Abstract
Cross sections of the 132Ba(n,2n)131m,gBa and 134Ba(n,2n)133m,gBa reactions and their isomeric cross section ratios σm/σg have been measured by means of the activation technique at three neutron energies in the range 13−15 MeV. BaCO3 samples and Nb monitor foils were activated together to determine the reaction cross section and the incident neutron flux. The quasimonoenergetic neutrons beam were produced via the 3H(d,n)4He reaction at the Pd-300 Neutron Generator of the Chinese Academy of Engineering Physics (CAEP). The activities induced in the reaction products were measured using high−resolution γ ray spectroscopy. The pure cross section of the ground-state was derived from the absolute cross section of the metastable state and the residual nuclear decay analysis. Cross sections were also evaluated theoretically using the numerical nuclear model code, TALYS-1.8 with different level density options at neutron energies varying from the reaction threshold to 20 MeV. Results are discussed and compared with the corresponding literature.
Acknowledgement
We would like to thank the Intense Neutron Generator group at the Chinese Academy of Engineering Physics for performing the irradiations and Professor Guoren Yue at Key Laboratory of Hexi Corridor Resources Utilization of Gansu for measuring the sample purity. This work was supported by the National Natural Science Foundation of China (Grant No. 11565012).
References
1. Qaim, S. M., Mushtaq, A., Uhl, M.: Isomeric cross-section ratio for the formation of 73m,gSe in various nuclear processes. Phys. Rev. C 38, 645 (1988).10.1103/PhysRevC.38.645Search in Google Scholar
2. Qaim, S. M.: Total (n,2n) cross sections and isomeric cross-section ratios at 14.7 MeV in the region of rare earths. Nucl. Phys. A 224, 319 (1974).10.1016/0375-9474(74)90690-3Search in Google Scholar
3. Qaim, S. M.: Activation cross sections, isomeric cross-section ratios and systematics of (n,2n) reactions at 14–15 MeV. Nucl. Phys. A 185, 614 (1972).10.1016/0375-9474(72)90036-XSearch in Google Scholar
4. Pepelnik, R., Anders, B., Bahal, B. M., Farooq, M.: 14 MeV neutron activation cross sections, GKSS Geesthacht, in Progress Report in Nuclear Data Research in the Federal Republic of Germany. S. M. Qaim (Ed.), NEANDC (E)-162 U Vol. V; INDC(Ger)-28/LN, 32 (1985).Search in Google Scholar
5. Sakane, H., Kasugai, Y., Shibata, M., Iida, T., Takahashi, A., Fukahori, T., Kawade, K.: Measurement of activation cross-sections for (n,2n) reactions producing short-lived nuclei in the energy range between 13.5 and 14.9 MeV. Ann. Nucl. Energy 28, 1175 (2001).10.1016/S0306-4549(00)00123-7Search in Google Scholar
6. Rurarz, E., Haratym, Z., Kozlowski, T., Oblozinsky, P.: Excitation of isomeric activities in 131,133,135Ba by 14.8 MeV neutrons. Acta Physica Polonica B 3, 637 (1972).Search in Google Scholar
7. Lu, W. D., Ranakumar, N., Fink, R. W.: Activation cross sections for (n,2n) reactions at 14.4 MeV in the region Z=40–60: precision measurements and systematics. Phys. Rev. C 1, 350 (1970).10.1103/PhysRevC.1.350Search in Google Scholar
8. Konno, C., Ikeda, Y., Oishi, K., Kawade, K., Yamamoto, H., Maekawa, H.: Activation cross section measurements at neutron energy from 13.3 to 14.9 MeV, Report. JAERI Reports; No. 1329 (1993).Search in Google Scholar
9. Lu, H., Zhao, W., Yu, W.: Activation cross section for element barium. Chin. J. Nucl. Phys. (Beijing) 14, 244 (1992).Search in Google Scholar
10. Wille, R. G., Fink, R. W.: Activation cross sections for 14.8 MeV neutrons and some new radioactive nuclides in the rare earth region. Phys. Rev. 118, 242 (1960).10.1103/PhysRev.118.242Search in Google Scholar
11. Ikeda, Y., Konno, C., Oishi, K., Nakamura, T., Miyade, H., Kawade, K., Yamamoto, H., Katoh, T.: Activation cross section measurements for fusion reactor structural materials at neutron energy from 13.3 to 15.0 MeV using FNS facility. JAERI Reports, No. 1312 (1988).Search in Google Scholar
12. Holub, E., Cindro, N.: Study of some systematic trends and non-equilibrium effects in (n,2n) reactions for nuclei far from the symmetry line. J. Phys. G 2, 405 (1976).10.1088/0305-4616/2/6/009Search in Google Scholar
