Abstract
We investigate the performance of a piezoelectric energy harvester with nonlinearity induced by wrinkles. Linear and nonlinear regimes are detected in the electric response of the device when sweeping the intensity of the external excitation. Those regimes are related to the activation of a nonlinear mechanical response that appears when increasing the excitation amplitude. The wrinkles have been found to improve the power density and the normalized power density, in a certain noise power range.
Introduction
Energy Harvesting (EH) has demonstrated to be a good solution for the power needs of the so called Information and Communication Technologies (ICTs) when energy autonomy and wireless communication are required (Seah, Eu, and Tan 2009; Priya and Inman 2009;Paradiso and Starner 2005;Orfei et al. 2013;Ferrari et al. 2008; Vocca et al. 2012). The main goal of EH is to enable electronic devices to be operated without batteries and, to achieve this, a minimum amount of a few mW is needed.
The role of mechanical nonlinearities for energy harvesting purposes has been widely addressed in the last years (Gammaitoni et al. 2012;Guyomar et al. 2005). In particular, many efforts have been devoted to study and characterize the response of bistable systems under wide-band mechanical (Ferrari et al. 2010; Soliman et al. 2008; Stanton, McGehee, and Mann 2010;Arrieta et al. 2010) and their capability of increasing the generated electric power in com parisonto the power output of linear oscillators (i.e. resonators). Bi-stability is commonly induced by means of electromagnetic repulsion (Cottone, Vocca, and Gammaitoni 2009) electrostatic interaction (López-Suárez et al. 2013) or mechanical stress (Cottone et al. 2012; López-Suárez et al. 2011). However bi-stability is not the only kind of nonlinearity which could help to increase the performance of energy harvesting devices (Gammaitoni, Neri, and Vocca 2009).
In this paper we present an analysis of a nonlinear energy harvesting device based on a piezoelectric membrane which presents internal mechanical stresses produced during the fabrication process by applying thermal gradients. The consequent mechanical nonlinearity produces an increment in two figure’s of merit commonly used to describe the performance of EH devices: power density (PD) and normalized power density (NPD) (Roundy 2005;Beeby et al. 2007).

(a) Optical image of the piezoelectric membrane showing the electric paths contacting the upper and lower electrodes. (b) Schematic cross section of the structure showing the materials stack that form the harvester. (c) Schematic of the experimental setup.
Material and methods
The considered harvester is an aluminium nitride (AlN),
The wrinkled membrane is mechanically excited through an external piezoelectric shaker (Piezo System TS18-H5-202). The membrane is mounted on a PCB board and connected to the shaker though an opto-mechanical support. The setup of the experiment is presented in Figure 1(c). The value of acceleration (
The performances of the harvester are evaluated in terms of PD, defined as
and in terms of NPD, defined as
The volume is computed considering the dimension of the active part of the membrane.
Notice that the PD does not take into account the value of acceleration under which the harvester is subjected, while the NPD accounts only on the value of acceleration but does not consider the frequency content.

Power spectral density of acceleration with
Electrical Response
The optimal load,

Generated PD (squares) and NPD (solid line) under a broadband mechanical excitation. The red dashed-line represents the trend of the PD for a linear system (i.e. proportional to
In order to maximize the electrical power generated by the harvester, it is necessary to maximize the mechanical power of the system. The mechanical power is dissipated partially through the mechanical-electrical coupling mechanism (i.e. piezoelectric effect), and partially by the structural and viscous damping. The viscous damping is usually produced by the interaction with the surroundings (i.e. air), thus it is quite common to consider energy harvester operating in partial vacuum (Cavallier et al. 2005; Stephen 2006; Elfrink et al. 2009).The magnitude of the output power for piezoelectric linear generators is given by:
where

Generated PD (squares) and NPD (solid line) at
Higher Order Spectral Analysis
To investigate the nonlinear behavior in more detail, we perform a higher order spectral analysis, using the HOSA toolbox (MathWorks et al. 1998) in Matlab. In particular bispectrum and bicoherence analysis can give information on Gaussianity and linearity of the signal respectively. Similar information can be extracted by statistical test like the Hinich’s Gaussianity and linearity tests (Hinich 1982). Three different electrical signal responses have been selected for the Gaussianity and linearity tests. The first one refers to the harvester subjected to an acceleration of 2.9 g, where the system is in the linear regime, according to the trend highlighted in the inset of Figure 3. The second and the third refer respectively to acceleration of 8.6 g and 17.2 g, both in the nonlinear regime.

