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Linear, spatio-temporally resolved ultrasound measurement of the liquid fraction distribution in froth

  • Hannes Emmerich

    Hannes Emmerich studied mechatronics at the TU Dresden and received his Diploma in 2019. Since 2020, he is a research fellow with the laboratory for measurement and sensor system techniques and member of the ultrasound imaging group. His research currently focusses on ultrasound measurement methods in the low kilohertz range. High attenuating materials as liquid foam restrict typical measurement methods. Overcoming this problem by using new materials, image and signal processing is therefore his main goal.

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    , Ludwig Schaller

    Ludwig Schaller was born in Schweinfurt, Germany, in 1993. He studied electrical engineering at the TU Dresden and received his Diploma degree in 2020. Since 2021 he has been a research assistant at the laboratory for measurement and sensor system techniques. He is a member of the ultrasound imaging group. His research interests include ultrasound measurement methods, signal processing and the development of electronic prototypes.

    , Richard Nauber

    Richard Nauber (Member, IEEE) received the Diploma degree in mechatronics and the Dr.Ing. degree in electrical engineering from the Technische Universität Dresden (TU Dresden), Dresden, Germany, in 2010 and 2018, respectively. He worked as an Embedded Software Developer for a renewable energy company afterwards. Since 2012, he has been a Research Fellow and Head of the Ultrasound Imaging Group at the Laboratory of Measurement and Sensor System Techniques. He currently works as Postdoctoral Researcher in the Micro- and Nanobiomedical Engineering Group at Leibniz IFW Dresden. His research interests include computational ultrasound and photoacoustical imaging especially for biomedical applications. Dr. Nauber received the Best Dissertation Award from the Gisela und Erwin Sick Foundation in 2018.

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    , Leon Knüpfer

    Leon Knüpfer studied mechanical engineering at the TU Dresden, where he graduated in 2020. Currently he is a research fellow with the institute of fluid dynamics at the Helmholtz-Zentrum Dresden-Rossendorf. His main research interests include the development of experimental techniques for characterization of liquid foam.

    , Sascha Heitkam

    Sascha Heitkam studied mechanical engineering at the TU Dresden and graduated best of class in 2010. In 2014 he received a Ph.D. (cotutelle) from the TU Dresden and the Université Paris Sud in the field of fluid mechanics. Since then, he is a research fellow and project leader at TU Dresden and Helmholtz-Zentrum Dresden-Rossendorf. Since 2018 he heads the group of Multiphase Flow and Measurement in the department of Transport Processes at Interfaces. Since 2020 he also heads an Emmy-Noether research group regarding Fluid Mechanics of Foam and Froth. His main research interest is the development of measurement techniques for aqueous foam and their application in generic flows as well as in froth flotation.

    , Jürgen Czarske

    Jürgen Czarske (SM’15) has received the Diploma and the Ph.D. degrees from Leibniz University of Hannover, Germany. From 1986 to 1991, he was supported by a scholarship from the company Siemens AG. From 1991 to 1996, he was with the Leibniz University. From 1995 to 2004, he was responsible for metrology at the Laser Center Hannover (LZH e. V.). As a visiting scholar, he conducted research in Japan and the USA from 1996 to 2001. Since 2004, he is the director of the Laboratory of Measurement and Sensor System Technique. Since January 2016, he is director of the Institute of Circuits and Systems. His awards include the 1996 AHMT Measurement Technology Award, one 2008 Berthold Leibinger Innovation Award, one 2014 Reinhart Koselleck project of the German Research Foundation, the 2019 Joseph Fraunhofer Prize and the Robert M. Burley Prize of the Optical Society (OSA) and the 2020 Laser Instrumentation Award of IEEE Photonics Society. Jürgen is associate editor of the Journal of the European Optical Society – Rapid Publications, advisor of the Student Chapter Dresden of SPIE, elected member of the Saxon Academy of Sciences and the Scientific Society for Laser Technology (WLT e. V.). Jürgen has published around 200 international articles in peer-reviewed journals, held over 100 invited lectures and holds more than 20 patents. His research aims on the universal control and application of coherent waves using adaptive digital systems. Jürgen is Life Fellow of OSA and SPIE, Fellow of EOS and IET (formerly IEE), and senior member of IEEE.

    and Lars Büttner

    Lars Büttner studied physics at Clausthal University of Technology, Clausthal-Zellerfeld, Germany. Since 1999, he was a research fellow with the Laser Zentrum Hannover (LZH e. V.), Germany. He received a Ph.D. degree in physics from Leibniz Universität Hannover, in 2004. Since 2005, he has been with TU Dresden, Germany, where he is currently the head of the Flow Measurement and Adaptive Laser Systems Group at the Laboratory of Measurement and Sensor System Technique. His current research interests include laser- and ultrasound-based measurement techniques and adaptive optical systems. He is co-recipient of the international Berthold Leibinger Innovation Prize (3rd prize) in 2008.

