Chromatographic generator systems for the actinides and natural decay series elements
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Daniel R. McAlister
and E. Philip Horwitz
Abstract
This work describes chromatographic radionuclide generator systems for the production of actinides and natural decay series elements. The generator systems begin with alpha emitting parent radioisotopes with half-lives (T1/2) of greater than one year and produce alpha or beta emitting radioisotopes with half-lives of hours to days. Chromatographic systems were chosen to minimize radiolytic damage to chromatographic supports, preserve the parent activity for repeated use, provide high purity daughter radionuclide tracers, and to minimize or eliminate the need for evaporation of solutions of the parent or daughter nuclides. Useful secondary separations involving the daughters of the initial parent radionuclide are also described. Separation systems for 210Bi, 210Po, 211Pb, 212Pb, 223Ra, 224Ra, 225Ra, 225Ac, 227Th, 228Th, 231Th, 234Th, and 239Np are outlined in detail.
© by Oldenbourg Wissenschaftsverlag, Lisle, IL 60532, Germany
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Articles in the same Issue
- Small scale production of high purity 193mPt by the 192Os(α,ߙ3n)-process
- Plutonium sorption onto hematite colloids at femto- and nanomolar concentrations
- Determination of 235U/238U ratio by low energy gamma rays: an experimental evaluation
- Chromatographic generator systems for the actinides and natural decay series elements
- Metal ion selectivities of the highly preorganized tetradentate ligand 1,10-phenanthroline-2,9-dicarboxamide with lanthanide(III) ions and some actinide ions
- Humic substances extraction, characterization and interaction with U(VI) at Ruprechtov site (CZ)
- Studies on the third-phase formation in DHDECMP/dodecane/HNO3
- Comparative performance of semi-absolute k0-instrumental neutron activation analysis and Inductively Coupled Plasma Optical Emission Spectrometry (ICP-OES) for compositional decoding of aluminum base alloys
- The thermal release of scandium from titanium metal – a simple way to produce pure 44Sc for PET application