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Synthesis and investigation of Pu-doped single crystal zircon, (Zr, Pu)SiO4
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B. E. Burakov
Published/Copyright:
September 25, 2009
Summary
Single crystals of zircon doped with 239Pu, up to 2 mm in size, were grown for the first time ever, using a Li-Mo flux. The crystals were transparent and free of inclusions of separated Pu phases. The zircon crystals were studied using optical and scanning electron microscopy, the electron microprobe, and cathodoluminescence imaging and spectroscopy. The incorporation of 239Pu ranged from 0.1 to 1.4 wt.% el. The intensity of the CL emission in the Pu-doped crystals is correlated with the Pu content.
Received: 2001-3-21
Accepted: 2001-7-31
Published Online: 2009-9-25
Published in Print: 2002-2-1
© Oldenbourg Wissenschaftsverlag, München
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Articles in the same Issue
- Measurement of fission neutron spectrum averaged cross sections of some threshold reactions on europium: small scale production of no-carrier-added 153Sm in a nuclear reactor
- Production and separation of 24Na and 28Mg from 7Li-irradiated aluminium target
- Kinetics of the oxidation of Pu(IV) by manganese dioxide
- Dissolution of uranium dioxide in simulated Boom clay water
- Single-column extraction chromatographic separation of U, Pu, Np and Am
- TBP extraction of lanthanides from molten calcium nitrate hydrate
- Synthesis and investigation of Pu-doped single crystal zircon, (Zr, Pu)SiO4
- Diffusion of HTO and cement pore fluids through host rock
- Gamma radiolysis studies of uranyl fluoride