First nuclear activation experiments using the new accelerator NUCLOTRON in Dubna
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J. Adam
, M. Yu. Barabanov , V. Bradnova , R. Brandt , P. Chaloun , Kh. M. Hella , S. R. Hashemi-Nezhad , V. G. Kalinnikov , V. A. Krasnov , M. I. Krivopustov , B. A. Kulakov , R. Odoj , V. S. Pronskikh , H. Robotham , A. A. Solnyshkin , A. N. Sosnin , V. I. Stegailov , V. M. Tsoupko-Sitnikov and W. Westmeier
Abstract
First nuclear activation experiments have been carried out using the new accelerator for relativistic particles NUCLOTRON in Dubna. The distribution of neutrons emitted during the irradiation with 0.65, 1.0 and 1.5 GeV protons from a lead target (∅ = 8 cm, l = 20 cm) and moderated by surrounding paraffin of 6 cm thickness was studied with radiochemical sensors along the beam axis on top of the moderator. Small 139Lasensors of approximately 1 g each were used to measure essentially the thermal neutron fluence at different depths near the surface: i. e. on top of the moderator, in 10 mm deep holes and in 20 mm deep holes, respectively. The reaction 139La (n, γ) 140La (τ1/2 = 40.27 h) was studied using standard procedures of gamma-ray spectrometry and data analysis. The induced activity of 140La increases strongly with the depth of the hole inside the moderator. Its activity distribution along the beam direction on top of the moderator has its maximum about 10 cm downstream the entrance of the protons into the lead and the activity increases about linearily with the proton energy. Some comparisons of the experimental results with model estimations based on the LAHET code are also presented. The experiments were carried out in the Veksler and Baldin Laboratory of High Energies of the Joint Institute for Nuclear Research in Dubna, Russian Federation.
Abstract
Erste Aktivierungsexperimente wurden durchgeführt mit Hilfe des neuen Beschleunigers NUCLOTRON in Dubna. Die Verteilung der Neutronen, die während der Bestrahlung mit 0,65, 1,0 und 1,5 GeV Protonen aus dem Bleitarget (∅ = 8 cm, l = 20 cm) emittiert und durch das umgebende 6 cm dicke Paraffin moderiert werden, wurde mit Hilfe radiochemischer Sensoren entlang der Strahlachse untersucht. Kleine 139La-Sensoren wurden verwendet um im Wesentlichen die thermische Neutronenfluenz in verschiedenen Tiefen nahe der Oberfläche zu messen. Die Reaktion 139La (n, γ) 140La (τ1/2 = 40.27 h) wurde untersucht mit Hilfe von Standardverfahren der Gammaspektrometrie und Datenanalyse. Die induzierte Aktivität von 140La erhöht sich stark mit der Tiefe des Loches innerhalb des Moderators. Das Maximum der Aktivitätsverteilung entlang der Strahlrichtung liegt bei etwa 10 cm unterhalb des Eintritts der Protonen in das Bleitarget und die Aktivität erhöht sich linear mit der Protonenenergie. Einige Vergleiche der experimentellen Ergebnisse mit Modellrechnungen des LAHET Computercodes werden vorgestellt. Die Experimente wurden durchgeführt im Veksler and Baldin Laboratory of High Energies des Joint Institute for Nuclear Research in Dubna, Russland.
Acknowledgements
All authors are very indebted to LHE Director, Prof. M. I. Malakhov and his colleagues, Prof. I.A. Shelaev and Prof. A. D. Kovalenko and the personnel of the LHE accelerator complex. One of us (Kh. M. Hella) acknowledges the kind hospitality of all colleagues at the LHE during his stay in Dubna working for his Ph.D.
