Startseite Influence of organic matter on smectite illitization: A comparison between red and dark mudstones from the Dongying Depression, China
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Influence of organic matter on smectite illitization: A comparison between red and dark mudstones from the Dongying Depression, China

  • Yingli Li , Jingong Cai EMAIL logo , Mingshui Song , Junfeng Ji und Yujin Bao
Veröffentlicht/Copyright: 9. Januar 2016
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American Mineralogist
Aus der Zeitschrift American Mineralogist Band 101 Heft 1

Abstract

Interactions between organic matter (OM) and clay minerals have received considerable attention in previous studies. The inflence of OM on smectite illitization has been analyzed primarily in simulation experiments rather than in diagenetic studies. The present study explores the influence of OM on smectite illitization during diagenesis. Thirty red and dark mudstone samples from the Dongying Depression were analyzed. X-ray diffraction (XRD) analyses revealed that the illite percentages in mixed-layer illite-smectite (I-S) of both types of samples were dispersive above 3100 m and more convergent below this depth. The stacking mode of I-S in dark mudstones above 3100 m remained primarily at R0–R0.5 ordering with the average number of layers (Nave) dispersively distributed between 2 and 4.5. In red mudstones, the I-S changed from the R0 to R0.5 mode with the Nave increasing from 2 to 5. Over this range, the smectite illitization in dark mudstones was slower than that in red mudstones. Below 3100 m, the I-S stacking mode of dark mudstones changed from R0.5 to R3 ordering with the Nave increasing sharply from 4 to 8. In red mudstones, the I-S displayed R1.5 and R3 ordering with the Nave varying between 4.5 and 6.5. Over this range, the smectite illitization in dark mudstones accelerated rapidly, whereas the process in red mudstones was retarded. Additionally, the red mudstone samples contained little OM, whereas the dark mudstone samples contained abundant total organic carbon (0.17–4.43%). Thermo-XRD, near-infrared (NIR) as well as mid-infrared (MIR) spectroscopy analyses suggested that the OM in dark mudstones exhibited a significant transition at 3100 m, coincident with the illitization change. Above 3100 m, the smectite illitization in dark mudstones was delayed due to the OM pillar effect in the interlayer spaces of smectite. Below 3100 m, the interlayer OM became varied and desorbed, discharging organic acid. This led to the dissolution of smectite structural layers. Consequently, illitization in the dark mudstone was accelerated. This study revealed that the existence and occurrence of OM could influence the smectite illitization in diagenesis. Further study on the interactions between OM and clay minerals is needed to facilitate our understanding on the mechanism of smectite illitization as well as its geological applications.

Keywords: Smectite illitization; dark mudstone; red mudstone; organic matter; Dongying Depression; reaction mechanisms

Acknowledgments

This work was financed by the National Natural Science Foundation of China (Grant No. 41072089; 41372130) and the National Oil and Gas Special Fund (Grant No. 2011ZX05006-001; 2016ZX05006-001). We acknowledge Yuanfeng Cai, Tong He, and Yuguan Pan (all in Nanjing) for their assistance with the X-ray diffraction and infrared spectroscopy. We are thankful to Hejing Wang (Beijing) for his help with the crystallinity analyses. Meng Xu (Shanghai) is thanked for providing assistance with the laboratory work.

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  1. Manuscript handled by Warren Huff.

Received: 2014-11-7
Accepted: 2015-7-14
Published Online: 2016-1-9
Published in Print: 2016-1-1

