Volume 3, Issue 6

We present a theoretical study of the optical angular momentum transfer from a circularly polarized plane wave to thin metal nanoparticles of different rotational symmetries. While absorption has been regarded as the predominant mechanism of torque generation on the nanoscale, we demonstrate numerically how the contribution from scattering can be enhanced by using multipolar plasmon resonance. The multipolar modes in non-circular particles can convert the angular momentum carried by the scattered field and thereby produce scattering-dominant optical torque, while a circularly symmetric particle cannot. Our results show that the optical torque induced by resonant scattering can contribute to 80% of the total optical torque in gold particles. This scattering-dominant torque generation is extremely mode-specific, and deserves to be distinguished from the absorption-dominant mechanism. Our findings might have applications in optical manipulation on the nanoscale as well as new designs in plasmonics and metamaterials.

Optical trapping and manipulation using focused laser beams has emerged as a powerful tool in the biological and physical sciences. However, scaling this technique to metallic nanoparticles remains challenging due to the strong scattering force and optical heating effect. In this work, we propose a novel strategy to optically trap metallic nanoparticles even under the resonant condition using engineered optical field. The distribution of the optical forces can be tailored through optimizing the spatial distribution of a vectorial optical illumination to favour the stable trapping of a variety of metallic nanoparticles under various conditions. It is shown that this optical tweezers has the ability of generating negative scattering force and supporting stable three-dimensional trapping for gold nanoparticles at resonance while avoiding trap destabilization due to optical overheating. The technique presented in this work offers a versatile solution for trapping metallic nanoparticles and may open up new avenues for optical manipulation.

Exploiting surface plasmon polaritons to enhance interactions between graphene and light has recently attracted much interest. In particular, nonlinear optical processes in graphene can be dramatically enhanced and controlled by plasmonic nanostructures. This work demonstrates Raman scattering enhancement in graphene based on plasmonic resonant enhancement of the Stokes emission, and compares this mechanism with the conventional Raman enhancement by resonant pump absorption. Arrays of optical nanoantennas with different resonant frequency are utilized to independently identify the effects of each mechanism on Raman scattering in graphene via the measured enhancement factor and its spectral linewidth. We demonstrate that, while both mechanisms offer large enhancement factors (scattering cross-section gains of 160 and 20 for individual nanoantennas, respectively), they affect the graphene Raman spectrum quite differently. Our results provide a benchmark to assess and quantify the role and merit of each mechanism in surface-plasmon-mediated Raman scattering in graphene, and may be employed for design and realization of a variety of graphene optoelectronic devices involving nonlinear optical processes.

Here the first photometric study of road-lighting white light-emitting diodes (WLEDs) integrated with semiconductor colloidal quantum dots (QDs) is reported enabling higher luminance than conventional light sources, specifically in mesopic vision regimes essential to street lighting. Investigating over 100 million designs uncovers that quality road-lighting QD-WLEDs, with a color quality scale and color rendering index ≥85, enables 13–35% higher mesopic luminance than the sources commonly used in street lighting. Furthermore, these QD-WLEDs were shown to be electrically more efficient than conventional sources with power conversion efficiencies ≥16–29%. Considering this fact, an experimental proof-of-concept QD-WLED was demonstrated, which is the first account of QD based color conversion custom designed for street lighting applications. The obtained white LED achieved the targeted mesopic luminance levels in accordance with the road lighting standards of the USA and the UK. These results indicate that road-lighting QD-WLEDs are strongly promising for energy-saving quality road lighting.

In order to detect biomolecules, different approaches using for instance biological, spectroscopic or imaging techniques are established. Due to the broad variety of these methods, this review is focused on surface enhanced Raman spectroscopy (SERS) as an analytical tool in biomolecule detection. Here, the molecular specificity of Raman spectroscopy is combined with metallic nanoparticles as sensor platform, which enhances the signal intensity by several orders of magnitude. Within this article, the characterization of diverse biomolecules by means of SERS is explained and moreover current application fields are presented. The SERS intensity and as a consequence thereof the reliable detection of the biomolecule of interest is effected by distance, orientation and affinity of the molecule towards the metal surface. Furthermore, the great capability of the SERS technique for cutting-edge applications like pathogen detection and cancer diagnosis is highlighted. We wish to motivate by this comprehensive and critical summary researchers from various scientific background to create their own ideas and schemes for a SERS-based detection and analysis of biomolecules.

The interaction of light and sound waves at the micro and nanoscale has attracted considerable interest in recent years. The main reason is that this interaction is responsible for a wide variety of intriguing physical phenomena, ranging from the laser-induced cooling of a micromechanical resonator down to its ground state to the management of the speed of guided light pulses by exciting sound waves. A common feature of all these phenomena is the feasibility to tightly confine photons and phonons of similar wavelengths in a very small volume. Amongst the different structures that enable such confinement, optomechanical or phoxonic crystals, which are periodic structures displaying forbidden frequency band gaps for light and sound waves, have revealed themselves as the most appropriate candidates to host nanoscale structures where the light-sound interaction can be boosted. In this review, we describe the theoretical tools that allow the modeling of the interaction between photons and acoustic phonons in nanoscale structures, namely cavities and waveguides, with special emphasis in phoxonic crystal structures. First, we start by summarizing the different optomechanical or phoxonic crystal structures proposed so far and discuss their main advantages and limitations. Then, we describe the different mechanisms that make light interact with sound, and show how to treat them from a theoretical point of view. We then illustrate the different photon-phonon interaction processes with numerical simulations in realistic phoxonic cavities and waveguides. Finally, we introduce some possible applications which can take enormous benefit from the enhanced interaction between light and sound at the nanoscale.