References
1 Kovalenko, A. D.: Proc. EPAC-94, London, June 1994, V.1. (1995), 161–164, and Internet ± http://sunhe1.jinr.ru/page/nucl/nuclotron.htmlSearch in Google Scholar
2 Tolstov, K. D.: Some aspects of accelerator breeding. JINR-preprint, 18-89-778, Dubna, (1989)Search in Google Scholar
3a Bowman, C. D. et al.: Nuclear energy generation and waste transmutation using an accelerator-driven intense thermal neutron source. Nucl. Instr. and Methods A 320 (1992) 33610.1016/0168-9002(92)90795-6Search in Google Scholar
3b Carminata, F.; Klapisch, R.; Revol, J. P.; Roche, Ch.; Rubio, J. A.; Rubbia, C.: An energy amplifier for cleaner and inexhaustible nuclear energy production driven by a particle beam accelerator. CERN, Geneva, print CERN/AT/93–47 (ET), November 1 (1993)Search in Google Scholar
4 Wan,. J.-S.; Ochs, M.; Abdullaev, I. G.; Adam, J.; Adloff, J. C.; Bamblevskij, V. P.; Bradnova, V.; Brandt, R.; Butsev, V. S.; Debeauvais, M.; Dwivedi, K. K.; Gelovani, L.; Golubev, P. I.; Kalinnikov, V. K.; Karachuk, J.; Krivopustov, M. I.; Kulakov, B. A.; Langrock, E.-J.; Modolo, G.; Odoj, R.; Perelygin, V. P.; Phlippen, P.-W.; Premyshev, A. N.; Pronskich, V. S.; Sosnin, A. N.; Stegailov, V. I.; Wilson, B.; Zamani-Valasiadou, M.; Zupko-Sitnikov, V. M.: Transmutation of radioactive waste with the help of relativistic heavy ions. Kerntechnik 63 (1998) 16710.1515/kern-1998-630404Search in Google Scholar
5 Ochs, M.: Experimente zur Neutronenfreisetzung durch Spallationsreaktionen in massiven Kupfer- und Bleitargets. Ph.D. Thesis, Department of Chemistry, Philipps-University, Marburg, Germany, ISBN 3-89703-050-0 (1997)Search in Google Scholar
6 J. Adam, J. C. Adloff, A. Balabekyan, V. P. Bamblevski, M. Yu. Barabanov, R. Brandt, V. Bradnova, P. Chaloun, M. Debeauvais, K. K. Dwivedi, S.-L. Guo, S. R. Hashemi-Nezhad, Kalinnikov, V. G.; Hella, Kh. M.; Kievits, M. K.; Krivopustov, M. I.; Kulakov, B. A.; Langrock, E.-J.; Li Li; Lomonossova, E. M.; Modolo, G.; Odoj, R.; Perelygin, V. P.; Pronskikh, V. S.; Solnyshkin, A. A.; Stegialov, V. I.; Tsoupko-Sitnikov, V. M.; Vater, P.; Wan, J.-S.; Westmeier, W.; Zamani-Valasiadou, M.; Zhuk, I. V.: Transmutation of 239Pu and other nuclides using spallation neutrons produced by relativistic protons reacting with massive U- and Pb-targets. Radiochimica Acta 90 (2002) 43110.1524/ract.2002.90.8_2002.431Search in Google Scholar
7 Wan, J.-S.; Langrock, E.-J.; Westmeier, W.; Vater, P.; Brandt, R.; Adam, J.; Bradnova, V.; Balabekian, A.; Kalinnikov, V G.; Pronskikh, V. S.; Solnyshkin, A. A.; Stegailov, V. I.; Tsoupko-Sitnikov, B. A. Kulakov,M. I. Krivopustov, A. N. Sosnin,G. Modolo, R. Odoj, S. R. Hashemi-Nezhad, V. M.; Zamani-Valasiadou, M.: First radiochemical studies on the transmutation of 239Pu with spallation neutrons. Journal of Radioanalytical and Nuclear Chemistry 247 (2001) 15110.1023/A:1006787703538Search in Google Scholar
8 Slowinski, B.; Hella, Kh. M.; Malkhov, A. I.; Comsan, M. N.: Transmutation of radioactive nuclides, basic concepts and results. Proc. of 3 rd Conference on Nuclear and Particle Physics 20–24 October 2001 ± Cairo, Egypt, and Annual Report for Institute of Atomic Energy, Otwock-Swierk-Poland (2001) 117–120Search in Google Scholar
9 Wan, J.-S.; Schmidt, Th.; Langrock, E.-J.; Vater, P.; Brandt, R.; Adam, J.; Bradnova, V.; Bamblevski, V. P.; Geloviani, l.; Gridnev, T. D.; Kalinnnikov, V. G.; Krivopustov,M. I.; Kulakov, B. A.; Sosnin, A. N.; Perelygin, V. P.; Pronskikh, V. S.; Stegailov, V. I.; Tsoupko-Sitnikov, V. M.; Modolo, G.; Odoj, R.; Phlippen, P.-W.; Zamani-Valasiadou, M.; Adloff, J. S.; Debeauvais, M.; Hashemi-Nezhad, S. R.; Guo, S.-L.; Li Li; Wang, Y.-L.; Dwivedi, K. K.; Zhuk, I. V.; Boulyga, S. F.; Lomonosova, E. M.; Kievitskaja, A. F.; Rakhnov, I. L.; Chigrinov, S. E.; Wilson, B.: Transmutation of 129I and 237Np using spallation neutrons produced by 1.5, 3.7 and 7.4 GeV protons. Special Issue on Accelerator Driven Systems, H.S. Plendl (Ed.), Nuclear Instruments and Methods in Physics Research A 463 (2001) 634–65210.1016/S0168-9002(01)00175-9Search in Google Scholar
10 Wan, J.-S.: Studies on spallation in massive targets and the transmutation of 129I and 237Np in subcritical systems. Ph.D. Thesis, Department of Chemistry, Philipps University Marburg, Germany, ISBN 3-89703-310 (1999)Search in Google Scholar
11 Kulakov, B. A.; Hella, Kh. M.; Barabanov, M. Yu.: Analysis of neutron yield in ransmutation experiments with different proton energies and targets using natural uranium and 139La Sensors. Proc. of 5th Conf. of Young Scientists, Dubna, JINR, Feb. 5–10, (2001) 170± 172Search in Google Scholar
