Abstract
High-precision detection of electric charge is critical for physical, chemical, and biological measurements. Nanophotonic optomechanical system confines the optical field at the nanoscale and enables a strong interaction between optical cavity and mechanical resonator. Its high optical quality factor cavity and strong optomechanical coupling are promising for precision sensing applications. Here an integrated optomechanical electrometer is proposed for the electric charge sensing using a zipper cavity with a suspended photonic crystal nanobeam (PCN) acting as a movable mechanical resonator. As the electrostatic force arising from the electric voltage to be measured interacts with the mechanical motion of the movable PCN and modulates its resonance through electrostatic stiffening effect, optomechanical coupling transduces the mechanical motion to the optical field with enhanced sensitivity. The resonance shift of the mechanical resonator can be monitored to detect the electric voltage with a sensitivity of 0.007
1 Introduction
Electron is well known as one of the natural elementary particles. Moving of electron flow defines the value of electric voltage and current. For many years, electrometers have been considered as one of the most fundamental instruments for the characterization of electric charge or voltage [1, 2]. Electrometers have found wide applications in the research fields of biological and chemical charge detection [3, 4], environment monitoring [5], mass spectrometry [6, 7], and space exploration [8]. The miniaturized electrometer with high sensitivity is desired for the precise measurement of weak electric voltages, and currents or quantities of electric charges in the research and industry fields. One of the cutting-edge nano-electronic electrometers is conducted using the cryogenically cooled single electron transistor (SET) to achieve a supreme detection resolution, but the SET-based electrometers suffer from limited bandwidth and cannot be operated at room temperature [9, 10]. To overcome these problems, micro- and nano-electromechanical system (M/NEMS) is another great technology to realize the chip-level electrometer with high performance and low energy consumption [1]. Currently, the M/NEMS-based electrometers have been developed for precision sensing based on three approaches, including modulated stiffness [11, 12], vibrating reed [5, 13] and coupled resonators [14]. Basically, the concept of M/NEMS-based electrometry refers to metrology that measures charge by monitoring the frequency variation of mechanical resonators. M/NEMS resonant sensing scheme has advantages of simple structures, reduced sizes and low power consumptions as well as simple postprocessing circuits. The working mechanisms for these sensitive M/NEMS-based electrometers rely on the electrostatic spring softening (ESS) effect. The voltage (V) or charged particle (Q) on the micro- or nano-scale capacitor results in an electrostatic force or stain on the movable structures, which could modify the effective stiffness of the mechanical resonator. Subsequently, an electrical circuit is developed to read the frequency shift of the vibration mode
Silicon photonics has attracted much attention over the past two decades [16]. Its CMOS compatibility with the semiconductor industry makes it a cost-effective approach to realize the optical routing at a chip level. Using moveable on-chip optical components by electrostatic force, the M/NEMS-enabled photonic integrated circuits can also serve as a superior approach for electrical detection [17]. In contrast to traditional M/NEMS-based sensing systems using the electric circuits to read out the signal, the optical readout mechanism has less detrimental noise reaching quantum-limited level and immunity to external electromagnetic interference [18]. Optical measurement and control of mechanical motion attract great attention from fundamental researches and industrial applications [19], [20], [21]. In particular, the nanophotonic optomechanical system localizes light to subwavelength volume, simultaneously enhancing optomechanical interaction between the localized optical radiation field and mechanical vibration mode at a nanoscale [20, 22]. In the cavity optomechanical system, the mechanical oscillation with a displacement amplitude (x) translates into perturbation of cavity mode and hence shifts the optical cavity resonance (ωc). At the same time, the mechanical motion modulates the intracavity field with a mechanical frequency