Published/Copyright: July 23, 2021

Abstract

Froth flotation is an important process for separating metal particles from gangue. A single flotation circuit for copper uses approx. 44 billion litres water a year. In situ process monitoring of the foam’s parameters and closed-loop control can reduce the resource use. However, no measurement technique is broadly employed that yields the liquid fraction distribution in the froth. Optical measurements are prevented by the bulk foam’s opacity. Though, ultrasound in the low frequency range is able to penetrate froth.

In this paper we investigate the application of ultrasound to measure the local liquid content of aqueous foam in the axis of the ultrasound beam. Assuming a dependency of the backscattering coefficient b on the foam’s liquid fraction ϕ, we developed a model to calculate b from the echo signal. Local backscattering coefficients b n can be determined for time gated windows and show a trend in the dependency on the foam’s liquid fraction ϕ (for ϕ < 0.8 %). The absolute uncertainty of the liquid fraction determined by means of an electrical reference measurement is σ ϕ = 0.079 %.

We demonstrated the capability of spatio-temporally resolved measurements with a frame rate of 0.33 Hz and an axial resolution of 7.9 mm in an experiment with a time-varying, inhomogeneous liquid fraction. This research work is contributing to a determination of in situ information of the foam’s parameter in a flotation process.

Zusammenfassung

Schaumflotation ist ein wichtiges Verfahren zur Trennung von Metallpartikeln vom tauben Gestein. Ein einziger Flotationskreislauf für Kupfer verbraucht ca. 44 Milliarden Liter Wasser pro Jahr. Eine In situ Prozessüberwachung der Schaumparameter und eine geschlossene Regelung können den Ressourcenverbrauch reduzieren. Dennoch ist keine Messtechnik etabliert, die den Flüssigkeitsgehalt im Schaum ermittelt. Optische Messungen werden durch die Opazität des Schaums verhindert. Geeignete In-situ-Messtechnik, insbesondere hinsichtlich der Strömung und der Zusammensetzung des Schaums, sind daher erforderlich. Ultraschall im niederen Frequenzbereich ist jedoch in der Lage, den Schaum zu durchdringen. In dieser Arbeit untersuchen wir die Anwendung von Ultraschall zur Messung des lokalen Flüssigkeitsgehaltes in wässrigem Schaum auf der Achse der Ultraschallausbreitung. Unter der Annahme einer Abhängigkeit des Rückstreuungskoeffizienten b vom Flüssigkeitsgehalt ϕ des Schaums entwickelten wir ein Modell zur Berechnung von b aus dem Echoignal. Lokale Rückstreuungskoeffizienten b n können für explizite Zeitfenster bestimmt werden und zeigen einen Trend in Abhängigkeit vom Flüssigkeitsgehalt des Schaums ϕ (für ϕ < 0 , 8 %). Die absolute Unsicherheit der Bestimmung des Flüssigkeitsgehaltes unter Nutzung einer elektrischen Referenz beträgt σ ϕ = 0 , 079 %. In einem Experiment mit zeitlich veränderlichem, inhomogenem Flüssigkeitsanteil haben wir die Möglichkeit aufgezeigt eine räumlich und zeitlich aufgelöste Messungen mit einer Bildrate von 0.33 Hz und einer axialen Auflösung von 7.9 mm durchzuführen. Diese Forschungsarbeit trägt dazu bei, in situ Informationen über die Parameter des Schaums in einem Flotationsprozess zu ermitteln.

Award Identifier / Grant number: 21151 BR

Funding statement: The IGF project No. 21151 BR of the research association DECHEMA, Gesellschaft für Chemische Technik und Biotechnologie e. V., Theodor-Heuss-Allee 25, 60486 Frankfurt am Main, Germany, was funded by the German Federal Ministry for Economic Affairs and Energy through the German Federation of Industrial Research Associations (AiF) within the framework of the program for the promotion of joint industrial research (IGF) on the basis of a resolution of the German Bundestag.

About the authors

Hannes Emmerich

Hannes Emmerich studied mechatronics at the TU Dresden and received his Diploma in 2019. Since 2020, he is a research fellow with the laboratory for measurement and sensor system techniques and member of the ultrasound imaging group. His research currently focusses on ultrasound measurement methods in the low kilohertz range. High attenuating materials as liquid foam restrict typical measurement methods. Overcoming this problem by using new materials, image and signal processing is therefore his main goal.