Bicoherence of three electric responses of the energy harvester. The first panel is relative to the electrical output of the harvester subjected to an acceleration of 2.9 g. This signal linear and only the resonant frequency is present on the plot. The second and third panels reefer to the electrical signal generated for a driving excitation of 8.6 g and 17.2 g, respectively. In those cases the signals are nonlinear and the plots show peaks out of the diagonal, indicating coupling, and thus energy transfer, between different frequencies.
By performing Gaussianity and linearity tests on the time-domain signals, using the respective functions from the HOSA toolbox, we find that for 2.9 g the system behaves linearly. The Hinich’s test reports a high probability of false alarm (
We now turn our attention to a more quantitative analysis of these nonlinearities, which appear to play a crucial role in the enhancement of the harvester response. The nonlinear interactions are examined by calculating the bicoherence of the generated piezoelectric signal under noise excitation, in the time-domain. In Figure 5 the bicoherence of three signals is presented. The first panel of Figure 5 is relative to the electrical output of the harvester subjected to an acceleration of 2.9 g. In this regime the system acts as a linear system and in fact the bicoherence analysis shows only one peak on the diagonal at the resonant frequency of the system. The second and third panels of Figure 5 reefer to the electrical signal generated for a driving excitation of 8.6 g and 17.2 g, respectively. In those cases the signals are not Gaussian and bicoherence is used to confirm nonlinearity. In those scenarios the bicoherence analysis shows a coupling between different modes of the system, that appears as an off-diagonal signal, indicating coupling, and thus energy transfer, between different frequencies. This behaviour is common in doubly clamped structures (Westra et al. 2010). In a harvester, this means that the response is enhanced as multiple modes participate in the transduction.
Conclusions
In conclusion we have measured the performance of a wrinkled piezoelectric energy harvester. We used two figures of merit to evaluate the response in linear and in the nonlinear regime. An optimum working point is found, by exploiting the nonlinearity that arises from the wrinkles. We investigated this nonlinearity in detail by measuring bicoherence, and found that the enhanced transduction can be explained by a significant coupling between the modes in the nonlinear regime. Our work suggests that wrinkled membranes offer an improved performance. It may have also consequences for energy harvesters based on 2-D materials, in which wrinkles occur naturally during fabrication.
Funding source: European Union’s Seventh Framework Programme (FP7/2007-2013) under Grant Agreement n.256959, NANOPOWER and Grant Agreement No. 318287, LANDAUER
Award Identifier / Grant number: 318287
Funding statement: The research leading to these results has received funding from the European Union’s Seventh Framework Programme (FP7/2007-2013) under Grant Agreement n.256959, NANOPOWER and Grant Agreement No. 318287, LANDAUER.
Acknowledgments
The authors wish to thank H. Vocca, L. Gammaitoni and W. Venstra for the useful discussions, and the VTT Technical Research Centre of Finland (Helsinki) for the membrane fabrication.