Currently, research efforts on using electrostatic force in optomechanical systems mainly focus on electrostatic actuation to control the interaction of the micro-opto-electro-mechanical-systems (MOEMS) [42]. In most of MOEMS devices, the electrostatic force acts as an actuation for optical re-configuration or mechanical switching which could be promising for a range of photonic applications including frequency conversion between electrical and optical domains [43]. On the other hand, several theoretical optomechanical schemes were analytically proposed for electrical charge measurements, including the sensing schemes utilizing optomechanically induced transparency [44, 45], and the nonlinear optomechanical interaction [46]. However, the related experimental work has rarely been demonstrated for electrical voltage or charge detection so far. In this paper, a nanoscale optomechanical electrometer is proposed and experimentally demonstrated for electric voltage detection. The key component of optomechanical electrometer is a zipper cavity that consists of two coupled one-dimensional photonic crystal nanobeam (PCN) cavities where one of the suspended PCN cavities works as a movable mechanical resonator. Perturbed by an electrostatic field on the motion of the movable mechanical resonator, the optomechanical cavity provides a sensitive approach for the precision probing of the weak electric voltage by tracking the RF signal from the cavity readout. Especially, when the pump optical power exceeds the intrinsic mechanical damping loss (above threshold power), the mechanical motion turns into a self-sustained optomechanical oscillation, yielding an optomechanical backaction limited RF linewidth with an amplified oscillation amplitude. Compared to the electric measurement operating below the threshold, the self-sustained optomechanical system is distinguished with a larger sensitivity of 0.014
2 Optomechanical electrometer design and fabrication
As shown in Figure 1, the proposed chip-scale optomechanical electrometer is operated to measure the bias voltage (Vbias) by an electro-opto-mechanical interaction from a zipper cavity. As seen from Figure 1(a), the nanophotonic zipper cavity consists of two PCN cavities. One of the PCN cavities is suspended with four flexural beams acting as a mechanical resonator (namely movable PCN). The optomechanical coupling occurs when the other fixed PCN cavity is radiation-driven by the pump light. This zipper cavity and driving bias electrode are electrically isolated by an air slot with an initial separation gap d = 150 nm. Besides, the silicon device layer patterned with the zipper cavity together with the silicon substrate layer is electrically grounded to avoid the floating voltages and the undesirable vertical electrostatic force on the zipper cavity. The sidewalls of the movable PCN and the stationary bias electrode form a nanoscale parallel-plate capacitor, which gives rise to an electrostatic force as presented in the inset of Figure 1(a). As shown in Figure 1(b), with an electric potential applied to this capacitor, the isolation slot gap is decreased due to the deflection of movable PCN driven by the electrostatic force. It can also be seen from FEM analysis in Figure 1(b) and(c) that the air isolation slot reduces while the electrostatic force quadratically increases as a function of the bias voltage. The electrostatically driven motion of the movable PCN can shift the optical resonance of the zipper cavity and modulate the natural frequency of movable mechanics. Subsequently, the optomechanical dynamical-backaction behaviours of the zipper cavity are determined under the combined actions of optical force and electrostatic force. Therefore, the precise measurement of the electrical voltage can be realized by observing the RF readout of the movable PCN.

Overview of the nanoscale optomechanical electrometer.
(a) Schematic diagram of the electrometry integrated with an optomechanical zipper cavity. Inset: Schematic of the optomechanical electrometry based on a parallel-plate capacitor. (b) The normalized FEM deflection of movable PCN forced by an electric potential. (c) Simulation results of the nanoscale capacitor under the applied bias voltage, the blue data point is the lateral separation of the isolation gap while the red data point shows the electrostatic force induced by the applied voltage.
