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Sorption behavior of natural uranium from aqueous solutions using modified activated carbon with quinoline

  • Soaad M. Elashry , Shiraz Labib EMAIL logo and Mohamed F. Attallah
Published/Copyright: December 22, 2021
Radiochimica Acta
From the journal Radiochimica Acta Volume 110 Issue 3

Abstract

The activated carbon (AC) was modified by molecules of quinoline (Q) and the new prepared AC impregnated by Q was characterized using Fourier transform infrared (FTIR), Raman spectroscopy, surface measurements, scanning electron microscope (SEM) and transmission electron microscope (TEM). These analytical techniques demonstrated a successful preparation of AC-Q as a new material which was examined for its sorption behavior for natural uranium. The sorption results by batch mode indicated the optimum conditions for 94.5% removal of U(VI) ions at pH 4.7 and an equilibrium contact time of 90 min. The analysis of sorption data revealed that the pseudo-second-order and Langmuir were more fitted than other estimated models. The sorption capacity of U(VI) was ∼63 mg/g onto AC-Q as adsorbent martial. The thermodynamic data demonstrated that the sorption of uranium is endothermic and spontaneous. New mechanism was supposed based on the role of the abrasive material quinoline on the mechanical removal of uranium from aqueous solution.

Keywords: activated carbon; quinoline; sorption; uranium
Corresponding author: Shiraz Labib, Nuclear Chemistry Department, Hot Laboratories Center, Egyptian Atomic Energy Authority, 13759 Abu Zaabal, Cairo, Egypt, E-mail:

  1. Author contributions: All the authors have accepted responsibility for the entire content of this submitted manuscript and approved submission.

  2. Research funding: This research did not receive any specific grant from funding agencies in the public, commercial, or not-for-profit sectors.

  3. Conflict of interest statement: The authors declare that they have no compete of interest.

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Received: 2021-06-24
Accepted: 2021-12-06
Published Online: 2021-12-22
Published in Print: 2022-03-28

© 2021 Walter de Gruyter GmbH, Berlin/Boston

Articles in the same Issue

  1. Frontmatter
  2. Original Papers
  3. Sorption behavior of natural uranium from aqueous solutions using modified activated carbon with quinoline
  4. Adsorption of UO2 2+ by AlBaNi-layered double hydroxide nano-particles: kinetic, isothermal, and thermodynamic studies
  5. Behaviour of DGA and Ln resin with alpha radiation dose
  6. Sintering Bi2O3–B2O3–ZnO ternary low temperature glass by hydration device to solidify iodine containing silver-coated silica gel
  7. Enhancement of the thermal and physicochemical properties of styrene butadiene rubber composite foam using nanoparticle fillers and electron beam radiation
  8. Co-transport of bentonite colloid and U(VI) in particulate granite column: role of colloid concentration, ionic strength, pH and flow rate
https://doi.org/10.1515/ract-2021-1071
Keywords for this article
activated carbon; quinoline; sorption; uranium

Articles in the same Issue

  1. Frontmatter
  2. Original Papers
  3. Sorption behavior of natural uranium from aqueous solutions using modified activated carbon with quinoline
  4. Adsorption of UO2 2+ by AlBaNi-layered double hydroxide nano-particles: kinetic, isothermal, and thermodynamic studies
  5. Behaviour of DGA and Ln resin with alpha radiation dose
  6. Sintering Bi2O3–B2O3–ZnO ternary low temperature glass by hydration device to solidify iodine containing silver-coated silica gel
  7. Enhancement of the thermal and physicochemical properties of styrene butadiene rubber composite foam using nanoparticle fillers and electron beam radiation
  8. Co-transport of bentonite colloid and U(VI) in particulate granite column: role of colloid concentration, ionic strength, pH and flow rate
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