Ludwig Schaller

Ludwig Schaller was born in Schweinfurt, Germany, in 1993. He studied electrical engineering at the TU Dresden and received his Diploma degree in 2020. Since 2021 he has been a research assistant at the laboratory for measurement and sensor system techniques. He is a member of the ultrasound imaging group. His research interests include ultrasound measurement methods, signal processing and the development of electronic prototypes.

Richard Nauber

Richard Nauber (Member, IEEE) received the Diploma degree in mechatronics and the Dr.Ing. degree in electrical engineering from the Technische Universität Dresden (TU Dresden), Dresden, Germany, in 2010 and 2018, respectively. He worked as an Embedded Software Developer for a renewable energy company afterwards. Since 2012, he has been a Research Fellow and Head of the Ultrasound Imaging Group at the Laboratory of Measurement and Sensor System Techniques. He currently works as Postdoctoral Researcher in the Micro- and Nanobiomedical Engineering Group at Leibniz IFW Dresden. His research interests include computational ultrasound and photoacoustical imaging especially for biomedical applications. Dr. Nauber received the Best Dissertation Award from the Gisela und Erwin Sick Foundation in 2018.

Leon Knüpfer

Leon Knüpfer studied mechanical engineering at the TU Dresden, where he graduated in 2020. Currently he is a research fellow with the institute of fluid dynamics at the Helmholtz-Zentrum Dresden-Rossendorf. His main research interests include the development of experimental techniques for characterization of liquid foam.

Sascha Heitkam

Sascha Heitkam studied mechanical engineering at the TU Dresden and graduated best of class in 2010. In 2014 he received a Ph.D. (cotutelle) from the TU Dresden and the Université Paris Sud in the field of fluid mechanics. Since then, he is a research fellow and project leader at TU Dresden and Helmholtz-Zentrum Dresden-Rossendorf. Since 2018 he heads the group of Multiphase Flow and Measurement in the department of Transport Processes at Interfaces. Since 2020 he also heads an Emmy-Noether research group regarding Fluid Mechanics of Foam and Froth. His main research interest is the development of measurement techniques for aqueous foam and their application in generic flows as well as in froth flotation.

Jürgen Czarske

Jürgen Czarske (SM’15) has received the Diploma and the Ph.D. degrees from Leibniz University of Hannover, Germany. From 1986 to 1991, he was supported by a scholarship from the company Siemens AG. From 1991 to 1996, he was with the Leibniz University. From 1995 to 2004, he was responsible for metrology at the Laser Center Hannover (LZH e. V.). As a visiting scholar, he conducted research in Japan and the USA from 1996 to 2001. Since 2004, he is the director of the Laboratory of Measurement and Sensor System Technique. Since January 2016, he is director of the Institute of Circuits and Systems. His awards include the 1996 AHMT Measurement Technology Award, one 2008 Berthold Leibinger Innovation Award, one 2014 Reinhart Koselleck project of the German Research Foundation, the 2019 Joseph Fraunhofer Prize and the Robert M. Burley Prize of the Optical Society (OSA) and the 2020 Laser Instrumentation Award of IEEE Photonics Society. Jürgen is associate editor of the Journal of the European Optical Society – Rapid Publications, advisor of the Student Chapter Dresden of SPIE, elected member of the Saxon Academy of Sciences and the Scientific Society for Laser Technology (WLT e. V.). Jürgen has published around 200 international articles in peer-reviewed journals, held over 100 invited lectures and holds more than 20 patents. His research aims on the universal control and application of coherent waves using adaptive digital systems. Jürgen is Life Fellow of OSA and SPIE, Fellow of EOS and IET (formerly IEE), and senior member of IEEE.

Lars Büttner

Lars Büttner studied physics at Clausthal University of Technology, Clausthal-Zellerfeld, Germany. Since 1999, he was a research fellow with the Laser Zentrum Hannover (LZH e. V.), Germany. He received a Ph.D. degree in physics from Leibniz Universität Hannover, in 2004. Since 2005, he has been with TU Dresden, Germany, where he is currently the head of the Flow Measurement and Adaptive Laser Systems Group at the Laboratory of Measurement and Sensor System Technique. His current research interests include laser- and ultrasound-based measurement techniques and adaptive optical systems. He is co-recipient of the international Berthold Leibinger Innovation Prize (3rd prize) in 2008.

