Polyacrylonitrile homogeneous blend hollow fiber membrane with stable structure as a substrate to support Fe/Mn oxide and its enhanced capability to purify dye wastewater
-
Zhifen Hao
,
Yan Feng
Abstract
Blending different molecular weight polyacrylonitrile (PAN) was adopted to solve the shrinkage problem of high molecular weight PAN hollow fiber membrane, to enhance the application performance of low molecular weight PAN membrane, and to adjust the porosity, pore size distribution, and hydrophilicity of the end product. The structurally-optimized membrane was chosen as a substrate to support Fe/Mn oxides and then used as a reactor to remove dyes from their solutions in the presence of H2O2. The results showed that the flux of methylene blue (MB) aqueous solution was 83.7 L/m2 h for the PAN homogeneous blend membrane, much higher than 29.1 L/m2 h of high molecular weight PAN membrane; MB removal efficiency was 97.3%, higher than 62.3% of low molecular weight PAN membrane, and it could be reused 25 times to remove dyes from their solutions without any loss in removal efficiency. The membrane was also found to have the application advantages of decreasing H2O2 dosage, reducing operation pressure, and raising MB removal efficiency compared with other membranes reported in the pieces of literature. Therefore, we were confident that the hollow fiber membrane fabricated by us would exhibit great application potential in the field of decontaminating dye wastewater.
Funding source: National Natural Science Foundation of China
Award Identifier / Grant number: 51103099
Funding source: Tianjin Municipal Natural Science Foundation
Award Identifier / Grant number: 12JCQNJC01600
Funding source: Research Fund for the Doctoral Program of Higher Education of China
Award Identifier / Grant number: 20111201120002
Funding source: China Postdoctoral Science Foundation
Award Identifier / Grant number: 2014M550143
Award Identifier / Grant number: 2015T80221
Funding source: Program of China Scholarship Council
Award Identifier / Grant number: 201809345019
Author contribution: All the authors have accepted responsibility for the entire content of this submitted manuscript and approved submission.
Research funding: The authors acknowledge the financial support provided by National Natural Science Foundation of China (project number: 51103099), Tianjin Municipal Natural Science Foundation (project number: 12JCQNJC01600), Research Fund for the Doctoral Program of Higher Education of China (project number: 20111201120002), China Postdoctoral Science Foundation (project numbers: 2014M550143; 2015T80221), and the Program of China Scholarship Council (project number: 201809345019).
Conflict of interest statement: The authors declare no conflicts of interest regarding this article.
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© 2020 Walter de Gruyter GmbH, Berlin/Boston
Articles in the same Issue
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- Editorial
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- Polymer genome–based prediction of gas permeabilities in polymers
- High gas permeability of nanoZIF-8/polymer-based mixed matrix membranes intended for biogas purification
- Polyacrylonitrile homogeneous blend hollow fiber membrane with stable structure as a substrate to support Fe/Mn oxide and its enhanced capability to purify dye wastewater
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Articles in the same Issue
- Frontmatter
- Editorial
- Special issue on industrial membranes
- Material properties
- Polymer genome–based prediction of gas permeabilities in polymers
- High gas permeability of nanoZIF-8/polymer-based mixed matrix membranes intended for biogas purification
- Polyacrylonitrile homogeneous blend hollow fiber membrane with stable structure as a substrate to support Fe/Mn oxide and its enhanced capability to purify dye wastewater
- Preparation and assembly
- Thiophene-based Schiff base ligand as ionophore for Ni(II)-selective polyvinyl chloride membrane electrode
- Electrospun polyacrylonitrile/polyvinyl pyrrolidone composite nanofibrous membranes with high-efficiency PM2.5 filter
- Composite proton exchange membranes produced using chitosan and kaolin solvent-free fluid
- Evaluation of the bioactive properties of Alternanthera sessilis extract and development of sodium alginate – Alternanthera sessilis membrane for wound management
- Blend polyethersulfone/zirconium oxychloride octahydrate membranes crosslinked by polyvinyl alcohol layer for high saline water desalination
- Engineering and processing
- Recent developments on polymeric membranes for CO2 capture from flue gas