References
Arrieta, A., P. Hagedorn, A. Erturk, and D. Inman. 2010. “A Piezoelectric Bistable Plate for Nonlinear Broadband Energy Harvesting.” Applied Physics Letters 97:104102.10.1063/1.3487780Suche in Google Scholar
Beeby, S. P., R. Torah, M. Tudor, P. Glynne-Jones, T. O’Donnell, C. Saha, and S. Roy. 2007. “A Micro Electromagnetic Generator for Vibration Energy Harvesting.” Journal of Micromechanics and Microengineering 17:1257.10.1088/0960-1317/17/7/007Suche in Google Scholar
Cavallier, B., P. Berthelot, H. Nouira, E. Foltête, L. Hirsinger, S. Ballandras, et al. 2005. “Energy Harvesting Using Vibrating Structures Excited by Shock.” IEEE Ultrasonics Symposium 2:943–5.10.1109/ULTSYM.2005.1603006Suche in Google Scholar
Cottone, F., L. Gammaitoni, H. Vocca, M. Ferrari, and V. Ferrari. 2012. “Piezoelectric Buckled Beams for Random Vibration Energy Harvesting.” Smart Materials and Structures 21:035021.10.1088/0964-1726/21/3/035021Suche in Google Scholar
Cottone, F., H. Vocca, and L. Gammaitoni. 2009. Nonlinear Energy Harvesting.” Physical Review Letters 102:080601.10.1103/PhysRevLett.102.080601Suche in Google Scholar PubMed
Elfrink, R., T. Kamel, M. Goedbloed, S. Matova, D. Hohlfeld, Y. Van Andel, and R. Van Schaijk. 2009. “Vibration Energy Harvesting with Aluminum Nitride-Based Piezoelectric Devices.” Journal of Micromechanics and Microengineering 19:094005.10.1088/0960-1317/19/9/094005Suche in Google Scholar
Ferrari, M., V. Ferrari, M. Guizzetti, B. Andò, S. Baglio, and C. Trigona. 2010. “Improved Energy Harvesting from Wideband Vibrations by Nonlinear Piezoelectric Converters.” Sensors and Actuators A: Physical 162:425–31.10.1016/j.sna.2010.05.022Suche in Google Scholar
Ferrari, M., V. Ferrari, M. Guizzetti, D. Marioli, and A. Taroni. 2008. “Piezoelectric Multifrequency Energy Converter for Power Harvesting in Autonomous Microsystems.” Sensors and Actuators A: Physical 142:329–35.10.1016/j.sna.2007.07.004Suche in Google Scholar
Gammaitoni, L., I. Neri, and H. Vocca. 2009. “Nonlinear Oscillators for Vibration Energy Harvesting.” Applied Physics Letters 94:164102.10.1063/1.3120279Suche in Google Scholar
Gammaitoni, L., H. Vocca, I. Neri, F. Travasso, and F. Orfei. 2012. “Vibration Energy Harvesting: Linear and Nonlinear Oscillator Approaches.” In Sustainable Energy Harvesting Technologies-Past, Present and Future, edited by D. Y. K. Tan, 169–88. InTech: Croatia EU.10.5772/25623Suche in Google Scholar
Guyomar, D., A. Badel, E. Lefeuvre, and C. Richard. 2005.”Toward Energy Harvesting Using Active Materials and Conversion Improvement by Nonlinear Processing.” Ultrasonics, Ferroelectrics and Frequency Control, IEEE Transactions on 52:584–95.10.1109/TUFFC.2005.1428041Suche in Google Scholar
Hinich, M. J. 1982. “Testing for Gaussianity and Linearity of a Stationary Time Series.” Journal of Time Series Analysis 3:169–76.10.1111/j.1467-9892.1982.tb00339.xSuche in Google Scholar
López-Suárez, M., J. Agusti, F. Torres, R. Rurali, and G. Abadal. 2013. “Inducing Bistability with Local Electret Technology in a Microcantilever Based Non-linear Vibration Energy Harvester.”’ Applied Physics Letters 102:153901.10.1063/1.4800926Suche in Google Scholar
López-Suárez, M., R. Rurali, L. Gammaitoni, and G. Abadal. 2011. “Nanostructured Graphene for Energy Harvesting.” Physical Review B 84:161401.10.1103/PhysRevB.84.161401Suche in Google Scholar
MathWorks, I., A. Swami, J. M. Mendel, and C. L. Nikias. 1998. Higher-order Spectral Analysis Toolbox: for Use with MATLAB: User’s Guide. Mathworks, Incorporated.Suche in Google Scholar