References

1. D. Bleiwas, “Estimated water requirements for the conventional flotation of copper ores, ” U.S. Geological Survey Open-File Report, 2012.10.3133/ofr20121085Search in Google Scholar

2. I. O. Ogunniyi and M. K. G. Vermaak, “Froth flotation for beneficiation of printed circuit boards comminution fines: An overview,” Mineral Processing and Extractive Metallurgy Review, vol. 30, no. 2, pp. 101–121, 2009.10.1080/08827500802333123Search in Google Scholar

3. K. A. Matis and P. Mavros, “Foam/froth flotation part ii. Removal of particulate matter,” Separation & Purification Reviews, vol. 20, no. 2, pp. 163–198, 1991.10.1080/03602549108021414Search in Google Scholar

4. M. Vera, A. Saint-Jalmes, and D. Durian, “Scattering optics of foam,” Applied optics, vol. 40, pp. 4210–4214, 09 2001.10.1364/AO.40.004210Search in Google Scholar

5. T. Lappan, A. Franz, H. Schwab, U. Kühn, S. Eckert, K. Eckert, and S. Heitkam, “X-ray particle tracking velocimetry in liquid foam flow,” Soft Matter, vol. 16, pp. 2093–2103, 2020.10.1039/C9SM02140JSearch in Google Scholar

6. S. Heitkam, M. Rudolph, T. Lappan, M. Sarma, S. Eckert, P. Trtik, E. Lehmann, P. Vontobel, and K. Eckert, “Neutron imaging of froth structure and particle motion,” Minerals Engineering, vol. 119, pp. 126–129, 2018.10.1016/j.mineng.2018.01.021Search in Google Scholar

7. B. Shean and J. Cilliers, “A review of froth flotation control,” International Journal of Mineral Processing, vol. 100, no. 3, pp. 57–71, 2011.10.1016/j.minpro.2011.05.002Search in Google Scholar

8. I. Ben Salem, R.-M. Guillermic, C. Sample, V. Leroy, A. Saint-Jalmes, and B. Dollet, “Propagation of ultrasound in aqueous foams: Bubble size dependence and resonance effects,” Soft Matter, vol. 9, pp. 1194–1202, 12 2012.10.1039/C2SM25545FSearch in Google Scholar

9. J. Pierre, F. Elias, and V. Leroy, “A technique for measuring velocity and attenuation of ultrasound in liquid foams,” Ultrasonics, vol. 53, no. 2, pp. 622–629, 2013.10.1016/j.ultras.2012.10.011Search in Google Scholar PubMed

10. M. Wolf, L. Timmermann, A. Juhrig, K. Rath, E. Leipner, F. Krujatz, and E. Kühnicke, “Ultrasonic temperature monitoring in tissue phantoms by locally resolved measurement of longitudinal and transverse wave speed,” Proceedings of Meetings on Acoustics, vol. 38, no. 1, p. 020004, 2019.10.1121/2.0001076Search in Google Scholar

11. R. Nauber, L. Büttner, K. Eckert, J. Fröhlich, J. Czarske, and S. Heitkam, “Ultrasonic measurements of the bulk flow field in foams,” Phys. Rev. E, vol. 97, p. 013113, 01 2018.10.1103/PhysRevE.97.013113Search in Google Scholar PubMed

12. P. Kowalczuk and J. Drzymala, “Physical meaning of the sauter mean diameter of spherical particulate matter,” Particulate Science and Technology, vol. 34, pp. 645–647, 10 2015.10.1080/02726351.2015.1099582Search in Google Scholar

13. S. Heitkam and K. Eckert, “Convective instability in sheared foam,” Journal of Fluid Mechanics, vol. 911, p. A54, 2021.10.1017/jfm.2020.1062Search in Google Scholar

14. K. Feitosa, S. Marze, A. Saint-Jalmes, and D. J. Durian, “Electrical conductivity of dispersions: From dry foams to dilute suspensions,” Journal of Physics Condensed Matter, vol. 17, no. 41, pp. 6301–6305, 2005.10.1088/0953-8984/17/41/001Search in Google Scholar

15. C. Kupsch, L. Feierabend, R. Nauber, L. Büttner, and J. Czarske, “Flow investigation of complex suspension electrodes for battery applications using ultrasound imaging velocimetry,” Experimental Thermal and Fluid Science, vol. 109, p. 109886, 2019.10.1016/j.expthermflusci.2019.109886Search in Google Scholar

16. M. Kalibatas, R. Nauber, C. Kupsch, and J. Czarske, “Flow field imaging with ultrasonic guided waves for exploring metallic melts,” IEEE Transactions on Ultrasonics, Ferroelectrics, and Frequency Control, vol. 65, pp. 112–119, 2018.10.1109/TUFFC.2017.2771525Search in Google Scholar PubMed

