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Destruction of Volatile Organic Compounds in Air by a Superimposed Barrier Discharge Plasma Reactor and Activated Carbon Filter Hybrid System

  • K. Urashima , T. Misaka , T. Ito and J.-S. Chang
Published/Copyright: November 30, 2016
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Abstract

Superimposed barrier discharge and activated carbon filter hybrid systems were used to remove toluene and TCE from air streams. The superimposed barrier-discharge consisted of silent and surface discharges. Experiments were conducted for the gas flow rates from 1 to 10 L/min, applied power from 0 to 7 W and toluene and TCE initial concentrations from 0 to 2,000 ppm for 60 Hz ac applied voltage conditions. Discharge by-products were measured by FTIR, GC, and TLV-VOC detectors. The results show that 1) the toluene-decomposition efficiency monotonically increases with increasing applied power; 2) approximately 90% of the toluene is removed by the plasma reactors and up to 98% is removed by the hybrid system; 3) TCE removal is enhanced by the hybrid system and up to 50% is removed by a discharge reactor alone; 4) the pressure drop of the reactor and carbon filter increase with increasing gas flow rate; 5) TCE is decomposed to form CO2, H2O and Cl2 and, except for the CO2 and H2O, these discharge by-products are absorbed in the activated carbon filters; 6) no COCl2 , HCl, CO, NOx and O3 are observed in the discharge by-products; and 7) the energy yield for toluene decomposition is as high as 26 g/kWh, and as high as 15 g/kWh for TCE decomposition.

Received: 2000-9-6
Revised: 2001-6-4
Accepted: 2001-7-27
Published Online: 2016-11-30
Published in Print: 2002-7-1

© 2016 by Walter de Gruyter Berlin/Boston

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  2. Destruction of Volatile Organic Compounds in Air by a Superimposed Barrier Discharge Plasma Reactor and Activated Carbon Filter Hybrid System
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