Article
Licensed
Unlicensed Requires Authentication

Research activities at GRS on fuel rod behaviour during extended dry storage

  • , , , and
Published/Copyright: January 23, 2019
Become an author with De Gruyter Brill

Abstract

As a common part of nuclear waste management strategies, used nuclear fuel is dry stored in casks. After a sufficient time of wet cooling in fuel pools, the fuel assemblies in Germany are dry stored in dual purpose casks mostly on-site until a deep geological repository will be available in the future. In the light of the extended and preliminary not foreseen timescales of up to 100 years of dry storage, open questions arise concerning the long term fuel rod behaviour. Most of these questions are linked to safety criteria e.g. the integrity and fuel encapsulation. Due to the variety of used nuclear fuels and cladding materials in Germany and the additional use of MOX fuels and very high burn-up values of 65 GWd/tHM averaged over a fuel assembly, some of the boundary conditions are unique and specific to the German situation. The GRS has a strong research program to investigate the long term behaviour of fuel assemblies under the German specific conditions of dry storage. Some aspects are presented in the following article.

Kurzfassung

Als gemeinsamer Bestandteil der Strategien zur Entsorgung nuklearer Abfälle wird der abgebrannte Kernbrennstoff trocken in Fässern gelagert. Nach einer ausreichenden Zeit der Nasskühlung in Lagerbecken werden die Brennelemente in Deutschland in Zweizweckbehältern meist vor Ort trocken gelagert, bis in Zukunft ein geologisches Tiefenlager zur Verfügung steht. Angesichts der verlängerten und vorläufigen, nicht vorhersehbaren Fristen von bis zu 100 Jahren Trockenlagerung stellen sich offene Fragen zum langfristigen Brennelementverhalten. Die meisten dieser Fragen sind mit Sicherheitskriterien wie z.B. der Integrität und der Kraftstoffverkapselung verbunden. Aufgrund der Vielfalt der verwendeten Kernbrennstoffe und Hüllstoffe in Deutschland und des zusätzlichen Einsatzes von MOX-Brennstoffen sowie sehr hoher Brennwerte von durchschnittlich 65 GWd/tHM über eine Brenneinheit sind einige der Randbedingungen einzigartig und spezifisch für die deutsche Situation. Die GRS verfügt über ein starkes Forschungsprogramm, um das Langzeitverhalten von Brennelementen unter den deutschen spezifischen Bedingungen der Trockenlagerung zu untersuchen. Einige Aspekte werden im folgenden Artikel vorgestellt.


* E-mail:

References

1 LombardoN. J.; et al.: COBRA-SFS: A Thermal-Hydraulic Analysis Computer Code, Volume III: Validation Assessments. Pacific Northwest Laboratory, December 198610.2172/6883584Search in Google Scholar

2 Michener, T. E.; Rector, D. R.; Cuta, J. M.; Adkins, Jr.H. E.: Cobra-SFS: A Thermal-Hydraulic Analysis Code For Spent Fuel Storage And Transportation Casks Cycle 4a. PNNL-24841, Pacific Northwest National Laboratory, October 201710.1080/00295450.2017.1305190Search in Google Scholar

3 RectorD. R.; et al.: COBRA-SFS: A Thermal-Hydraulic Analysis Computer Code, Volume I: Mathematical Models and Solution Method. Pacific Northwest Laboratory, November 198610.2172/6912964Search in Google Scholar

4 Rector, D. R.; et al.: COBRA-SFS: A Thermal-Hydraulic Analysis Computer Code, Volume II: User's Manual. Pacific Northwest Laboratory, November 198610.2172/6928785Search in Google Scholar

5 Ayachit, U.: The ParaView Guide: A Parallel Visualization Application. Kitware, ISBN 978-1930934306, 2015Search in Google Scholar

6 Stewering, J.; Schwarz, S.; Sonnenkalb, M.: Berechnung der Brennstabhüllrohr-temperaturen in einem generischen Transport- und Lagerbehälter. GRS Technical Report, April 2014Search in Google Scholar

7 GRS gGmbH: COCOSYS: https://www.grs.de/en/content/cocosys; 11.07.2018Search in Google Scholar

8 ANSYS CFX: https://www.ansys.com/products/fluids/ansys-cfx; 11.07.2018Search in Google Scholar

9 Hunter, J. D.; Matplotlib: A 2D graphics environment, Computing In Science & Engineering9 (2007) 9095, IEEE Compute Soc. 10.1109/MCSE.2007.55Search in Google Scholar