13. Jong Do, A., Dresler, J., Garuska, U., Herman, M., Marcinkowski, A.: The cross sections of the (n,2n) reactions on 134Ba,142Nd,150Nd and 144Sm. J. Phys. G 10, 91 (1984).10.1088/0305-4616/10/1/014Search in Google Scholar
14. Fan, Y., Wang, Z., Han, R., Wang, Z., Liu, Z., Du, H., Xiao, Z.: The activation reaction cross section measurement of some barium nuclides induced by 14.7 MeV neutron. Chin. J. Nucl. Phys. (Beijing) 10, 108 (1988).Search in Google Scholar
15. Strohmaier, B., Uhl, M., Matthes, W. K.: Application of nuclear reaction models for neutron nuclear data evaluation: statistical and optical model calculations for 134−138Ba. Nucl. Sci. Eng. 65, 368 (1978).10.13182/NSE78-A27164Search in Google Scholar
16. Csikai, J., Buczko, Cs. M., Pepelnik, R., Agrawal, H. M.: Activation cross-sections related to nuclear heating of high T(c) superconductors. Ann. Nucl. Energy 18, 1 (1991).10.1016/0306-4549(91)90030-2Search in Google Scholar
17. Kong, X., Wang, Y., Yang, J., Yuan, J.: The cross section measurements for the Ba(n,x)134Cs, 134Ba(n,2n)133Ba, 140Ce(n,2n)139Ce, 142Ce(n,2n)141Ce and 23Na(n,2n)22Na reactions. High Energ. Phys. Nucl. Phys., Chinese ed. 19, 781 (1995).Search in Google Scholar
18. Wagner, M., Vonach, H., Pavlik, A., Strohmaier, B., Tagesen, S., Martinez Rico, J.: Physikdaten-physics data, evaluation of cross sections for 14 important neutron dosimetry reactions, Fachinformationszentrum Karlsruhe, Gesellschaft für wissenschaftlich-technische Information mbH. Federal Republic of Germany. No.13-5 (1990).Search in Google Scholar
19. Luo, J., Du, L., Zhao, J.: A method to determine fast neutron energies in large sample. Nucl. Instrum. Meth. B 298, 61 (2013).10.1016/j.nimb.2013.01.029Search in Google Scholar
20. Evaluated Nuclear Structure Data File (ENSDF). http://www.nndc.bnl.gov/ensdf/.Search in Google Scholar
21. Luo, J., Jiang, L.: Ground-state and isomeric-state cross sections for 165Ho(n,2n)164Ho reaction from the reaction threshold to 20 MeV. Phys. Rev. C 89, 014604 (2014).10.1103/PhysRevC.89.014604Search in Google Scholar
22. Luo, J., Wu, C., Jiang, L., He, L.: Cross sections for d-3H neutron interactions with samarium isotopes. Radiochim. Acta 104, 523 (2016).10.1515/ract-2016-0001Search in Google Scholar
23. McCallum, G. J., Coote, G. E.: Influence of source-detector distance on relative intensity and angular correlation measurements with Ge(Li) spectrometers. Nucl. Instr. Meth. 130, 189 (1975).10.1016/0029-554X(75)90173-1Search in Google Scholar
24. Hubbell, J. H., Seltzer, S. M.: Tables of X-ray mass attenuation coefficients and mass energy-absorption coefficients from 1 keV to 20 MeV for elements Z=1 to 92 and 48 additional substances of dosimetric interest. (2017). http://physics.nist.gov/PhysRefData/XrayMassCoef/tab3.html.Search in Google Scholar
25. Luo, J., An, L., Jiang, L.: Ground-state and isomeric-state cross sections for the 138Ce(n,2n)137Ce reaction from its threshold to 20 MeV. Radiochim. Acta 103, 613 (2015).10.1515/ract-2015-2402Search in Google Scholar
26. Luo, J., Liu, R., Jiang, L., Liu, Z., Sun, G., Ge, S.: Cross-sections of 45Sc(n,2n)44m,gSc reaction from the reaction threshold to 20 MeV. Radiochim. Acta 101, 607 (2013).10.1524/ract.2013.2065Search in Google Scholar
27. Koning, A., Hilaire, S., Goriely, S.: TALYS-1.8, A Nuclear Reaction Program, NRG-1755 ZG Petten. The Netherlands. (2015). http://www.talys.eu.Search in Google Scholar
28. RIPL-2 Reference Input Parameter Library, IAEA, A-1400 Vienna, IAEA-NDS. http://www-nds.iaea.org/RIPL-2/.Search in Google Scholar
29. Molla, N. I., Qaim, S. M., Uhl, M.: Activation cross section and isomeric cross-section ratio for the 46Ti(n,p)46m,gSc process. Phys. Rev. C 42, 1540 (1990).10.1103/PhysRevC.42.1540Search in Google Scholar PubMed
30. Qaim, S. M., Ibn Majah, M., Wölfle, R., Strohmaier, B.: Excitation functions and isomeric cross-section ratios for the 90Zr(n,p)90m,gY and 91Zr(n,p)91m,gY processes. Phys. Rev. C 42, 363 (1990).10.1103/PhysRevC.42.363Search in Google Scholar PubMed