As illustrated in Figure 2(a), the zipper cavity is formed with a pair of coupled PCN resonators with a slot gap. The fixed PCN cavity is used for light pumping by a dimpled fiber taper due to its larger rigidity. The other PCN cavity is suspended by four 120 nm-wide and 5 μm-long silicon beams. As a result, the entire suspended structure enables a feasible in-plane mechanical movement under the combined actuation of optical gradient force and electrostatic force. The nanoscale PCN cavity is fabricated from the 220 nm thick silicon device layer that is patterned with (i) a parameterized transition of air hole and unit cell in the defect region (ii) and two symmetric mirror regions. To achieve high optical quality resonant modes, the physical dimensions of PCN cavity (Figure 2(b)) are designed with reference to the developed optimization methods [41, 47] by Lumerical FDTD simulations. In this work, the PCN cavity is featured with 15 holes in the central defect region and 11 mirror holes at two sides of the nanobeam to achieve desirable cavity mode frequencies and high optical Q-factors. The PCN cavity is specified by the unit cell geometric sizes of the defect region varying gradually from the defect unit values (a0, w,

Optomechanical zipper cavity.
(a) SEM images of the nanoscale optomechanical electrometer on an SOI chip. Inset: Zoom-in view of the zipper cavity electrically isolated with a bias electrode with a gap width d. The PCN cavity is formed with defect region (i) and mirror region (ii). (b) SEM image of the zipper PCN cavities that are parameterized with beam width w and beam slot s.
3 Measurements and analysis
3.1 Experimental setup and optical characterization of optomechanical electrometer
Characterization of the optomechanical electrometer is performed under a low-pressure environment (1×10−3 mbar) and at room temperature. As shown in Figure 3, light launching from a tunable laser (TSL, Santec TSL710, Japan) is split into two parts: 90% optical intensity into subsequent optical fiber circuits and 10% intensity to a power meter to monitor the light stability. The 90% pump light is sent to an optical attenuator to reduce the pump light intensity when necessary to avoid optical nonlinear effects. Then its polarization is adjusted to excite transverse electric (TE) mode through a fiber polarized controller to ensure an efficient optical coupling between the dimpled fiber taper and the zipper cavity. Next, this TE-polarized light is launched into the on-chip device. Light escaping from the zipper cavity is coupled back into the fiber via the same fiber taper and is directly received by two photodetectors (PDs). Subsequently, signal from PD1 (10 MHz bandwidth, Femto FMG-OE-300-IN-01-FC, Germany) is sent to the data acquisition device (DAQ) and signal from PD2 (125 MHz bandwidth, Newport 1811, USA) is sent to the electrical signal analyzer (ESA, Agilent N9020A, USA). To characterize the optical properties of the optomechanical electrometer, synchronization is established between DAQ and TSL to obtain the swept optical spectrum from PD1. Meanwhile, the PD2 signal sent to ESA is monitored to obtain the mechanical properties of the optomechanical electrometer. In the detection of mechanical spectra, the laser wavelength should be set and swept across the optical resonance by simultaneously controlling ESA and TSL to obtain the RF spectra as a function of laser-cavity detuning. Both optical and mechanical spectra data are finally processed in the computer. For purpose of detection of electric voltage, a DC power supply (Agilent E3631A, USA) is used to generate and calibrate the electric potential between the zipper cavity and bias electrode. In this work, a dimpled fiber taper is evanescently coupled with the zipper cavity, as illustrated in the inset of Figure 3. The fiber taper is precisely positioned with a triaxial nanopositioner, and with the help of an optical microscope, the dimple of fiber taper is accurately aligned and mechanically attached with the rigid side of the zipper cavity (i.e. fixed PCN).

Experimental setup for the optomechanical electrometer. Inset indicates the precise alignment of fiber taper and on-chip zipper cavity. A microscopic image shows the observation of fiber taper attached to the fixed PCN cavity.
First, we investigate the optical properties of the optomechanical electrometer. The optical transmission spectrum through the fiber taper is used to observe the optical resonance of zipper cavity. When the cavity is driven by a pump laser intensity of 30 μW in the telecom band (1480–1630 nm), the fundamental and the second-order modes of cavity can be observed in the transmission spectrum. As shown in Figure 4(a), the fundamental modes TE1,o and TE1,e of the zipper cavity are measured at λ1,o = 1532.469 nm and λ1,e = 1538.892 nm, respectively. With a Lorentzian fitting of the TE1,e resonance, full width at half maximum of 10 pm (Qo ≈1.5×105) can be found. These measured results are in good agreement with the FEM results which indicates a high-quality fabrication of device. With the increase of pump laser power, as presented in Figure 4(b), the line shape of the optical resonance becomes increasingly asymmetrical and broadened due to the thermal and optomechanical nonlinearities inside the zipper cavity.