10 Sonnenburg, H.-G.; Boldt, F.: Brennstabverhalten im Normalbetrieb, bei Störfällen und bei Langzeitlagerung. GRS-Bericht: GRS – 464, ISBN 978-3-946607-47-2, August 2017Search in Google Scholar

11 Sonnenburg, H.-G.: TESPA-ROD code prediction of the fuel rod behaviour during long-term storage, In: International Journal for Nuclear Power atw, Vol. 63, Issue 6/7 (2018), 374377Search in Google Scholar

12 Raynaud, P.; Einziger, R.: Cladding stress during extended storage of high burnup spent nuclear fuel, Journal of Nuclear Materials464 (2015) 30431210.1016/j.jnucmat.2015.05.008Search in Google Scholar

13 U.S. Department of Energy (DOE): Three dimensional Fuel Pin Model Validation by Prediction of Hydrogen Distribution in Cladding and Comparison with Experiment. Final Report DOE Nuclear Energy University Program (NEUP), Project No. 13–5180, 2018Search in Google Scholar

14 Cinbiz, M. N.; KossD. A.; MottaA. T.: The Effect of Stress Biaxiality on Hydride Reorientation Threshold Stress. PennState University, TopFuel 2015, September 13–17, 2015, Zurich, Switzerland, paper A0151Search in Google Scholar

15 Herb, J.; Sievers, J.; Sonnenburg, H.-G.: A new cladding embrittlement criterion derived from ring compression tests, Nuclear Engineering and Design273 (2014) 61563010.1016/j.nucengdes.2014.03.047Search in Google Scholar

16 Marino, G.: Hydrogen supercharging in zircaloy, Materials Science and Engineering7 (1971) 33534110.1016/0025-5416(71)90016-4Search in Google Scholar

17 Kearns, J.: Terminal solubility and partitioning of hydrogen in the alpha phase of zirconium, zircaloy-2 and zircaloy-4, Journal of Nuclear Materials22 (1967) 29230310.1016/0022-3115(67)90047-5Search in Google Scholar

18 Sawatzky, A.; Wilkins, B.: Hydrogen solubility in zirconium alloys determined by thermal diffusion, Journal of Nuclear Materials22 (1967) 30431010.1016/0022-3115(67)90048-7Search in Google Scholar

19 Slattery, G.: The terminal solubility of hydrogen in zirconium alloys between 30 and 400°C, Journal of the Institute of Metals95 (1967) 743Search in Google Scholar

20 McMinn, A.; Darby, E.; Schonfield, J.: The terminal solid solubility of hydrogen in zirconium alloys, Zirconium in the Nuclear Industry. Proceedings of the 12th International Symposium on Zirconium in the Nuclear Industry, 173–195, 200010.1520/STP14300SSearch in Google Scholar

21 Blackmur, M. S.; Robson, J. D.; Preuss, M.; Zanellato, O.; Cernik, R. J.; Shi, S.-Q.; Ribeiro, F.; Andrieux, J.: Zirconium hydride precipitation kinetics in zircaloy-4 observed with synchrotron X-ray diffraction, Journal of Nuclear materials464 (2015) 16016910.1016/j.jnucmat.2015.04.025Search in Google Scholar

22 Pan, Z.; Ritchie, I.; Puls, M.: The terminal solid solubility of hydrogen and deuterium in Zr-2.5 Nb alloys, Journal of Nuclear Materials228 (1996) 22723710.1016/S0022-3115(95)00217-0Search in Google Scholar

23 Barrow, A. T. W.; Toffolon-Masclet, C.; Almer, J.; Daymond, M. R.: The role of chemical free energy and elastic strain in the nucleation of zirconium hydride, Journal of Nuclear Materials441 (2013) 39540110.1016/j.jnucmat.2013.06.013Search in Google Scholar

24 Denisov, E. A.; Kompaniets, T. N.; Voyt, A. P.: Kinetics of the isothermal decomposition of zirconium hydride: terminal solid solubility for precipitation and dissolution, Journal of Nuclear Materials503 (2018) 19519710.1016/j.jnucmat.2018.03.007Search in Google Scholar

25 Sonnenburg, H. G.; Boldt, F.: Dynamic Hydride Precipitation During LOCA Quench Process can Significantly Preserve Cladding's Ductility. TopFuel2018, paper A0187, Prague (2018)Search in Google Scholar

Received: 2018-09-11
Published Online: 2019-01-23
Published in Print: 2018-12-17

© 2018, Carl Hanser Verlag, München

Downloaded on 8.4.2026 from https://www.degruyterbrill.com/document/doi/10.3139/124.110950/html
Scroll to top button