Orfei, F., I. Neri, H. Vocca, and L. Gammaitoni. 2013. “Nonlinear Vibration Energy Harvesting at Work: An Application for the Automotive Sector.” In Circuits and Systems (ISCAS), 2013 IEEE International Symposium on, IEEE, 2735–2738.10.1109/ISCAS.2013.6572444Suche in Google Scholar
Paradiso, J. A. and T. Starner. 2005. “Energy Scavenging for Mobile and Wireless Electronics.” Pervasive Computing, IEEE 4:18–27.10.1109/MPRV.2005.9Suche in Google Scholar
Priya, S. and D. J. Inman. 2009. Energy Harvesting Technologies, vol. 21. Spinger: US.10.1007/978-0-387-76464-1Suche in Google Scholar
Roundy, S. 2005. “On the Effectiveness of Vibration-based Energy Harvesting.” Journal of Intelligent Material Systems and Structures 16:809–23.10.1177/1045389X05054042Suche in Google Scholar
Seah, W. K., Z. A. Eu, and H.-P. Tan. 2009. “Wireless Sensor Networks Powered by Ambient Energy Harvesting (WSN-Heap)-Survey and Challenges.” In Wireless Communication, Vehicular Technology, Information Theory and Aerospace & Electronic Systems Technology, 2009. Wireless VITAE 2009. 1st International Conference on, IEEE, 1–5.10.1109/WIRELESSVITAE.2009.5172411Suche in Google Scholar
Soliman, M., E. Abdel-Rahman, E. El-Saadany, and R. Mansour. 2008. “A Wideband Vibration-based Energy Harvester.” Journal of Micromechanics and Microengineering 18:115021.10.1088/0960-1317/18/11/115021Suche in Google Scholar
Stanton, S. C., C. C. McGehee, and B. P. Mann. 2010. “Nonlinear Dynamics for Broadband Energy Harvesting: Investigation of a Bistable Piezoelectric Inertial Generator.”’ Physica D: Nonlinear Phenomena 239:640–53.10.1016/j.physd.2010.01.019Suche in Google Scholar
Stephen, N. 2006. “On Energy Harvesting from Ambient Vibration.” Journal of Sound and Vibration 293:409–25.10.1016/j.jsv.2005.10.003Suche in Google Scholar
Vocca, H., I. Neri, F. Travasso, and L. Gammaitoni. 2012. “Kinetic Energy Harvesting with Bistable Oscillators.” Applied Energy 97:771–6.10.1016/j.apenergy.2011.12.087Suche in Google Scholar
Westra, H., M. Poot, H. Van der Zant, and W. Venstra. 2010. “Nonlinear Modal Interactions in Clamped-Clamped Mechanical Resonators.” Physical Review Letters 105:117205.10.1103/PhysRevLett.105.117205Suche in Google Scholar PubMed
©2016 by De Gruyter
Artikel in diesem Heft
- Frontmatter
- Articles
- Integrated Piezoelectric Energy Harvesting and Organic Storage System
- Design Considerations for Optimal Absorption of Energy from a Vibration Source by an Array of Harvesters
- Efficient Nonlinear Energy Harvesting with Wrinkled Piezoelectric Membranes
- Micro Wind Turbine for Powering Wireless Sensor Nodes
- Autonomous Flyback Converter for Energy Harvesting from Microbial Fuel Cells
- An Approach to a Flexible Thermoelectric Generator Fabricated using Bulk Materials
- Magnetoelectric Alternator
- Giant Magnetoelectric Effect in PZT Thin Film Deposited on Nickel
- Triboelectric Power Generation from Paper Vibration Induced by Sonic Waves
Artikel in diesem Heft
- Frontmatter
- Articles
- Integrated Piezoelectric Energy Harvesting and Organic Storage System
- Design Considerations for Optimal Absorption of Energy from a Vibration Source by an Array of Harvesters
- Efficient Nonlinear Energy Harvesting with Wrinkled Piezoelectric Membranes
- Micro Wind Turbine for Powering Wireless Sensor Nodes
- Autonomous Flyback Converter for Energy Harvesting from Microbial Fuel Cells
- An Approach to a Flexible Thermoelectric Generator Fabricated using Bulk Materials
- Magnetoelectric Alternator
- Giant Magnetoelectric Effect in PZT Thin Film Deposited on Nickel
- Triboelectric Power Generation from Paper Vibration Induced by Sonic Waves