Optical transmission spectrum of the optomechanical zipper cavity.
(a) The fundamental TE1,o and TE1,e modes of the zipper cavity. Inset shows the resonance of TE1,e mode with Lorentzian fitting to obtain an optical Q-factor up to
To verify the electrostatic force-induced resonance shift of the zipper cavity, the optomechanical electrometer is driven by an increasing bias voltage from 0 V to 5 V. Figure 5(a) and (b) indicate the resonant wavelength shifts of the detected modes of the zipper cavity. With an applied bias voltage on the optomechanical electrometer, an electrostatic force

Electrostatic force-induced optical resonance shift of the zipper cavity.
(a) and (b) optical resonant wavelength shift of TE1,o and TE1,e under the increasing applied bias voltages. (c) Resonance shift of the fundamental and second-order optical modes under the increasing bias voltages (from 0 V to 5 V, step 0.5 V) with a linear fitting to identify the dispersion sensitivity.
3.2 Characterization of optomechanical electrometer below threshold power
The in-plane mechanical displacement of movable PCN in the optomechanical electrometer is sensitively coupled to the optical resonance of the zipper cavity due to a strong optomechanical interaction. With the laser wavelength detuned at the shoulder of the optical resonance, this in-plane motion is optically read out by ESA. When the optomechanical cavity is pumped with an incident power of Pin = 30 μW, the in-plane fundamental mechanical mode and other two harmonic peaks of the movable PCN arise from its thermal Brownian motion, as shown in the power spectral density (PSD) spectrum in Figure 6(a). The FEM simulated in-plane eigenmode profile of movable PCN in the inset agrees well with the measured frequency
where,

RF spectra of the optomechanical electrometer below the threshold power.
(a) Measured RF spectrum of the fundamental in-plane mechanical mode of the moveable PCN (resolution bandwidth (RBW) of ESA is set at 100 Hz). Insets are FEM-calculated in-plane mechanical mode of the movable PCN and zoom-in view of the RF spectrum of the fundamental vibrating mode at
With the laser wavelength and power fixed (pump laser wavelength at 1538.345 nm and pump power 30 μW), the optomechanical electrometer can measure the applied bias voltages by monitoring the cavity readout and detecting the mechanical resonance shift. It should be noted that the energy stored in the parallel-plate capacitor charged with VBias = 120 mV is calculated as about
where
3.3 Measurement of optomechanical electrometer above threshold power
When the optomechanical electrometer works above the threshold power, a self-sustained optomechanical oscillation is realized with a narrow mechanical linewidth and a high oscillation amplitude (see Supplementary V). As shown in Figure 7(a), tuning the optomechanical cavity through the optical TE1,e resonance (white-colored curve) with a detuning range of 50 pm with a pump power Pin = 180 μW (above threshold), the RF-spectra indicates a significant parametric oscillation effect in the blue-detuned regime. Due to the nonlinear optical resonance resulting from the high pump power, as presented in Figure 7(b), both the optical spring and damping effects have only emerged in the blue-detuned regime. At the laser-cavity detuned wavelength of 8 pm (equals to the blue-detuned frequency of about 1 GHz), a self-induced optomechanical oscillation reaches a minimal linewidth of Γm/2π≈ 12 Hz (corresponding to an effective mechanical Qm ≈ 1×105). Here, the mechanical resonance linewidth is greatly reduced compared with that of the optomechanical cavity driven below threshold power. It is noted that this optomechanical electrometer operating in the self-sustained oscillation mode can greatly reduce the mechanical damping rate, thus overcoming the extensive damping rates existed in the traditional M/NEMS resonant electrometers. It is also interesting to note that, due to the increased nonlinearity in the optomechanical nanocavity, high-order harmonics (up to 13th harmonic) of the in-plane fundamental oscillation mode are excited as presented in Figure 7(c). Furthermore, for the fundamental in-plane oscillation mode at

Optomechanical backaction RF spectra above threshold power.