31. Sudár, S., Szelecsényi, F., Qaim, S. M.: Excitation function and isomeric cross-section ratio for the 61Ni(p,α)58m,gCo process. Phys. Rev. C 48, 3115 (1993).10.1103/PhysRevC.48.3115Search in Google Scholar PubMed
32. Cserpák, F., Sudár, S., Csikai, J., Qaim, S. M.: Excitation functions and isomeric cross section ratios of the 63Cu(n,α)60m,gCo, 65Cu(n,α)62m,gCo, and 60Ni(n,p)60m,gCo processes from 6 to 15 MeV. Phys. Rev. C 49, 1525 (1994).10.1103/PhysRevC.49.1525Search in Google Scholar
33. Birn, I.-G., Strohmaier, B., Freiesleben, H., Qaim, S. M.: Isomeric cross-section ratios for the formation of 75m,gGe in (n,p), (n,α), and (n,2n) reactions from 6 to 15 MeV. Phys. Rev. C 52, 2546 (1995).10.1103/PhysRevC.52.2546Search in Google Scholar
34. Sudár, S., Qaim S. M.: Isomeric cross-section ratio for the formation of 58m,gCo in neutron, proton, deuteron, and alpha-particle induced reactions in the energy region up to 25 MeV. Phys. Rev. C 53, 2885 (1996).10.1103/PhysRevC.53.2885Search in Google Scholar PubMed
35. Nesaraja, C. D., Sudár, S., Qaim, S. M.: Cross sections for the formation of 69m,gZn and 71m,gZn in neutron induced reactions near their thresholds: Effect of reaction channel on the isomeric cross-section ratio. Phys. Rev. C 68, 024603 (2003).10.1103/PhysRevC.68.024603Search in Google Scholar
36. Sudár, S., Qaim, S. M.: Cross sections for the formation of 195m,gHg, 197m,gHg, and 196m,gAu in α and 3He-particle induced reactions on Pt: effect of level density parameters on the calculated isomeric cross-section ratio. Phys. Rev. C 73, 034613 (2006).10.1103/PhysRevC.73.034613Search in Google Scholar
37. Al-Abyad, M., Sudár, S., Comsan, M. N. H., Qaim, S. M.: Cross sections and isomeric cross-section ratios in the interactions of fast neutrons with isotopes of mercury. Phys. Rev. C 73, 064608 (2006).10.1103/PhysRevC.73.064608Search in Google Scholar
©2017 Walter de Gruyter GmbH, Berlin/Boston
Articles in the same Issue
- Frontmatter
- Activation cross section and isomeric cross-section ratio for the (n,2n) reaction on 132,134Ba
- Measurement of photo-neutron cross sections and isomeric yield ratios in the 89Y(γ,xn)89−x Y reactions at the bremsstrahlung end-point energies of 65, 70 and 75 MeV
- Production, separation and target preparation of 171Tm and 147Pm for neutron cross section measurements
- Solid phase extraction of uranium from phosphoric acid: kinetic and thermodynamic study
- Natural silica sand modified by calcium oxide as a new adsorbent for uranyl ions removal from aqueous solutions
- Radiochemical separation of 231Pa from siliceous cake prior to its determination by gamma ray spectrometry
- Investigation of selenium compounds as targets for 76,77Br production using protons of energies up to 34 MeV
- Attenuation properties of radiation shielding materials such as granite and marble against γ-ray energies between 80 and 1350 keV
- Controlled release fertilizers using superabsorbent hydrogel prepared by gamma radiation
Articles in the same Issue
- Frontmatter
- Activation cross section and isomeric cross-section ratio for the (n,2n) reaction on 132,134Ba
- Measurement of photo-neutron cross sections and isomeric yield ratios in the 89Y(γ,xn)89−x Y reactions at the bremsstrahlung end-point energies of 65, 70 and 75 MeV
- Production, separation and target preparation of 171Tm and 147Pm for neutron cross section measurements
- Solid phase extraction of uranium from phosphoric acid: kinetic and thermodynamic study
- Natural silica sand modified by calcium oxide as a new adsorbent for uranyl ions removal from aqueous solutions
- Radiochemical separation of 231Pa from siliceous cake prior to its determination by gamma ray spectrometry
- Investigation of selenium compounds as targets for 76,77Br production using protons of energies up to 34 MeV
- Attenuation properties of radiation shielding materials such as granite and marble against γ-ray energies between 80 and 1350 keV
- Controlled release fertilizers using superabsorbent hydrogel prepared by gamma radiation