17. C. Kupsch, L. Feierabend, R. Nauber, L. Büttner, and J. Czarske, “Ultrasound super-resolution flow measurement of suspensions in narrow channels,” IEEE Transactions on Ultrasonics, Ferroelectrics, and Frequency Control, pp. 1–1, 2020.10.1109/TUFFC.2020.3007483Search in Google Scholar PubMed

18. K. Mäder, R. Nauber, V. Galindo, H. Beyer, L. Büttner, S. Eckert, and J. Czarske, “Phased array ultrasound system for planar flow mapping in liquid metals,” IEEE Transactions on Ultrasonics, Ferroelectrics, and Frequency Control, vol. 64, no. 9, pp. 1327–1335, 2017.10.1109/TUFFC.2017.2693920Search in Google Scholar PubMed

19. D. Dawidowski, R. Nauber, L. Büttner, and J. Czarske, “Time reversal ultrasound focusing through multimode waveguides,” tm – Technisches Messen, vol. 84, no. 9, pp. 568–574, 2017.10.1515/teme-2016-0062Search in Google Scholar

20. K. Mäder, R. Nauber, H. Beyer, A. Klaß, N. Thieme, L. Büttner, and J. Czarske, “Modular ultrasound platform for flow mapping in magnetohydrodynamics,” tm – Technisches Messen, vol. 82, no. 11, pp. 578–584, 2015.10.1515/teme-2015-0084Search in Google Scholar

21. M. Vogt and H. Ermert, “Quantitative analysis of liquids and emulsions by means of high-frequency ultrasound (15–35 mhz),” in 2011 IEEE International Ultrasonics Symposium, pp. 68–71, 2011.10.1109/ULTSYM.2011.0018Search in Google Scholar

22. I. Cantat, S. Cohen-Addad, F. Elias, F. Graner, R. Hoehler, O. Pitois, F. Rouyer, and A. Saint-Jalmes, Foams Structure and Dynamics. Great Clarendon Street, Oxford, OX2 6DP, United Kingdom: Oxford University Press, 2013.10.1093/acprof:oso/9780199662890.001.0001Search in Google Scholar

23. P. Del, A. Chinnayya, L. Domergue, A. Hadjadj, and J.-F. Haas, “Blast wave mitigation by dry aqueous foams,” Shock Waves, vol. 23, 02 2012.10.1007/s00193-012-0400-0Search in Google Scholar

24. R. Weser, S. Wöckel, B. Wessely, and U. Hempel, “Particle characterisation in highly concentrated dispersions using ultrasonic backscattering method,” Ultrasonics, vol. 53, no. 3, pp. 706–716, 2013.10.1016/j.ultras.2012.10.013Search in Google Scholar PubMed

25. J. J. Faran, “Sound scattering by solid cylinders and spheres,” The Journal of the Acoustical Society of America, vol. 23, no. 4, pp. 405–418, 1951.10.1121/1.1906780Search in Google Scholar

26. Q. Xu, Y.-Z. Liang, and Y.-P. Du, “Monte carlo cross-validation for selecting a model and estimating the prediction error in multivariate calibration,” Journal of Chemometrics, vol. 18, pp. 112–120, 02 2004.10.1002/cem.858Search in Google Scholar

27. “GUM evaluation of measurement data – guide to the expression of uncertainty in measurement.” https://www.bipm.org/en/publications/guides/gum.html. Accessed: 2021-03-08.Search in Google Scholar

28. L. Büttner, R. Nauber, M. Burger, D. Räbiger, S. Franke, S. Eckert, and J. Czarske, “Dual-plane ultrasound flow measurements in liquid metals,” Measurement Science and Technology, vol. 24, p. 055302, 03 2013.10.1088/0957-0233/24/5/055302Search in Google Scholar

29. M. Burger, R. Nauber, M. Neumann, L. Büttner, and J. Czarske, “Modulares ultraschall-array-doppler-velozimeter zur messung von komplexen strömungen in flüssigmetallen,” tm – Technisches Messen, vol. 79, no. 9, pp. 417–425, 2012.10.1524/teme.2012.0266Search in Google Scholar

30. R. Nauber, L. Büttner, and J. Czarske, “Measurement uncertainty analysis of field-programmable gate-array-based, real-time signal processing for ultrasound flow imaging,” Journal of Sensors and Sensor Systems, vol. 9, no. 2, pp. 227–238, 2020.10.5194/jsss-9-227-2020Search in Google Scholar

Received: 2021-03-19
Accepted: 2021-06-27
Published Online: 2021-07-23
Published in Print: 2021-09-26

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