(a) PSD map of the measured RF spectrum as functions of laser-cavity detuning to verify and mechanical resonance shift from the in-plane fundamental mode above the threshold power. At the pump power of 180 μW, the RF spectrum is obtained by sweeping through the cavity TE1,e resonance as the white-colored curve. (b) Mechanical resonant frequency shift and mechanical linewidth versus laser-cavity detuning at the pump power of 180 μW. The light-yellow region indicates the operation position of the pump light for bias voltage detection. (c) RF harmonics of the optomechanical cavity above the threshold, up to the 13th harmonic at 16.7 MHz. The RBW is 100 Hz. (d) Zoom-in view of the spectrum in the red-dashed box of Figure 7(c). The RBW is 1 Hz to characterize the RF spectrum. The green-colored curve is the theoretically calculated thermal noise floor.
Benefiting from the linewidth-narrowing of the mechanical sensing mode, the optomechanical electrometer is driven above the threshold power to track the variation of mechanical resonance frequency shift under various applied bias voltage as shown in Figure 8. Figure 8(a) shows the mechanical resonance spectra of the fundamental in-plane oscillation mode ((in an RBW of 1 Hz) as a function of increasing applied electrical voltage from 0 mV to 120 mV. The inset in Figure 8(a) illustrates three selected peaks of the mechanical resonance spectra under 0 mV (red), 60 mV (black) and 120 mV (blue) to clearly show the ESS effect. Figure 8(b) further highlights a zoom-in view captured from the resonance peak region. Compared to Figure 6(e), a more prominent decreasing resonance shift is observed in Figure 8(b) with a larger frequency shift of 230 Hz due to the ESS effect. Figure 8(c) shows that the extracted peak position of the RF spectra has a quadratic declining trend with the increase of the applied bias voltage, which also agrees well with Eq. (2). Converting the horizontal axis to the square of the applied bias voltage as shown in the inset of Figure 8(c), a linear relation can be fitted with an experimental sensitivity of

Bias voltage detection in the optomechanical electrometer above threshold power.
(a) RF spectra above threshold power tracked for measurement of the applied bias voltage from 0 mV to 120 mV. Inset is the zoom-in view of the resonance peak area to observe the shift of mechanical frequency at 0 mV (red), 60 mV (black) and 120 mV (blue). (b) Zoom-in view of the spectra at the resonance peak area as a function of the applied bias voltages. The black dashed curve indicates the variation of the resonance peaks. (c) Mechanical resonant frequency versus applied bias voltages. Inset is the measured data converted to a linear relationship between resonance shift and applied voltage squared.
Moreover, the RF frequency is measured as a function of time to calculate the Allan deviation to estimate the long-term stability of mechanical resonant frequency, as shown in Figure 9. This is also a significant method to evaluate the performance of the optomechanical electrometer as Allan deviation allows extraction of the detection resolution by investigating the noise and stability from the time-domain data. In the analysis on Allan deviation, of greatest importance for sensing applications are white noise and bias instability. The white noise dominants in the lower integration time and it is highly relevant to thermal effects. Besides, the bias instability indicates the minimum achievable resolution limited by flicker noise contribution and fluctuation on the motion of movable PCN or the optical field. When the optomechanical electrometer works below the threshold, as illustrated in Figure 9(a), the Allan deviation of

Allan deviation
(a) Allan deviation below the threshold (Pin = 30 μW), where the black line is resonant frequency Allan deviation and the red line is converted Allan deviation (=S×σ y (τ)×Ωm/2π) in the term of the square of bias voltage. (b) Allan deviation above the threshold (Pin = 180 μW), where the black line is resonant frequency Allan deviation and the blue line is the converted Allan deviation in the term of the square of bias voltage. Overall, the bias instability (brown dotted line) and white noise (green dotted line) are estimated at the −1/2 slope and zero slopes.
