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Selective Fenton-like catalytic oxidation of acid orange II on inorganic heterogeneous molecular imprinted catalysts

  • Yanqun Song , Jiaobo Shang , Chuan Rong , Yinghui Wang , Yuanyuan Zhang EMAIL logo , Kefu Yu EMAIL logo and Liyuan Chen
Published/Copyright: February 11, 2017
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Journal of Advanced Oxidation Technologies
From the journal Journal of Advanced Oxidation Technologies Volume 20 Issue 1

Abstract

In order to realize the selective oxidation of Fenton-like reaction, an inorganic molecularly imprinted Fe/Al/SiO2 composite (IMIPF) was synthesized by sol-gel method using acid orange II as template. As a comparison, the Fe/Al/SiO2 composite without molecular imprinting was referred to as INIPF. The adsorption performance and Fenton-like catalytic selectivity were also studied with sodium dodecyl benzene sulfonate as the coexistence interference. Adsorption results in single systems and binary systems proved that IMIPF owned special molecular recognition and priority adsorption ability of the target pollutant. In addition, both IMIPF and INIPF exhibited high catalytic activity toward the degradation of acid orange II in single systems. Benefited from the preferential adsorption and Fenton-like activity, IMIPF could achieve the goal of selective removal of target pollutants at low concentration in the presence of other pollutants at high concentration in binary systems. Moreover, IMIPF possessed a wide applicable pH range and good reusability.

Keywords: molecular imprinting; acid orange II; priority adsorption; heterogeneous Fenton-like; selective removal

Funding statement: This research was supported by Nature Science Foundations of China (51668005, 21267002, 21367003, 41473118, and 41273139), the China Postdoctoral Science Foundation (No. 2016M592607, 2016M590846), the National Key Basic Research Program of China (No. 2013CB956102), Nature Foundations of Guangxi Province (2015GXNSFBB139009, 2014GXNSFAA118296, 2014GXNSFBA118217, 2013GXNSFEA053001) and the BaGui Scholars Program Foundation (2014).

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Received: 2016-8-15
Revised: 2016-10-4
Accepted: 2016-10-24
Published Online: 2017-2-11
Published in Print: 2017-1-1

© 2017 by Walter De Gruyter GmbH

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  4. Photooxidative Degradation of Pesticides in Water; Response Surface Modeling Approach
  5. The treatment of aniline in aqueous solutions by gamma irradiation
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  8. Catalytic Degradation of Safranin T in Aqueous Medium Using Non-conventional Processes
  9. Oxidation of 1, 2-dichlorobenzene on a commercial V2O5-WO3/nano-TiO2 catalyst: Effect of HCl addition
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  18. Reaction characteristics of oxygen generation from plate-like potassium superoxide within a confined space
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  20. Role of oxygen-containing functional surface groups of activated carbons on the elimination of 2-hydroxybenzothiazole from waters in A hybrid heterogeneous ozonation system
  21. The degradation efficiency and mechanism of meclofenamic acid in aqueous solution by UV irradiation
  22. Effect of electrode oxide film in micro arc oxidation on water treatment
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https://doi.org/10.1515/jaots-2016-0195
Keywords for this article
molecular imprinting; acid orange II; priority adsorption; heterogeneous Fenton-like; selective removal

Articles in the same Issue

  2. Editorial: The importance of advanced oxidation processes in degrading persistent pollutants
  3. An overview on heterogeneous Fenton and photoFenton reactions using zerovalent iron materials
  4. Photooxidative Degradation of Pesticides in Water; Response Surface Modeling Approach
  5. The treatment of aniline in aqueous solutions by gamma irradiation
  6. Microwave regeneration of biological activated carbon
  7. Molecular iodine/aqueous NH4OAc: a green reaction system for direct oxidative synthesis of nitriles from amines
  8. Catalytic Degradation of Safranin T in Aqueous Medium Using Non-conventional Processes
  9. Oxidation of 1, 2-dichlorobenzene on a commercial V2O5-WO3/nano-TiO2 catalyst: Effect of HCl addition
  10. Current conduction mechanisms in thermal nitride and dry gate oxide grown on 4H-silicon carbide (SiC)
  11. Effect of light and oxygen on repetitive bacterial inactivation on uniform, adhesive, robust and stable Cu-polyester surfaces
  12. Wet oxidation of an industrial high concentration pharmaceutical wastewater using hydrogen peroxide as an oxidant
  13. Oxidation characteristics of heavy crude oil in ignition process
  14. Comparative studies on the performance of porous Ti/Sno2-Sb2O3/Pbo2 enhanced by CNT and Bi Co-doped electrodes for methyl orange oxidation
  15. Application of photocatalytic paint for destruction of benzo[a]pyrene. Impact of air humidity
  16. Spray-drying synthesis and characterization of Li4Ti5O12 anode material for lithium ion batteries
  17. Kinetics analysis of photocatalytic degradation of Acid Orange 7 by Co/N/Er3+: Y3Al5O12/TiO2 films
  18. Reaction characteristics of oxygen generation from plate-like potassium superoxide within a confined space
  19. Electrochemical reduction of CO2 on a Cu2O/polyaniline /stainless steel based electrode
  20. Role of oxygen-containing functional surface groups of activated carbons on the elimination of 2-hydroxybenzothiazole from waters in A hybrid heterogeneous ozonation system
  21. The degradation efficiency and mechanism of meclofenamic acid in aqueous solution by UV irradiation
  22. Effect of electrode oxide film in micro arc oxidation on water treatment
  23. Photocurrent response and photocatalytic activity of Nd-doped TiO2 thin films prepared by sol-gel method
  24. Mathematical model involving chemical reaction and mass transfer for the ozonation of dimethyl phthalate in water in a bubble column reactor
  25. Elimination of organic micro-contaminants in municipal wastewater by a combined immobilized biomass reactor and solar photo-Fenton tertiary treatment
  26. Degradation of catechol on BiOCl: charge transfer complex formation and photoactivity
  27. Photocatalytic degradation of phenol on strontium titanate supported on HZSM-5
  28. Selective Fenton-like catalytic oxidation of acid orange II on inorganic heterogeneous molecular imprinted catalysts
  29. Decoloration of azo dye methyl orange by a novel electro-Fenton internal circulation batch reactor
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