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Facile formation of STO/gC3N4 hybrid composite to effectively degrade the dye and antibiotic under white light

  • Kombiah Aravinthkumar , Smagul Karazhanov and Chinnan Raja Mohan EMAIL logo
Published/Copyright: February 15, 2024
Zeitschrift für Physikalische Chemie
From the journal Zeitschrift für Physikalische Chemie Volume 238 Issue 11

Abstract

A novel organic-inorganic photocatalyst like layer structured graphitic carbon nitride (g-C3N4 or CN) hybrid with strontium titanate (SrTiO3 or STO) was prepared by a precipitation-sonication technique for photocatalytic activity. The crystal phases, morphologies, elemental composition, optical properties, and porous structure of the prepared pristine and STO/CN hybrid composite were measured using various physicochemical characterizations. It is indicated that STO nanospheres were effectively loaded on the g-C3N4 nanosheets, resulting in the STO/CN hybrid composite, high surface area, enhanced visible-light absorption, enhancing photoinduced charge separation and suppressing the recombination rate. Furthermore, the 3 wt% of g-C3N4 composited STO (STO/CN-3) catalyst demonstrated higher photocatalytic activity than pristine STO in 100 min under white light irradiation, reaching the degradation efficiency of 92.66 % and 93.31 % toward methylene blue (MB) and tetracycline (TC), respectively. The improved photocatalytic activity of STO/gCN hybrid composite could be ascribed to the synergistic effect between STO and CN with strong interfacial interaction facilitating efficient charge separation and inhibiting the charge recombination of photogenerated electron-hole pairs. Moreover, a possible photocatalytic mechanism has been proposed for the degradation of MB and TC. Besides, the excellent photocatalytic performance, STO/CN-3 nanocomposite also exhibits outstanding photostability under the current factors, suggesting that they are suitable for practical applications.

Keywords: photodegradation; advanced oxidation processes; nanocomposites; methylene blue; tetracycline
Corresponding author: Chinnan Raja Mohan, Nanostructure Lab, Department of Physics, The Gandhigram Rural Institute – Deemed to be University, Gandhigram 624302, Tamil Nadu, India, E-mail:

Acknowledgements

The author K. Aravinthkumar thank the Joint Council of Scientific & Industrial Research (CSIR) – University Grants Commission (UGC), Government of India for the financial support in the form of fellowship for this work through the NET-SRF Award (NTA Ref. No.: 201610274875 dated 01.04.2021). C.Raja Mohan Thanks Prof.G.Muralidharan for useful discussions.

  1. Research ethics: Not applicable.

  2. Author contributions: K. Aravinthkumar: Conceptualization, Methodology, Investigation, Formal analysis, Writing – Original Draft. S. Karazhanov: Formal analysis, Software and Review. C. Raja Mohan: Conceptualization, Validation, Visualization, Writing – Review & Editing, Supervision.

  3. Competing interests: The authors declare that they have no conflict of interest to the publication of this article.

  4. Research funding: None declared.

  5. Data availability: Data will be made available on request.

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Received: 2023-10-31
Accepted: 2024-01-17
Published Online: 2024-02-15
Published in Print: 2024-11-26

© 2024 Walter de Gruyter GmbH, Berlin/Boston

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https://doi.org/10.1515/zpch-2023-0398
Keywords for this article
photodegradation; advanced oxidation processes; nanocomposites; methylene blue; tetracycline

Articles in the same Issue

  1. Frontmatter
  2. Contributions to “Materials for Solar Water Splitting”
  3. Unveiling the role of rare earth dopant in metal molybdate nanocomposites via facile microwave-combustion strategy and their effect on antibacterial activity
  4. Effect of lanthanum (La) substitution on the magnetic and electrical properties of nickel ferrites: an investigation of its doping concentrations
  5. The relationship between environmental factors and dust accumulation by machine learning
  6. Facile formation of STO/gC3N4 hybrid composite to effectively degrade the dye and antibiotic under white light
  7. Investigation of the composition and morphology of raw materials from the Aral Sea region
  8. Chemical state and atomic structure in stoichiovariants photochromic oxidized yttrium hydride thin films
  9. Single crystal of barium bis para-nitrophenolate para-nitrophenol tetrahydrate for NLO applications: crystal growth and DFT analysis
  10. Characterization of single-crystal phenothiazine synthesized using the vertical Bridgman method
  11. Amidoxime functionalized mesoporous silica nanoparticles for pH-responsive delivery of anticancer drug
  12. Exploring optical and electrochemical studies on thulium selenite (TmSeO3)
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