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Binary solvent systems for durable self-adhesive conductive hydrogels

  • Yunxuan Wu , Jie Li , Yangfu Jin and Mi Zhou EMAIL logo
Published/Copyright: January 24, 2020
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Abstract

Conductive hydrogels without adhesiveness and durability characteristics face great challenges in practical applications, such as inconvenient use, unstable contact voltage, and difficult to store. Herein, we present sodium polyacrylate (PAANa) hydrogels with binary solvent systems composed of water and an alcohol [ethylene glycol (EG), glycerol (GLY), or poly(ethylene glycol) (PEG)] as solvent instead of traditional water to research their self-adhesiveness, durability, conductivity, and mechanical properties. PAANa hydrogels exhibited higher self-adhesive properties and durability after alcohol content increased, and GLY/water hydrogels showed the best self-adhesive and stable properties. With more alcohols added, the weaker conductivity became, and EG/water hydrogels showed the highest conductivity. It was observed the long carbon chain length of alcohol could help improve the rheological properties of hydrogels. Thus, PEG/water hydrogels had the highest storage modulus, loss modulus, and consistency. The results demonstrated that the GLY/water binary solvent could provide good self-adhesiveness and durability, but EG/water and PEG/water showed better conductivity and mechanical properties, respectively. Therefore, our work may provide novel physical insights into the long-term usage of self-adhesive conductive hydrogels to practical requirements.

Acknowledgements

This work was financially supported by the Key Research and Development Program of Zhejiang Province (grant 2017C01068).

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Received: 2019-09-20
Accepted: 2019-12-12
Published Online: 2020-01-24
Published in Print: 2020-02-25

©2020 Walter de Gruyter GmbH, Berlin/Boston

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