© 2016 by Walter de Gruyter Berlin/Boston

Artikel in diesem Heft

  1. Highlights and Breakthroughs
  2. A spin on lower mantle mineralogy
  3. Highlights and Breakthroughs
  4. Safe long-term immobilization of heavy metals: Looking at natural rocks
  5. Highlights and Breakthroughs
  6. Spinel in planetary systems
  7. Review
  8. Pathways for nitrogen cycling in Earth's crust and upper mantle: A review and new results for microporous beryl and cordierite
  9. Invited Centennial Article
  10. Metamorphic chronology—a tool for all ages: Past achievements and future prospects
  11. Review
  12. K-bentonites: A review
  13. Chemistry and Mineralogy of Earth's Mantle
  14. Ca-Al-silicate inclusions in natural moissanite (SiC)
  15. Special Collection: Advances in Ultrahigh-Pressure Metamorphism
  16. Immiscible melt droplets in garnet, as represented by ilmenite–magnetite–spinel spheroids in an eclogite-garnet peridotite association, Blanský les Granulite Massif, Czech Republic
  17. Special Collection: Advances in Ultrahigh-Pressure Metamorphism
  18. Tetrahedral boron in natural and synthetic HP/UHP tourmaline: Evidence from Raman spectroscopy, EMPA, and single-crystal XRD
  19. Article
  20. Radiation damage haloes in biotite investigated using high-resolution transmission electron microscopy
  21. Article
  22. A spreadsheet for calculating normative mole fractions of end-member species for Na-Ca-Li-Fe2+-Mg-Al tourmalines from electron microprobe data
  23. Article
  24. Preservation of organic matter in nontronite against iron redox cycling
  25. Article
  26. Influence of organic matter on smectite illitization: A comparison between red and dark mudstones from the Dongying Depression, China
  27. Article
  28. Intermediate members of the lime-monteponite solid solutions (Ca1–xCdxO, x = 0.36–0.55): Discovery in natural occurrence
  29. Article
  30. Ab initio investigation of majorite and pyrope garnets: Lattice dynamics and vibrational spectra
  31. Article
  32. FTIR spectroscopy of D2O and HDO molecules in the c-axis channels of synthetic beryl
  33. Article
  34. Experimental constraints on mantle sulfide melting up to 8 GPa
  35. Article
  36. Excess mixing volume, microstrain, and stability of pyrope-grossular garnets
  37. Article
  38. Phase stabilities and spin transitions of Fe3(S1−xPx) at high pressure and its implications in meteorites
  39. Special Collection: Building Planets: The Dynamics and Geochemistry of Core Formation
  40. The W-WO2 oxygen fugacity buffer (WWO) at high pressure and temperature: Implications for fO2 buffering and metal-silicate partitioning
  41. Special Collection: Rates and Depths of Magma Ascent on Earth
  42. Timescales of magma storage and migration recorded by olivine crystals in basalts of the March-April 2010 eruption at Eyjafjallajökull volcano, Iceland
  43. Letter
  44. In-situ crystal structure determination of seifertite SiO2 at 129 GPa: Studying a minor phase near Earth's core–mantle boundary
  45. New Mineral Names
  46. New Mineral Names*,†
  47. Book Review
  48. A Pictorial Guide to Metamorphic Rocks in the Field
https://doi.org/10.2138/am-2016-5263
Schlagwörter für diesen Artikel
Smectite illitization; dark mudstone; red mudstone; organic matter; Dongying Depression; reaction mechanisms

Artikel in diesem Heft

  1. Highlights and Breakthroughs
  2. A spin on lower mantle mineralogy
  3. Highlights and Breakthroughs
  4. Safe long-term immobilization of heavy metals: Looking at natural rocks
  5. Highlights and Breakthroughs
  6. Spinel in planetary systems
  7. Review
  8. Pathways for nitrogen cycling in Earth's crust and upper mantle: A review and new results for microporous beryl and cordierite
  9. Invited Centennial Article
  10. Metamorphic chronology—a tool for all ages: Past achievements and future prospects
  11. Review
  12. K-bentonites: A review
  13. Chemistry and Mineralogy of Earth's Mantle
  14. Ca-Al-silicate inclusions in natural moissanite (SiC)
  15. Special Collection: Advances in Ultrahigh-Pressure Metamorphism
  16. Immiscible melt droplets in garnet, as represented by ilmenite–magnetite–spinel spheroids in an eclogite-garnet peridotite association, Blanský les Granulite Massif, Czech Republic
  17. Special Collection: Advances in Ultrahigh-Pressure Metamorphism
  18. Tetrahedral boron in natural and synthetic HP/UHP tourmaline: Evidence from Raman spectroscopy, EMPA, and single-crystal XRD
  19. Article
  20. Radiation damage haloes in biotite investigated using high-resolution transmission electron microscopy
  21. Article
  22. A spreadsheet for calculating normative mole fractions of end-member species for Na-Ca-Li-Fe2+-Mg-Al tourmalines from electron microprobe data
  23. Article
  24. Preservation of organic matter in nontronite against iron redox cycling
  25. Article
  26. Influence of organic matter on smectite illitization: A comparison between red and dark mudstones from the Dongying Depression, China
  27. Article
  28. Intermediate members of the lime-monteponite solid solutions (Ca1–xCdxO, x = 0.36–0.55): Discovery in natural occurrence
  29. Article
  30. Ab initio investigation of majorite and pyrope garnets: Lattice dynamics and vibrational spectra
  31. Article
  32. FTIR spectroscopy of D2O and HDO molecules in the c-axis channels of synthetic beryl
  33. Article
  34. Experimental constraints on mantle sulfide melting up to 8 GPa
  35. Article
  36. Excess mixing volume, microstrain, and stability of pyrope-grossular garnets
  37. Article
  38. Phase stabilities and spin transitions of Fe3(S1−xPx) at high pressure and its implications in meteorites
  39. Special Collection: Building Planets: The Dynamics and Geochemistry of Core Formation
  40. The W-WO2 oxygen fugacity buffer (WWO) at high pressure and temperature: Implications for fO2 buffering and metal-silicate partitioning
  41. Special Collection: Rates and Depths of Magma Ascent on Earth
  42. Timescales of magma storage and migration recorded by olivine crystals in basalts of the March-April 2010 eruption at Eyjafjallajökull volcano, Iceland
  43. Letter
  44. In-situ crystal structure determination of seifertite SiO2 at 129 GPa: Studying a minor phase near Earth's core–mantle boundary
  45. New Mineral Names
  46. New Mineral Names*,†
  47. Book Review
  48. A Pictorial Guide to Metamorphic Rocks in the Field
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