4 Conclusions
In this paper, a nanoscale optomechanical electrometer is experimentally demonstrated using the self-sustained oscillation in cavity optomechanics, for the first time, to enhance the resolution of electric voltage detection. Owing to the strong optomechanical coupling in a zipper cavity, the optical readout of mechanical resonant frequency shift of a movable PCN resonator enables the sensitive detection of bias voltage. Compared to traditional M/NEMS resonant electrometers, this optomechanical electrometer has the following outstanding advantages and improvements: (1) we implement cavity optomechanics to realize a CMOS-compatible electrometer with low noise and high sensing resolution. This optomechanical electrometer demonstrates a significant sensing scheme for electric charge detection in the MOEMS devices, which is superior to traditional M/NEMS sensors considering its sensing performance (see the performance comparison in Supplementary VI). (2) In this optomechanical electrometer, the light pump excites an optical force-driven interaction between the optical cavity and the movable mechanical resonator, and optical readout of mechanical resonant frequency shift allows probing of electrical voltage. Compared with the electronic noises limited M/NEMS resonant electrometers, this all-optical light pump and readout approach could suppress these noises arising from the electrical readout circuits effectively and allow the detection noise level close to the thermal noise limit. (3) Instead of optical readout of resonant wavelength shift, or linewidth and amplitude variation of optical resonance, this optomechanical electrometer employs the RF readout to characterize the performance of the sensor. Benefiting from the strong optomechanical coupling and the dynamic backaction induced amplification (e.g., the self-sustained oscillation), a combination of large
To summarize, we have proposed and investigated an optomechanical electrometer for the first time in this work. When the optomechanical electrometer works below threshold power, an electrical sensitivity of 0.007 Hz/mV2 is obtained with an inadequate resolution of
Funding source: Singapore Ministry of Education
Award Identifier / Grant number: MOE2019-T2-2-104
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Author contribution: All the authors have accepted responsibility for the entire content of this submitted manuscript and approved submission.
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Research funding: This research was funded by the SINGAPORE MINISTRY OF EDUCATION (MOE), grant number MOE2019-T2-2-104.
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Conflict of interest statement: The authors declare no conflicts of interest regarding this article.
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Supplementary Material
The online version of this article offers supplementary material (https://doi.org/10.1515/nanoph-2021-0820).
© 2022 Ji Xia et al., published by De Gruyter, Berlin/Boston
This work is licensed under the Creative Commons Attribution 4.0 International License.
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Articles in the same Issue
- Frontmatter
- Reviews
- Photoactive nanomaterials enabled integrated photo-rechargeable batteries
- Recent progress in terahertz metamaterial modulators
- Research Articles
- Droplet epitaxy symmetric InAs/InP quantum dots for quantum emission in the third telecom window: morphology, optical and electronic properties
- Monolithic dual-wedge prism-based spectroscopic single-molecule localization microscopy
- Four-dimensional multi-particle tracking in living cells based on lifetime imaging
- Orthogonal gap-enhanced Raman tags for interference-free and ultrastable surface-enhanced Raman scattering
- Parallel wave-based analog computing using metagratings
- Gauge-independent emission spectra and quantum correlations in the ultrastrong coupling regime of open system cavity-QED
- Combining one and two photon polymerization for accelerated high performance (3 + 1)D photonic integration
- High power downconversion deep-red emission from Ho3+-doped fiber lasers
- Topological optical parametric oscillation
- Optically tunable split-ring resonators controlled lead sulfide quantum dots modulator for wide THz radiation
- Ultrasensitive nanoscale optomechanical electrometer using photonic crystal cavities
- Negative index metamaterial at ultraviolet range for subwavelength photolithography
- Erratum
- Erratum to: Physics and applications of quantum dot lasers for silicon photonics