12 Peker, I. R.: in: “Nuclear Data Shetts for A = 140”, Vol. 73 (1994) 261 and U. Reus and W. Westmeier, personal communication (2000), to be published in Landolt-Börnstein10.1006/ndsh.1994.1044Search in Google Scholar
13 Cumming, J. B.: Annual Review of Nuclear Science 13 (1963) 26110.1146/annurev.ns.13.120163.001401Search in Google Scholar
14 Wan, J.-S.; Ochs, M.; Vater, P.; Song, X. P.; Langrock, E.-J.; Brandt, R.; Adam, J.; Bamblevski, V. P.; Kulakov, B. A.; Krivopustov, M. I.; Sosnin, A. N.; Modolo, G.; Odoj, R.: Monitor reactions in Alfoils for high energy proton beams bombarding a thick target. Nuclear Instruments and Methods B (Beam Interactions with Materials & Atoms) 155 (1999) 11010.1016/S0168-583X(99)00293-1Search in Google Scholar
15 Hella, Kh. M.: Experimental study of transmutation of selected radioactive waste using the beams of relativistic protons. Ph.D. Thesis, Joint Institute for Nuclear Research, Dubna, Russian Federation (2003)Search in Google Scholar
16 Westmeier, W.: Benutzerhandbuch des Gamma-Spektrenanalyse ProgrammesGAMMAW. Version 10.32. Gesellschaft für Kernspektrometrie mbH, 35085-Ebsdorfergrund-Mölln, GermanySearch in Google Scholar
17 Prael, R. E.; Lichtenstein, H.: User Guide to LCS: The LAHET Code System. Los Alamos National Laboratory, Report LA-UR89–3014, (Sept. 1989)Search in Google Scholar
18 Hashemi-Nezhad, S. R.; Brandt, R.;Westmeier,W.; Bamblevski, V. P.; Krivopustov, M. I.;Kulakov, B. A.; Sosnin, A.N.;Wan, J.-S.; Odoj, R.: Monte Carlo calculations on transmutation of transuranic nuclear waste isotopes using spallation neutrons: Difference of lead and graphite moderators. Nuclear Instruments and Methods in Physics Research A 482 (2002) 54710.1016/S0168-9002(01)01508-XSearch in Google Scholar
19 Hashemi-Nezhad, S. R.; Brandt, R.;Westmeier,W.; Bamblevski, V. P.; Krivopustov, M. I.;Kulakov, B. A.; Sosnin, A.N.;Wan, J.-S.; Odoj, R.: Monte Carlo analysis of accelerator driven systems: Studies on spallation neutron yield and energy gain. Kerntechnik 66 (2001) 4710.1515/kern-2001-0013Search in Google Scholar
© 2003 Carl Hanser Verlag, München
Articles in the same Issue
- Frontmatter
- Summaries
- Summaries/Kurzfassungen
- Biokinetic model for the calculation of dose coefficients for oral and intravenous administration of 14C labeled drugs
- First nuclear activation experiments using the new accelerator NUCLOTRON in Dubna
- Charge fragmentation in cosmic radiation – and the question of physical anomalons
- Measurements of gamma and neutron flux spectra in iron-water configurations
- Experimental and analytical investigation of the ITU TRIGA Mark-II reactor core
- Books. Bücher
- Books. Bücher
- Experimental studies on condensation of steam mixed with noncondensable gas inside the vertical tube in a pool filled with subcooled water
- Books. Bücher
- Books. Bücher
- A mathematic model of two-phase flow taking account of sub-cooled boiling, condensation, and void flashing
- Books. Bücher
- A new approach to authorisation in the field of radiological protection
- Experimental study on natural convection in the vertical enclosure of a double coaxial cylinder
- Technical Note
- Integral nucleus-nucleus cross-sections
- Books. Bücher
- Books. Bücher
- Technical Note
- Fermat’s optics in nuclear materials
- Advances
- Patent
- Patent
- Note. Mitteilung
Articles in the same Issue
- Frontmatter
- Summaries
- Summaries/Kurzfassungen
- Biokinetic model for the calculation of dose coefficients for oral and intravenous administration of 14C labeled drugs
- First nuclear activation experiments using the new accelerator NUCLOTRON in Dubna
- Charge fragmentation in cosmic radiation – and the question of physical anomalons
- Measurements of gamma and neutron flux spectra in iron-water configurations
- Experimental and analytical investigation of the ITU TRIGA Mark-II reactor core
- Books. Bücher
- Books. Bücher
- Experimental studies on condensation of steam mixed with noncondensable gas inside the vertical tube in a pool filled with subcooled water
- Books. Bücher
- Books. Bücher
- A mathematic model of two-phase flow taking account of sub-cooled boiling, condensation, and void flashing
- Books. Bücher
- A new approach to authorisation in the field of radiological protection
- Experimental study on natural convection in the vertical enclosure of a double coaxial cylinder
- Technical Note
- Integral nucleus-nucleus cross-sections
- Books. Bücher
- Books. Bücher
- Technical Note
- Fermat’s optics in nuclear materials
- Advances
- Patent
- Patent
- Note. Mitteilung