronic devices. In this study, the directional emission of quantum dots controlled by optical traveling wave antennas based on 1D silver nanowires (NWs) was investigated. Both leaky waves and surface waves on a single NW are utilized for fluorescence emission control, and we show that the coupled fluorescence transforms from bidirectional to unidirectional emission when the surrounding medium changes from air to water. Moreover, in the unidirectional case, we obtain an ultra-narrow half-power bandwidth about 20°. Finite-difference time-domain simulations and Green’s function method in a stratified medium are used to calculate the far-field emission patterns of the hybrid structures, which agree well with the experiments. Further analyses based on typical modes and the dipole-chain model also reveal the mechanism behind the bidirectional and unidirectional fluorescence emission. These results show that the structures have great potential in integrated on-chip, sensing and photon-collection devices.

Vector beams with phase modulation in a high numerical aperture system are able to break through the diffraction limit. However, the implementation of such a device requires a combination of several discrete bulky optical elements, increasing its complexity and possibility of the optical loss. Dielectric metalens, an ultrathin and planar nanostructure, has a potential to replace bulky optical elements, but its optimization with full-wave simulations is time-consuming. In this paper, an accurate and efficient theoretical model of planar metalens is developed. Based on this model, a twofold optimization scheme is proposed for optimizing the phase profile of metalenses so as to achieve subdiffraction focusing with high focusing efficiency. Then, a metalens that enables to simultaneously generate radially polarized beam (RPB) and modulate its phase under the incidence of x -polarized light with the wavelength of 532 nm is designed. Full-wave simulations show that the designed metalens of NA = 0.95 can achieve subdiffraction focusing (FWHM = 0.429λ) with high transmission efficiency (77.6%) and focusing efficiency (17.2%). Additionally, superoscillation phenomenon is found, leading to a compromise between the subdiffraction spot and high efficiency. The proposed method may provide an accurate and efficient way to achieve sub-wavelength imaging with the expected performances, which shows a potential application in super-resolution imaging.

The mathematical concept of fractals is widely applied to photonics as planar structures ranging from terahertz resonators, optical antennas, to photodetectors. Here, instead of a direct mathematical abstract, we design a plasmonic leaf with fractal geometry from the outline of a leaf from Wargrave Pink. The enhanced light-matter interactions are observed numerically from the improvement in both absorption and near-field intensification. To demonstrate the effect experimentally, a three-dimensional fractal structure is realised through direct laser writing, which significantly improves the photothermal conversion. By virtue of the self-similarity in geometry, the artificial leaf improves the absorption of a 10-nm-thick gold film with 14 ×  temperature increment compared to flat Au film. Not limited to the proof-of-concept photothermal experiment demonstrated here, the fractal structure with improved light-matter interactions can be utilised in a variety of applications ranging from non-linear harmonic generation, plasmonic-enhanced fluorescence, to hot electron generation for photocatalysis.

Single-molecule localization microscopy (SMLM) provides a powerful toolkit to specifically resolve intracellular structures on the nanometer scale, even approaching resolution classically reserved for electron microscopy (EM). Although instruments for SMLM are technically simple to implement, researchers tend to stick to commercial microscopes for SMLM implementations. Here we report the construction and use of a “custom-built” multi-color channel SMLM system to study liver sinusoidal endothelial cells (LSECs) and platelets, which costs significantly less than a commercial system. This microscope allows the introduction of highly affordable and low-maintenance SMLM hardware and methods to laboratories that, for example, lack access to core facilities housing high-end commercial microscopes for SMLM and EM. Using our custom-built microscope and freely available software from image acquisition to analysis, we image LSECs and platelets with lateral resolution down to about 50 nm. Furthermore, we use this microscope to examine the effect of drugs and toxins on cellular morphology.